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Bulletin of the Russian Academy of Sciences Physics

Nonreciprocity in the Behavior of Photon Echoes inside YLiF4:Er3+ and LuLiF4:Er3+ Crystals in Constant and Pulsed Magnetic Fields

Шегеда Анатолий Михайлович, Кораблева Стелла Леонидовна, Oleg G. Morozov

Published Dec 1, 2024• 1 citation
Publisher

Abstract

Abstract Studies of the effect of nanosecond pulsed magnetic fields have on the behavior of photon echoes in samples of YLiF4:Er3+ and LuLiF4:Er3+ show they depend strongly on the magnitude and direction of a change in the constant magnetic field. An unexpected increase in the intensity of the photon echo is observed when two identical magnetic pulses are switched on, one after the first laser pulse and the second after the second laser pulse.

DOI
10.1134/s1062873824708572

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Abstract A study of the effect of nanosecond pulsed magnetic fields on the behavior of a photon echo in Y(Lu)LiF4:Er3+ samples determined that the action of a pulsed field leads to nonreciprocity and an asymmetric amplification of the photon echo signal. The effect strongly depends on the orientation of the crystals in the external magnetic field and on the orientation of the pulsed magnetic field relative to the direction of the laser pulses.

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We report the first observation and study of the photon echo in Er3+:LuLiF4. The energy transition is 4 I 15/2 → 4 F 9/2 (λ = 6536 Å). The density of ErF3 is 0.025 wt %. The operation temperature is 1.9 K. Measurements were made at low (up to 1200 Oe) and even zero external magnetic fields. We studied the behavior of the photon echo intensity vs. the magnetic field magnitude and direction about the crystal axis C and vs. the laser pulse separation t 12 and observed an exponential growth and then, after a certain plateau, an exponential decrease in the photon echo intensity as a function of magnetic field upon increasing the magnetic field from zero. The parameters describing the exponential growth and decrease are independent of the direction of magnetic field. The value of the magnetic field (∼20–200 Oe) at which the echo intensity is maximal and the value of the maximum itself decrease with increasing pulse separation t 12 and the angle Θ between the magnetic field and crystal axis. The echo intensity decreases exponentially with increasing Θ. The parameter describing the exponential decrease is independent of the magnitude of the field. The echo intensity as a function of pulse separation shows exponential decay. The phase relaxation time depends on the magnitude and direction of the magnetic field. T 2 is equal to 202 ± 16 ns at zero magnetic field. A phenomenological formula is suggested, which qualitatively presents the mentioned dependences, and the polarization properties of the backward photon echo in this crystal are studied. Because the ion of trivalent erbium is an optimum data carrier, the above results show that fine control of the multichannel transfer of processed optical information may be achieved by weak magnetic fields.

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Journal of Physics Conference Series•Oct 1, 2020•0 citations
Abstract Studies of the effect of nanosecond pulsed magnetic fields have on the behavior of photon echoes in samples of YLiF4:Er3+ and LuLiF4:Er3+ show they depend strongly on the magnitude and direction of a change in the constant magnetic field. An unexpected increase in the intensity of the photon echo is observed when two identical magnetic pulses are switched on, one after the first laser pulse and the second after the second laser pulse.
The effect of nanosecond magnetic pulses on a photon echo signal in the Er3+-doped YLiF4 and LuLiF4 samples has been considered. A strong dependence of the photon echo intensity on the parameters of the magnetic pulse and the direction of variation of the external magnetic field H has been found. The application of magnetic pulses can increase the echo intensity by a factor of 5–6. The irreversibility (nonreciprocity) effect is explained by the occurrence of the spatial dispersion of the permittivity.
It is reported about the first observation and studying of the photon echo in LuLiF4:Er3+. The energy transition is 4I15/2→4F9/2 (λ=6536 Å). The density of ErF3 is 0.025 wt%. The operation temperature is 1.9 K. Measurements were spent at low (up to 1200 Oe) and even zero external magnetic fields. It was studied a behavior of the photon echo intensity versus the magnetic field magnitude and direction about the crystal axis C and versus the laser pulse separation t 12. It was observed an exponential growth and then, after some plateau, an exponential decreasing of the photon echo intensity as a function of magnetic field with increasing of the magnetic field from zero value. The parameters describing the exponential growth and decreasing are not depended on direction of magnetic field. Value of a magnetic field at which the echo intensity accepts the maximum, and quantity of this maximum decrease with increased the pulse separation t 12 and the angle θ between the magnetic field and crystal axis. The echo intensity exponentially decreases with increased θ. The parameter describing the exponential decreasing is not depended on the magnitude of the field. The echo intensity as a function of pulse separation shows exponential decay. The phase relaxation time is depended on the magnitude and direction of the magnetic field. T 2 is equal to 202±16 ns at zero magnetic field. Phenomenological formula is suggested, which qualitatively presents the mentioned dependencies. Polarization properties of the backward photon echo in this crystal are studied also.
We report the first observation and study of the photon echo in Er3+:LuLiF4. The energy transition is 4 I 15/2 → 4 F 9/2 (λ = 6536 Å). The density of ErF3 is 0.025 wt %. The operation temperature is 1.9 K. Measurements were made at low (up to 1200 Oe) and even zero external magnetic fields. We studied the behavior of the photon echo intensity vs. the magnetic field magnitude and direction about the crystal axis C and vs. the laser pulse separation t 12 and observed an exponential growth and then, after a certain plateau, an exponential decrease in the photon echo intensity as a function of magnetic field upon increasing the magnetic field from zero. The parameters describing the exponential growth and decrease are independent of the direction of magnetic field. The value of the magnetic field (∼20–200 Oe) at which the echo intensity is maximal and the value of the maximum itself decrease with increasing pulse separation t 12 and the angle Θ between the magnetic field and crystal axis. The echo intensity decreases exponentially with increasing Θ. The parameter describing the exponential decrease is independent of the magnitude of the field. The echo intensity as a function of pulse separation shows exponential decay. The phase relaxation time depends on the magnitude and direction of the magnetic field. T 2 is equal to 202 ± 16 ns at zero magnetic field. A phenomenological formula is suggested, which qualitatively presents the mentioned dependences, and the polarization properties of the backward photon echo in this crystal are studied. Because the ion of trivalent erbium is an optimum data carrier, the above results show that fine control of the multichannel transfer of processed optical information may be achieved by weak magnetic fields.