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Soviet Journal of Low Temperature Physics

Nonlinear spin wave theory for ferromagnetic chains with uniaxial anisotropy of the easy plane type

Andrey V. Chubukov

Published Nov 1, 1984• 0 citations
Publisher

Abstract

We consider the determination of the ground state energy and the lowest lying excitations for ferromagnetic Heisenberg spin chains with uniaxial anisotropy of the “easy plane” type in an external magnetic field directly along the anisotropy axis. The ratio of the anisotropy and exchange constants (α) is assumed small, but the size of the site spin S is arbitrary. To first order in α the exact results are shown to differ from the quasiclassical results only by the substitution α→α˜=α[1−(1/2)S]. The asymptotic behavior of the transverse spin correlation function is discussed, and a comparison is made between the theoretical results and recent experiment data.

DOI
10.1063/10.0031204

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Journal of the Physical Society of Japan•Oct 15, 1996•138 citations
We consider the determination of the ground state energy and the lowest lying excitations for ferromagnetic Heisenberg spin chains with uniaxial anisotropy of the “easy plane” type in an external magnetic field directly along the anisotropy axis. The ratio of the anisotropy and exchange constants (α) is assumed small, but the size of the site spin S is arbitrary. To first order in α the exact results are shown to differ from the quasiclassical results only by the substitution α→α˜=α[1−(1/2)S]. The asymptotic behavior of the transverse spin correlation function is discussed, and a comparison is made between the theoretical results and recent experiment data.
A variational estimate of the free energy of a quantum spin chain based on the stochastic behavior of the quantization axes is proposed. It allows a description of the nonlinear excitations and quantum spin waves within the same framework. For an easy-plane ferromagnet with an external field in the plane it reveals that the nonlinear excitations (solitons) are predominantly described by the classical degrees of freedom. Considerable effort has been devoted to the theoretical description1 and experimental verification of the existence of nonlinear excitations. In this field magnetic chain systems have played an important part.2 Chain systems with an easy-plane anisotropy, such as (C6 H11 NH3 )CuBr3 (CHAB) and CsNiF3 , which are subjected to a symmetry breaking field, were found to be soliton bearing.3 Theoretically the description of the nonlinear effect is based on the mapping of the spin dynamics on a sine-Gordon model. Further research4 indicated that the interpretation of the thermodynamical properties of real systems in terms of the sine-Gordon model required however quantum and anisotropy corrections. Since the dipolar interactions between the spins in the chain are considered to be negligible, the direction of the spin chain in configuration space with respect to any preferred direction in spin space does not enter explicitly in the Hamiltonian. This makes it interesting to define a site-dependent z direction in spin space which makes an angle (Θn ,φn ) with the z direction in configuration space. The model Hamiltonian can then be written in terms of the spin operators defined with respect to the site-dependent quantization axis. The representation with equal quantization axis for all the sites is related to the representation with different quantization axes at each site by a rotation in spin space. The unitary transformation that describes the rotation contains the angles (Θn ,φn ), which we have treated as random variables. Based on this observation we have proposed a new variational approach for the quantum spin chain. We will outline the main results here. A full account is published elsewhere.5 In our approach the free energy of the system can be separated in a quantum part and a classical part. The free energy F of the chain is then approximated by an upper bound F<Fcl +Fqm , where βFcl =−ln[E(exp−βVcl )] and βFqm =−ln Tr(exp−β〈Hqm 〉). The first part is a configurational classical free energy, depending on the choice of the probability distribution for the quantization axes via the expectation E. The second contribution is the free energy of a modified quantum chain, whose parameters are classical averages and can be obtained from the configurational classical free energy. For easy-plane ferromagnetic chains, the nonlinear excitations are comprised in the classical part, whereas the quantum part contains predominantly linear excitations. For those thermodynamical quantities that are insensitive to the contribution of the quantum excitations, the chain is thermodynamically equivalent with a classical sine-Gordon system. The out-of-plane corrections are incorporated in the quantum part of the free energy. This behavior is corroborated experimentally by measurements of the excess heat capacity of CHAB for different magnetic fields with the same in-plane component.6 The validity of our approach is, however, not restricted to easy-plane ferromagnetic chains. Also for more complex systems with, for example, an orthorhombic or helical symmetry, the introduction of stochastic quantization axes can shed new light on some of the thermodynamical properties of these quantum systems in terms of their classical equivalent.
This article presents the results of studies of the linear antiferromagnetic spin chain with uniaxial anisotropy (XXZ– model) placed in a transverse magnetic field directed along the anisotropy axis of the chain with a constant gradient along the chain. A spin Hamiltonian for the states close to the ground was written in the spin-wave approximation. It was diagonalized by an asymptotic expansion in the small parameter describing the magnitude of the field gradient. Local energy of the ground state and the reduced density matrix of the quantum states for a selected pair of spins in the chain have been considered in the gapped and gapless cases. Local spin polarization and the local toroidal magnetic moment have also been found. Local pair entanglement of quantum states as a characteristic of quantum correlations in the spin chain was studied.
We investigate ground-state and low-lying excited states of the S = 1 antiferromagnetic Heisenberg chain with exchange anisotropy, single-ion anisotropy and biquadratic exchange and with free boundary conditions. We present an approximate mapping of the S = 1 model to an effective S = 1/2 chain in an external magnetic field, which can be solved exactly in several limiting cases. We obtain results for the phase diagram, correlation functions and the excitation spectrum. The transition to the Haldane phase is related to the condensation of the lowest soliton modes and the hidden order parameter of the Haldane phase is identified as transverse long-range order in the effective S = 1/2 chain.
The exact analytical forms of the low-temperature thermodynamic quantities and correlation functions are obtained for classical one-dimensional Heisenberg ferromagnets with single-site anisotropy including both the systems with an easy axis and with an easy plane. The problem has been managed on the basis of the functional integral method. The calculated results have a few leading terms in series-expansion with respect to the reduced temperature, exhibiting the characteristic points borne out in the recent numerical studies. In particular, the longitudinal correlation function and susceptibility of the system with an easy axis show Ising-like behaviours and the transverse counterparts of the system with an easy plane show isotropic XY- or Heisenberg-like behaviours. Physical implications of the calculated results are also discussed.
Ground-state properties of the spin-1 antiferromagnetic Heisenberg chain with bond alternation and uniaxial single-ion-type anisotropy, which is described by the Hamiltonian \({\cal H}_0 = \sum_{\ell=1}^N\{1-(-1)^\ell\alpha\}{\mib S}_\ell\cdot{\mib S}_{\ell+1} + D\sum_{\ell=1}^N\;(S_\ell^z)^2\) (0.0 ≤α≤1.0, -∞< D < ∞), are studied. An exact diagonalization method by means of the Lanczös technique is used. The ground-state phase diagram on the α versus D plane at the thermodynamic limit is determined by analyzing the Binder parameters associated with Néel order and z -direction string order for finite-size ( N = 6, 8, …, 16) chains. It is found that there exists a multicritical point at which the Haldane, Néel, and singlet-dimer phases meet and that the singlet-dimer phase and the large- D phase belong to the same unique phase. The ground-state magnetization curves at the thermodynamic limit for various values of α and D are obtained for the system described by the Hamiltonian, H 0 plus the Zeeman term - H ∑ ℓ=1 N S ℓ z . The results show that the 1/2-plateau appears in the magnetization curve at least when D ≥0.0 and 0.0≲α≤1.00.0\lesssim\alpha \leq 1.00.0≲α≤1.0.