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Electronics

Double Resonance of Electromagnetically Induced Transparency of Rydberg Atom in Counter-Propagating Configuration

Chao Li, Ma Guo, Mingwei Lei, Meng Shi

Published Nov 8, 2024• 4 citations
Publisher

Abstract

The double resonance phenomenon of EIT is studied through the ladder three-level Rydberg system. A probe laser with the wavelength λp=852.35 nm is used to coupling the ground state 6S1/2 to the middle state 6P3/2, and a coupling laser with the wavelength λc=509.08 nm is implemented to couple the state 6P3/2 to the Rydberg state 62D5/2. A special optical scheme is designed, in which the co-propagating and counter-propagating configurations are both used. As a result, the double resonance of electromagnetically induced transparency (EIT) with the Rydberg atom is observed. By comparing the distance between the double peaks, it is found that the double resonance phenomenon comes from the Doppler effect, and the distance between the two resonance peaks in the absorption spectrum is related to the detuning of the resonant lasers.

DOI
10.3390/electronics13224391

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arXiv:1403.5724•Physical Review A•Oct 9, 2014•12 citations
The double resonance phenomenon of EIT is studied through the ladder three-level Rydberg system. A probe laser with the wavelength λp=852.35 nm is used to coupling the ground state 6S1/2 to the middle state 6P3/2, and a coupling laser with the wavelength λc=509.08 nm is implemented to couple the state 6P3/2 to the Rydberg state 62D5/2. A special optical scheme is designed, in which the co-propagating and counter-propagating configurations are both used. As a result, the double resonance of electromagnetically induced transparency (EIT) with the Rydberg atom is observed. By comparing the distance between the double peaks, it is found that the double resonance phenomenon comes from the Doppler effect, and the distance between the two resonance peaks in the absorption spectrum is related to the detuning of the resonant lasers.
Abstract The double resonance phenomenon of electromagnetically induced transparency (EIT) in a ladder-type Rydberg atomic system is theoretically investigated. Based on the cesium 6 S 1 / 2 → 6 P 3 / 2 → n D 5 / 2 transition, we establish a density-matrix model incorporating the Doppler effect and simulate the absorption spectra under counter-propagating laser configurations. The numerical approach is adopted: a two-velocity-group approximation (Lorentzian line-shape superposition). The results show that when the probe detuning Δ p is fixed and nonzero, scanning the coupling laser frequency yields two symmetric transparency peaks separated by δ = 2 ( λ p / λ c ) | Δ p | , in excellent agreement with recent experimental observations. The two-velocity-group approximation is computationally efficient and physically transparent, while the high-precision integration confirms its validity. We also reveal that conventional uniform velocity averaging fails to resolve the narrow EIT peaks due to insufficient sampling, and propose effective numerical strategies. This work provides a reliable theoretical tool for simulating Rydberg EIT spectra and offers insights into Doppler-induced double resonance, which may find applications in laser frequency stabilization and self-calibration of Rydberg atom-based sensors.
Rydberg atoms, with large principal quantum number n, have been widely investigated in recent years due to their peculiar properties, such as big sizes, long lifetimes and strong interactions with fields and other Rydberg atoms. Rydberg atoms are very sensitive to external fields due to their large polarizabilities scaling as n7.These make Rydberg atoms an ideal candidate for the quantum information, the many-body interaction, etc.In this work, we investigate the Rydberg atoms using electromagneticlly induced transparency (EIT) in a ladder three-level system. The EIT is a quantum interference effect between two excitation path-ways driven by two laser fields. The main idea is performed in a room temperature cesium vapor cell, where the probe laser frequency is modulated. The ground state (6P1/2), excited state (6P3/2), and Rydberg state (nS1/2) constitute a Rydberg three-level system, in which the probe laser is fixed to the 6S1/2 (F = 4)6P3/2 (F = 5) transition by saturated absorption spectrum technique, whereas the coupling laser is scanned across the 6P3/249S1/2 transition. We detect the demodulated EIT signal with the lock-in amplifier (SR830). The modulated EIT signal shows a two-peak structure. The measured spacing between two peaks increases with the frequency detuning, caused by the modulation amplitude, and half the spacing between the peak-to-peak is nearly 1.67 times the modulation amplitude of the probe laser; the measured result shows that the splitting is independent of the modulation frequency. The experimental results are in agreement with the theoretical calculations. The results in our work can be used for real-time monitoring of the laser-line profiles and the fluctuation of laser frequency.
Rydberg atoms, with large principal quantum number, exhibit certain properties, such as long lifetimes and strong interactions with fields and other atoms, which have been extensively investigated recently. One of the properties is the electromagnetically induced transparency (EIT) of Rydberg ladder system, which can be used to measure the radio frequency (RF) field with high sensitivity. In this paper, we investigate the quantum coherent effect of cesium Rydberg atom in a three-level ladder system involving the ground state (6S1/2), the excited state (6P3/2) and 49S1/2 Rydberg state in room temperature vapor cell. The probe laser (852 nm) drives the transition of 6S1/2(F=4)→6P3/2(F'=5), while the coupling laser (510 nm) couples the Rydberg transition of 6P3/2 (F'=5)→nS1/2. A typical electromagnetically induced transparency spectrum is obtained when the weak probe laser is scanned through the transition of 6S1/2(F=4)→6P3/2(F'=5) and the coupling laser tuning to Rydberg transition. The two-photon RF spectra are observed when the RF field with a frequency of ~16.9 GHz couples the Rydberg transition of 49S1/2→47D3/2, where the EIT signal is split into two EIT peaks due to the interaction between the RF field and Rydberg atoms. The dependences of EIT splitting on the power of RF field are investigated. The results show that the EIT splitting increases with the power of RF field, which can inversely be used to measure the RF field with a higher spatial resolution in the future.
In a Doppler-broadened ladder-type Rubidium atomic system [Formula: see text]–[Formula: see text]–[Formula: see text], three-photon electromagnetically induced absorption (EIA) and transparency (EIT) in two schemes of two coupling lasers with different propagation directions are comprehensively studied. Two coupling fields are entangled tightly with each other and induce constructive interference such that we observe EIA as two coupling fields are counter-propagating. Two coupling fields are independent and cause destructive interference such that only enhanced EIT occurs when two coupling fields are co-propagating, although all of the Doppler-broadened atoms satisfy the condition for three-photon resonance. The experimental results are coincided with the numerically calculated spectra using the dressed perturbation method. The mechanisms of EIT and EIA could also be understood by the dressed-state pictures.
Rydberg atoms are highly excited atoms with large principal quantum number n, big sizes (~n2) and long lifetimes (~n3). Rydberg atoms are very sensitive to an external field due to the large polarizabilities of Rydberg atoms (~n7). Electromagnetically induced transparency (EIT) of Rydberg atom provides an ideal method to detect Rydberg atoms without destroying atoms, and can be used to measure the external direct current and radio frequency (RF) field. In this paper, we study the EIT effect of a cesium ladder-type three-level atom involving Rydberg state exposed to a weak RF field. The ground state (6S1/2), the excited state (6P3/2) and Rydberg state (48D5/2) constitute the Rydberg three-level system, in which the probe laser couples 6S1/2(F=4)6P3/2(F'=5) transition, whereas the coupling laser scans across the 6P3/248D5/2 Rydberg transition. The coupling laser (510 nm laser, propagating in the z-axis direction and linear polarization in the y-axis direction) and the probe laser (852 nm laser, linear polarization in the y-axis direction) counter-propagate through a 50-mm-long cesium vapor cell at room temperature, yielding Rydberg EIT spectra. Rydberg EIT signal is detected as a function of the detuning of the coupling laser. When a weak RF (80 MHz) electric field polarized in the x-axis direction is applied to a pair of electrode plates located on both sides of the cesium cell, the EIT spectrum of Rydberg 48D5/2 shows the Stark splitting and the even order harmonic sidebands. The experimental results are analyzed by using the Floquet theory. The simulation results accord well with the experimentally measured results. Furthermore, we also investigate the influence of the self-ionization effect of Rydberg atom on the Stark spectrum by changing the RF frequency. We put forward a proposal to avoid the effect of ionization by placing electrode plates in the cesium cell. In the weak RF-field domain, mj=5/2 Stark line crosses mj=1/2, 3/2 sidebands, these cross points provide an antenna-free method of accurately calibrating the RF electric field based on Rydberg atoms.
We study the electromagnetically induced transparency (EIT) effect with two individually addressed four-level Rydberg atoms subjected to the interatomic van der Waals interaction. We derive an effectively atomic Raman transition model where two ladders of the usual Rydberg EIT setting terminating at the same upper Rydberg level of long radiative lifetime are turned into a Rydberg EIT $\ensuremath{\lambda}$ setup via two-photon transitions, leaving the middle levels of each ladder largely detuned from the coupling and probe laser beams. It can hence overcome the limits of applications for EIT with atoms of the ladder-type level configuration involving a strongly decaying intermediate state by inducing coherence between two ground states. By probing one of the atoms, we observe four doublets of absorption induced by the Autler-Townes splitting and the van der Waals interaction. In particular, we find that the location of the EIT center remains unchanged compared to the interatomic-interaction-free case, which demonstrates that the interference among the multiple transition channels is basically destructive. The EIT with controlled Rydberg-Rydberg interaction among a few atoms provides a versatile tool for engineering the propagation dynamics of light.