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Journal of Experimental and Theoretical Physics Letters

Ramsey Spectroscopy of CPT Resonances on the D1 Line of Alkali Metal Atoms in Miniature Cells in the Field of Counterpropagating Waves with Opposite Circular Polarizations

Valeriy I. Yudin, M. Yu. Basalaev, Daba A. Radnatarov, Ivan Gromov, M. D. Radchenko, Sergey M Kobtsev, A. V. Taǐchenachev

Published Oct 1, 2024• 0 citations
Publisher

Abstract

In this study, the Ramsey spectroscopy of coherent population trapping resonances excited on the D1 line of alkali metal atoms in miniature vapor cells has been studied theoretically and experimentally. The configuration of the field produced by two counterpropagating waves with opposite circular polarizations has been considered. A counterpropagating wave is formed as a result of reflection from a partially transmitting output mirror, while the signal from the initial wave transmitted through the mirror is detected. It is shown that such a scheme is characterized by the optimal mirror reflection coefficient, for which the short-term stability can be substantially improved relative to the standard scheme without the counterpropagating wave. The three-fold improvement of the short-term stability of the atomic clock based on the coherent population trapping resonance in a vapor cell with 87Rb atoms has been demonstrated experimentally.

DOI
10.1134/s0021364024603130

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In this study, the Ramsey spectroscopy of coherent population trapping resonances excited on the D1 line of alkali metal atoms in miniature vapor cells has been studied theoretically and experimentally. The configuration of the field produced by two counterpropagating waves with opposite circular polarizations has been considered. A counterpropagating wave is formed as a result of reflection from a partially transmitting output mirror, while the signal from the initial wave transmitted through the mirror is detected. It is shown that such a scheme is characterized by the optimal mirror reflection coefficient, for which the short-term stability can be substantially improved relative to the standard scheme without the counterpropagating wave. The three-fold improvement of the short-term stability of the atomic clock based on the coherent population trapping resonance in a vapor cell with 87Rb atoms has been demonstrated experimentally.
State-of-the-art miniature atomic clocks (MACs) are based on the phenomenon of coherent population trapping (CPT) in alkali-metal atomic vapors (Rb\mathrm{Rb}Rb or Cs\mathrm{Cs}Cs). Improving the stability of the clock frequency is a crucial issue; resolving it would result in significant progress in numerous applications. Here, we examine the configuration of the light field, which is composed of two bichromatic beams with opposing handedness of circular polarization. The beams are in resonance with optical transitions in the Cs\mathrm{Cs}Cs D1{D}_{1}D1​ line ($\ensuremath{\lambda}\ensuremath{\approx}895$ nm). This configuration has previously been shown to produce observed CPT resonances with higher contrast than a standard single-beam scheme; however, our scheme implements pump and probe beams that operate independently, with the transmission of the probe beam being monitored separately. This approach differs from previous studies. The experiments are carried out using a cubic $5\ifmmode\times\else\texttimes\fi{}5\ifmmode\times\else\texttimes\fi{}5\phantom{\rule{0.2em}{0ex}}{\mathrm{mm}}^{3}$ vapor cell filled with buffer gas. It is shown that the line shape of the resonance acquires an asymmetry that can be efficiently controlled by a microwave (Raman) phase between the beams. As a proof of concept, we study the way in which this asymmetry can help to mitigate the influence of the ac Stark (light) shift on the long-term frequency stability of CPT clocks based on vapor microcells ($V\ensuremath{\ll}1\phantom{\rule{0.2em}{0ex}}{\mathrm{cm}}^{3}$). Experimental verification is performed with both a distributed-Bragg-reflector laser and a vertical-cavity surface-emitting laser. The latter is of particular importance for the development of MACs. The experimental results are in qualitative agreement with the analytical theory based on a double-$\mathrm{\ensuremath{\Lambda}}$ scheme of atomic energy levels.
We present a joint theoretical and experimental characterization of the coherent population trapping (CPT) resonance excited on the D1{D}_{1}D1​ line of 87Rb^{87}\mathrm{Rb}87Rb atoms by bichromatic linearly polarized laser light. We observe high-contrast transmission resonances (up to $\ensuremath{\approx}25%$), which makes this excitation scheme promising for miniature all-optical atomic clock applications. We also demonstrate cancellation of the first-order light shift by proper choice of the frequencies and relative intensities of the two laser-field components. Our theoretical predictions are in good agreement with the experimental results.
We present preliminary results showing that some noise sources in vapor cell atomic clocks based on coherent population trapping (CPT) can be suppressed with differential detection. The scheme we propose differs from more conventional differential detection in that both optical fields pass through the alkali vapor cell but have different polarizations, one circular and one linear. Because CPT resonances are only excited by the circularly polarized beam, the linearly polarized beam can be used to reduce several important sources of noise. With this technique, we demonstrate reduction of the short-term frequency instability of a CPT atomic frequency reference by a factor of about 1.5.
A gas cell atomic frequency standard based on coherent population trapping (CPT) with Ramsey interrogation pulses is developed. The clock resonance is detected in a Cs cell with buffer gas using two phase-locked diode lasers tuned to the D1 line. A preliminary short-term stability of3.5×10−12t−1/23.5 \times 10^{-12}t^{-1/2}3.5×10−12t−1/2is reported. The CPT specificity allows a new interrogation–detection sequence, i.e., the continuous pulse train, which, with phase modulation, could lead to better short-term stability compared to usual continuous CPT clocks. The parameters optimizing the stability include a high Rabi frequency, a very short measurement time, and an interrogation time equal to the lifetime of the hyperfine coherence.
In this paper we present our spectroscopic studies on Coherent Population Trapping (CPT) in micro-fabricated Caesium cells and our evaluation of its application in miniature atomic frequency standards (atomic clocks). We observe the CPT signal on the Cs D1-line by coupling two hyperfine ground-state Zeeman sub-levels to a common excited state using two coherent electromagnetic fields created with a modulated DFB laser. Contrarily to double resonance, CPT does not require any microwave cavity, which should facilitate the miniaturization of a future atomic clock device. We study and report here on the light shift phenomena at different cell temperatures and laser wavelength. We also present resonance shifts due to cell temperature variations and clock frequency stability measurements. To the best of our knowledge, this article is the first report on light shift with Cs D1 line in a CPT vapour-cell atomic clock.
We present a prospective experimental study on double-resonance Ramsey spectroscopy in a micro fabricated Rb vapor cell, in view of future miniature atomic clocks with improved stability performance. Ramsey signals with a narrow central fringe width of 1.5 kHz combined with a competitive contrast of > 5 % are observed, resulting in a clock short-term stability of ≈ 1×10-11τ−1/2. The employed pulsed optical pumping (POP) scheme bears promise for reduced light-shift effects and thus for improved clock stability on medium- to long-term timescales.