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Nature Communications

Higher-order and fractional discrete time crystals in Floquet-driven Rydberg atoms

Bang Liu, Li-Hua Zhang, Qifeng Wang, Yu Ma, Tian-Yu Han, Jun Zhang, Zhengyuan Zhang, Shi-Yao Shao, Qing 'an Li, Han-Chao Chen, Bao-Sen Shi, Dong-Sheng Ding

Published Nov 10, 2024• 37 citations
Publisher

Abstract

Higher-order and fractional discrete time crystals (DTCs) are exotic phases of matter where the discrete time translation symmetry is broken into higher-order and non-integer category. Generation of these unique DTCs has been widely studied theoretically in different systems. However, no current experimental methods can probe these higher-order and fractional DTCs in any quantum many-body systems. We demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases. We have discovered multiple n-DTCs with integer values of n = 2, 3, and 4, and others ranging up to 14, along with fractional n-DTCs with n values beyond the integers. The system response can transition between adjacent integer DTCs, during which the fractional DTCs are investigated. Study of higher-order and fractional DTCs expands fundamental knowledge of non-equilibrium dynamics and is promising for discovery of more complex temporal symmetries beyond the single discrete time translation symmetry. Discrete-time crystal (DTC) is a special phase of matter that exhibits a spontaneous breaking of the discrete time translational symmetry. Here, Bang Liu et al. demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases.

DOI
10.1038/s41467-024-53712-5

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Higher-order and fractional discrete time crystals (DTCs) are exotic phases of matter where the discrete time translation symmetry is broken into higher-order and non-integer category. Generation of these unique DTCs has been widely studied theoretically in different systems. However, no current experimental methods can probe these higher-order and fractional DTCs in any quantum many-body systems. We demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases. We have discovered multiple n-DTCs with integer values of n = 2, 3, and 4, and others ranging up to 14, along with fractional n-DTCs with n values beyond the integers. The system response can transition between adjacent integer DTCs, during which the fractional DTCs are investigated. Study of higher-order and fractional DTCs expands fundamental knowledge of non-equilibrium dynamics and is promising for discovery of more complex temporal symmetries beyond the single discrete time translation symmetry. Discrete-time crystal (DTC) is a special phase of matter that exhibits a spontaneous breaking of the discrete time translational symmetry. Here, Bang Liu et al. demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases.
Higher-order and fractional discrete time crystals (DTCs) are exotic phases of matter where the discrete time translation symmetry is broken into higher-order and non-integer category. Generation of these unique DTCs has been widely studied theoretically in different systems. However, no current experimental methods can probe these higher-order and fractional DTCs in any quantum many-body systems. We demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases. We have discovered multiple nnn-DTCs with integer values of nnn = 2, 3, and 4, and others ranging up to 14, along with fractional nnn-DTCs with nnn values beyond the integers. The system response can transition between adjacent integer DTCs, during which the fractional DTCs are investigated. Study of higher-order and fractional DTCs expands fundamental knowledge of non-equilibrium dynamics and is promising for discovery of more complex temporal symmetries beyond the single discrete time translation symmetry.
Discrete time quasicrystals (DTQC) constitute a class of non-equilibrium matter characterized by temporal order without strict periodicity, in contrast to conventional time crystals. Investigating these phenomena is essential for expanding our fundamental understanding of far-from-equilibrium quantum matter and spontaneous symmetry breaking beyond periodic regimes. Here, we experimentally observe a DTQC in a driven-dissipative ensemble of strongly interacting Rydberg atoms, displaying non-equilibrium dynamical response with a different finite Abelian group symmetry Zm×Zn{{\mathbb{Z}}}_{m}\times {{\mathbb{Z}}}_{n}Zm​×Zn​. By applying a quasiperiodic drive using a dual-frequency drive with incommensurate frequencies, we demonstrate that the system exhibits a robust subharmonic response at multiple incommensurate frequencies, signifying the emergence of a DTQC phase. We map the full phase diagram of the system, which includes the DTQC phase, and demonstrate its rigidity against perturbations in both RF field intensity and laser detuning. Moreover, we observe a cyclic group symmetry effect that constrains the construction of Z2×Z3{{\mathbb{Z}}}_{2}\times {{\mathbb{Z}}}_{3}Z2​×Z3​-symmetric DTQC. This work establishes a versatile platform for studying non-equilibrium phases of matter and provides insights into the dynamics of time-translation symmetry breaking in quantum many-body systems. Time-crystal phases have raised both theoretical and experimental interest across various platforms. Here, the authors report the observation of a discrete time-quasicrystal in a driven-dissipative ensemble of interacting Rydberg atoms, advancing the understanding of symmetry breaking in these systems.
Discrete time crystals (DTCs) are non-equilibrium phases in periodically driven systems that exhibit spontaneous breaking of discrete time-translation symmetry. The stabilization of most DTC phases is achieved via the disorder-induced many-body localization. In this work, we propose an experimental scheme to realize disorder-free DTCs in a periodically driven Rydberg atom array. Our scheme utilizes a linear potential in the atomic detuning to enhance the DTC order, without being tired to (Stark) many-body localization. We numerically demonstrate that the Stark potential enhances the robustness of the DTC against the flip imperfections and extends its lifetime, which are independent of initial states. Thus, our scheme provides a promising way to explore DTCs in Rydberg atom arrays without disorder averaging and special state preparation.
Discrete time crystals (DTCs) are non-equilibrium phases of matter that break the discrete time-translation symmetry and is characterized by a robust subharmonic response in periodically driven quantum systems. Here, we explore the DTC in a disorder-free, periodically kicked XXZ spin chain, which is stabilized by the Floquet strong Hilbert space fragmentation. We numerically show the period-doubling response of the conventional DTC order, and uncover a multiple-period response with beating dynamics due to the coherent interplay of multiple πππ-pairs in the Floquet spectrum of small-size systems. The lifetime of the DTC order exhibits independence of the driving frequency and a power-law dependence on the ZZ interaction strength. It also grows exponentially with the system size, as a hallmark of the strong fragmentation inherent to the Floquet model. We analytically reveal the approximate conservation of the magnetization and domain-wall number in the Floquet operator for the emergent strong fragmentation, which is consistent with numerical results of the dimensionality ratio of symmetry subspaces. The rigidity and phase regime of the DTC order are identified through finite-size scaling of the Floquet-spectrum-averaged mutual information, as well as via dynamical probes. Our work establishes the Floquet Hilbert space fragmentation as a disorder-free mechanism for sustaining nontrivial temporal orders in out-of-equilibrium quantum many-body systems.
A time crystal is an exotic phase of matter where time-translational symmetry is broken; this phase differs from the spatial symmetry breaking induced in crystals in space. Lots of experiments report the transition from a thermal equilibrium phase to time crystal phase. However, there is no experimental method to probe the bifurcation effect of distinct time crystals in quantum many-body systems. Here, in a driven and dissipative many-body Rydberg atom system, we observe multiple continuous dissipative time crystals and emergence of more complex temporal symmetries beyond the single time crystal phase. Bifurcation of time crystals in strongly interacting Rydberg atoms is observed; the process manifests as a transition from a time crystal state of long temporal order to one of short temporal order, or vice versa. By manipulating the driving field parameters, we observe the time crystal's bistability and a hysteresis loop. These investigations indicate new possibilities for control and manipulation of the temporal symmetries of non-equilibrium systems.
A time crystal is an exotic phase of matter where time-translational symmetry is broken; this phase differs from the spatial symmetry breaking induced in conventional crystals. Lots of experiments report the transition from a thermal equilibrium phase to a time crystal phase. However, there is no experimental method to probe the bifurcation effect of distinct continuous time crystals in quantum many-body systems. Here, in a driven and dissipative many-body Rydberg atom system, we observe multiple continuous dissipative time crystals and emergence of more complex temporal symmetries beyond the single time crystal phase. Bifurcation of time crystals in strongly interacting Rydberg atoms is observed; the process manifests as a transition from a time crystal of long periodicity to a time crystal of short periodicity, or vice versa. By manipulating the driving field parameters, we observe the time crystal’s bistability and a hysteresis loop. These investigations indicate new possibilities for control and manipulation of the temporal symmetries of non-equilibrium systems. The time crystal is an exotic phase of matter where time-translational symmetry is broken. Here, the authors observe multiple continuous dissipative time crystals and bifurcation of time crystals in driven and dissipative Rydberg atomic gas.