In waveguide quantum electrodynamics (QED) systems, noninteracting quantum entities can be coupled through the vacuum field of the waveguide, leading to both coherent and dissipative interactions. We systematically demonstrate that the reflection spectrum is clear and direct in representing the collective interaction using the mirror reflection properties of semi-infinite waveguides. Due to the destructive interference with its mirror image, the emitter is decoupled from the waveguide, suppressing the decay so that the reflection spectrum shows an anticrossing phenomenon induced by coherent interaction. Moreover, the reflection spectrum of an anti-parity-time symmetric Hamiltonian caused by dissipative coupling exhibits an unconventional splitting characterized by level attraction transitioning at exceptional points. Our findings highlight the significance of exploring non-Hermitian effects in waveguide quantum systems, offering potential applications in quantum networks reliant on long-distance interactions. Published by the American Physical Society 2024
In waveguide quantum electrodynamics (QED) systems, noninteracting quantum entities can be coupled through the vacuum field of the waveguide, leading to both coherent and dissipative interactions. We systematically demonstrate that the reflection spectrum is clear and direct in representing the collective interaction using the mirror reflection properties of semi-infinite waveguides. Due to the destructive interference with its mirror image, the emitter is decoupled from the waveguide, suppressing the decay so that the reflection spectrum shows an anticrossing phenomenon induced by coherent interaction. Moreover, the reflection spectrum of an anti-parity-time symmetric Hamiltonian caused by dissipative coupling exhibits an unconventional splitting characterized by level attraction transitioning at exceptional points. Our findings highlight the significance of exploring non-Hermitian effects in waveguide quantum systems, offering potential applications in quantum networks reliant on long-distance interactions. Published by the American Physical Society 2024
Dissipative light-matter coupling plays a vital role in non-Hermitian physics, but it remains largely unexplored in waveguide QED systems. In this work, we find that by employing pseudo-Hermitian symmetry rather than anti- PT symmetry, the concept of dissipative coupling could be generalized and applied to the field of waveguide QED. This leads to a series of intriguing results, such as spontaneous breaking of pseudo-Hermitian symmetry across the exceptional points (EPs), level attraction between the bound states, and critical transition across the EPs for the population of quantum emitters in the bound state. Thanks to the tunability of photonic bands in crystal waveguides, we also demonstrate that dissipative light-matter coupling leads to the emergence of nonstandard third-order exceptional points with chiral spatial profiles in a topological waveguide QED system. This work provides a promising paradigm for studying non-Hermitian quantum phenomena in waveguide QED systems.
Spontaneous emission of a quantum emitter, such as an excited atom, is a fundamental process in quantum electrodynamics (QED), typically associated with exponential decay to the ground state accompanied by irreversible photon emission. This simple Markovian picture, however, is profoundly modified in the presence of time-delayed feedback, structured continua, or cooperative emission, as occurs when an emitter radiates in front of a mirror, when several emitters radiate collectively, or in the case of a giant atom. In such regimes, strong non-Markovian dynamics arise from photon reabsorption and interference effects, leading to pronounced deviations from exponential decay. Here we demonstrate the emergence of exceptional points (EPs) in these highly non-Markovian waveguide-QED environments, i.e., non-Markovian EPs. These EPs appear directly in the relaxation dynamics as sharp transitions to oscillatory behavior, manifested by the appearance of real zeros in the excited-state amplitude. We analyze in detail the spontaneous emission of giant atoms with two or more coupling points, highlighting the mechanisms leading to non-Markovian EPs, and show that similar phenomena arise in other waveguide-QED settings, such as the collective spontaneous emission of spatially separated point-like emitters. Our results reveal waveguide-QED systems as experimentally accessible platforms for realizing and exploring non-Markovian EP physics.
Waveguide quantum electrodynamics constitutes a modern paradigm for the interaction of light and matter, in which strong coupling, bath structure, and propagation delays can break the radiative conditions that quantum emitters typically encounter in free space. These characteristics intertwine the excitations of quantum emitters and guided radiation modes to form complex multiphoton dynamics. So far, combining the collective decay of the emitters with the non-Markovian effects induced by the modes has escaped a full solution and the detailed physics behind these systems remains unknown. Here we analyze such a collective non-Markovian decay in a minimal system of two excited emitters coupled to a one-dimensional single-band waveguide. We develop an exact solution for this system in terms of elementary functions that unveils hidden symmetries and predicts new forms of spontaneous decay. The collective non-Markovian dynamics, which are strongly dependent on the vacuum coupling and the detuning from the center of the band, show exotic features that can be characterized with a simple and readily available criterion. Our analytic methods shed light on the complexity of collective light-matter interactions and open up a pathway for understanding multiparticle open quantum systems. Published by the American Physical Society 2024
We study two-level systems (2LS) coupled at different points to a one-dimensional waveguide in which one end is open and the other is either open (infinite waveguide) or closed by a mirror (semi-infinite). Upon injection of two photons (corresponding to weak coherent driving), the resonance fluorescence and photon correlations are shaped by the effective qubit transition frequencies and decay rates, which are substantially modified by interference effects. In contrast to the well-known result in an infinite waveguide, photons reflected by a single 2LS coupled to a semi-infinite waveguide are initially bunched, a result that can be simply explained by stimulated emission. As the number of 2LS increases (up to 10 are considered here), rapid oscillations build up in the correlations that persist for a very long time. For instance, when the incoming photons are slightly detuned, the transmitted photons in the infinite waveguide are highly antibunched. On the other hand, upon resonant driving, incoherently reflected photons are mostly distributed within the photonic band gap and several sharp side peaks. These features can be explained by considering the poles of the single particle Green function in the Markovian regime combined with the time delay. Our calculation is not restricted to the Markovian regime, and we obtain several fully non-Markovian results. We show that a single 2LS in a semi-infinite waveguide can not be decoupled by placing it at the node of the photonic field, in contrast to recent results in the Markovian regime. Our results illustrate the complexities that ensue when several qubits are strongly coupled to a bus (the waveguide) as might happen in quantum information processing.
Waveguide circuit quantum electrodynamics (waveguide circuit QED) studies light-matter interaction with superconducting circuits in one dimension. In circuit QED, natural atoms are replaced by superconducting qubits consisting of a non-linear Josephson junction, resulting in an anharmonic energy spectrum just like real atoms. With superconducting qubits, it is possible to study quantum optical phenomena and reach new regimes hard to achieve with real atoms due to weak coupling to the electromagnetic field. The reduction to one dimension in waveguide QED increases the electromagnetic field's directionality, which results in reduced losses. In this thesis, we first introduce circuit quantisation, giving the basis for the next part, where we investigate a transmon, a charge-insensitive artificial atom, coupled to a semi-infinite transmission line. An atom coupled to a semi-infinite waveguide is referred to as an atom in front of a mirror and is the subject of all appended papers. We proceed by summarising Paper I and III's main results: in Paper I, we investigate the spontaneous emission of a transmon coupled to a semi-infinite transmission line, where we take time-delay effects into account. We find that the system dynamics strongly depend on the coupling strength to the transmission line and the atom's position with respect to the electromagnetic field, leading to the Purcell effect or the convergence to a dark state with finite excitation probability. In the high-impedance regime, which we investigate in Paper III, the properties of the transmon coupled to the high-impedance transmission line change drastically. It becomes highly reflective and creates its own cavity with the mirror, resulting in the emergence of cavity modes and vacuum Rabi oscillations in the spontaneous emission dynamics. In the next chapter of the thesis, we demonstrate how to quantise an electromagnetic field and derive a light-matter interaction Hamiltonian within dipole approximation. We then give an introduction to open quantum systems and derive the quantum-optical master equation in Lindblad form. Furthermore, we introduce the dressed state picture, where the interaction of light and matter is so strong that the individual energy levels of light and matter are no longer separable. Both the quantum optical master equation and the dressed state picture are relevant in Paper II and IV. In Paper II, an experimental collaboration, we perform several experiments to characterise and discriminate different decay rates of a superconducting qubit coupled to the end of a transmission line. One experiment measured the atomic fluorescence spectral density, which shows an asymmetry for off-resonant driving, resulting from pure dephasing: an effect that we explain in more detail in this thesis and Paper II. In Paper IV, we theoretically investigate amplification mechanisms realised by different set-ups of an atom coupled to a semi-infinite waveguide. In the considered systems, the amplification of a probe field happens either due to population inversion between the pure states or dressed states or multi-photon processes. We find that compared to an open waveguide, we can achieve a higher gain in the amplification with a semi-infinite waveguide.
We study two-level systems (2LS) coupled at different points to a one-dimensional waveguide in which one end is open and the other is either open (infinite waveguide) or closed by a mirror (semi-infinite). Upon injection of two photons (corresponding to weak coherent driving), the resonance fluorescence and photon correlations are shaped by the effective qubit transition frequencies and decay rates, which are substantially modified by interference effects. In contrast to the well-known result in an infinite waveguide, photons reflected by a single 2LS coupled to a semi-infinite waveguide are initially bunched, a result that can be simply explained by stimulated emission. As the number of 2LS increases (up to 10 are considered here), rapid oscillations build up in the correlations that persist for a very long time. For instance, when the incoming photons are slightly detuned, the transmitted photons in the infinite waveguide are highly antibunched. On the other hand, upon resonant driving, incoherently reflected photons are mostly distributed within the photonic band gap and several sharp side peaks. These features can be explained by considering the poles of the single-particle Green function in the Markovian regime combined with the time delay. Our calculation is not restricted to the Markovian regime, and we obtain several fully non-Markovian results. We show that a single 2LS in a semi-infinite waveguide can not be decoupled by placing it at the node of the photonic field, in contrast to recent results in the Markovian regime. Our results illustrate the complexities that ensue when several qubits are strongly coupled to a bus (the waveguide) as might happen in quantum information processing.