Quantum multicriticality not only has fundamental research significance but also can promote the development of emerging quantum technologies, owing to its rich phase transition mechanisms and quantum resources. While theoretical studies have predicted the multicritical phenomena in the light-matter systems, the experimental demonstration remains elusive for the challenges of achieving the system's ground or steady states in strong coupling regimes. Here, by implementing the quantum adiabatic algorithm and the dissipative-system variational quantum algorithm on nuclear magnetic resonance quantum simulator, we successfully demonstrate the tricritical phenomena both in the closed and open systems described by the two-axis Rabi model. The experimental results clearly show that, beyond the decoherence effect, dissipation leads to the emergence of a novel multicritical phenomenon: it splits the first-order phase transition line of the closed Rabi model, and doubles the tricritical point. Our work provides a feasible technique for engineering the open quantum systems and opens a new avenue for exploring nonequilibrium many-body physics.
Quantum multicriticality not only has fundamental research significance but also can promote the development of emerging quantum technologies, owing to its rich phase transition mechanisms and quantum resources. While theoretical studies have predicted the multicritical phenomena in the light-matter systems, the experimental demonstration remains elusive for the challenges of achieving the system's ground or steady states in strong coupling regimes. Here, by implementing the quantum adiabatic algorithm and the dissipative-system variational quantum algorithm on nuclear magnetic resonance quantum simulator, we successfully demonstrate the tricritical phenomena both in the closed and open systems described by the two-axis Rabi model. The experimental results clearly show that, beyond the decoherence effect, dissipation leads to the emergence of a novel multicritical phenomenon: it splits the first-order phase transition line of the closed Rabi model, and doubles the tricritical point. Our work provides a feasible technique for engineering the open quantum systems and opens a new avenue for exploring nonequilibrium many-body physics.
We investigate the nonequilibrium steady state of the anisotropic open quantum Rabi model, which exhibits first-order and second-order dissipative phase transitions upon varying the degree of anisotropy between the coupling strengths of rotating and counter-rotating terms. Using both semiclassical and quantum approaches, we find a rich phase diagram resulting from the interplay between the anisotropy and the dissipation. First, there exists a bistable phase where both the normal and superradiant phases are stable. Second, there are multicritical points where the phase boundaries for the first- and second-order phase transitions meet. We show that a new set of critical exponents governs the scaling of the multicritical points. Finally, we discuss the feasibility of observing the multicritical transitions and bistability using a pair of trapped ions where the anisotropy can be tuned by controlling the intensity of the Raman transitions. Our study enlarges the scope of critical phenomena that may occur in finite-component quantum systems, which could be useful for applications in critical quantum sensing. Published by the American Physical Society 2024
We explore the influence of dissipation on a paradigmatic driven-dissipative model where a collection of two level atoms interact with both quadratures of a quantum cavity mode. The closed system exhibits multiple phase transitions involving discrete and continuous symmetries breaking and all phases culminate in a multicritical point. In the open system, we show that infinitesimal dissipation erases the phase with broken continuous symmetry and radically alters the model's phase diagram. The multicritical point now becomes brittle and splits into two tricritical points where first- and second-order symmetry-breaking transitions meet. A quantum fluctuations analysis shows that, surprisingly, the tricritical points exhibit anomalous finite fluctuations, as opposed to standard tricritical points arising in ^{3}He-^{4}He mixtures. Our work has direct implications for a variety of fields, including cold atoms and ions in optical cavities, circuit-quantum electrodynamics as well as optomechanical systems.
We demonstrate a novel mechanism driving complex critical phenomena in open light-atom interacting systems by investigating a parametrically amplified quantum Rabi model (QRM) subject to both single- and two-photon decay. In the classical oscillator limit, four composite phases emerge, arising from the possible normal or superradiant regimes across the upper and lower spin branches. A mean-field analysis reveals that the two-photon decay activates the intrinsic nonlinearity of the QRM. The synergy of the coherent and dissipative two-photon processes, together with the spin-boson coupling, constitutes an ``inverted" regime where superradiance emerges exclusively at weak coupling. This regime features first- and second-order superradiant DPTs separated by a tricritical point. Utilizing an adiabatic approach and the semi-classical Langevin formalism, we further study the steady-state structure beyond the mean-field level. The universality classes of the DPTs are identified, with the corresponding critical and finite-size scaling exponents derived and a scaling ansatz proposed to describe the critical behavior.
Precise control of criticality in superradiant phase transitions is essential for quantum state engineering and the simulation of nonequilibrium phase transitions. Here, we investigate theoretically multicritical phenomena in a dissipative two-Rydberg-atom cavity--QED system. The intrinisic dipole--dipole interaction between the two Rydberg atoms restructures the energy-level landscape of the atomic subsystem, thereby significantly modifying the boundary of the continuous second-order superradiant phase transition, and shifting both the phase boundary and the multicritical point toward weaker atom--cavity strengths. For sufficiently strong dipole--dipole interactions, the continuous second-order phase transition and the multicritical point both disappear, leaving only a discontinuous first--order phase transition that enables the emergence of a superradiant phase even at arbitrarily weak atom--cavity coupling. This work is of fundamental interest for studying dissipative quantum phase transitions, with potential implications for quantum precision measurement and quantum sensing.
Quantum optics is the field of physics that studies the interaction between light and matter under a fully quantum mechanical treatment. In recent decades, relentless advances in the technologies used for trapping, cooling, and controlling atoms and molecules have allowed us to finally start exploring experimentally the physics displayed by different cornerstone models of quantum optics originally proposed in the second half of the 20th century. In this thesis, we propose multiple extensions to those fundamental models, expanding the already interesting physics displayed by them into new and exciting directions. More specficially, we study these generalized models in the context of quantum phase transitions both in and out of equilibrium and show how new phases of matter can be unlocked in these extended models. In Chapters 1 and 2 we briefly introduce the reader to the realms of quantum phase transitions and quantum optics. Once the fundamental aspects of both of these fields are covered, we present the superradiant phase transition displayed in the Dicke and Rabi models in Chapter 3. This phase transition will be the central topic we will be orbiting around in the subsequent chapters. In Chapter 4 we propose a generalization of the quantum Rabi model, where N cavities, instead of one, are connected to each other through photon hopping. In this system, named the quantum Rabi ring, interesting chiral superradiant phases can develop as a function of the hopping phase and the geometry of the ring. In particular, we find that geometrical frustration plays a key role in determining the stable phases in equilibrium. Moreover, frustration manifests itself in the quantum Rabi ring through unconventional non-symmetric critical exponents, a phenomenon reported before, but hardly observed in condensed matter materials. Finally, in Chapter 5, we introduce a different extension to the Dicke model where instead of two-level atoms, three-level atoms are considered. In this system, which we have named the tricritical Dicke model, the superradiant phase transition can occur through first-order, second-order, and third-order critical points. We study the critical properties of the system in and out of equilibrium and find that in the open-system description, the tricritical points are still present but are now accompanied by regions of bistability where the final fate depends highly on the initial conditions. These regions of bistability represent potentially interesting environments to investigate dynamical features and steady-state preparation schemes. The critical phenomena displayed by the extended models proposed here, such as multicriticality, geometrically frustrated quantum phases, and chiral phases breaking time-reversal symmetry, are all features that have been observed, although not abundantly, or proposed in condensed matter physics. However, the unmatched tunability and control of atomic and molecular experimental platforms, where the models presented in this thesis are proposed to be realized, causes these extended models to become promising candidates for investigating these features in parameter regimes and conditions never explored before.
We investigate the dissipative phase transitions of the anisotropic quantum Rabi model with cavity decay and demonstrate that large spin fluctuations persist in the stationary state, having important consequences on the phase diagram and the critical properties. In the second-order phase transition to the superradiant phase, there is a significant suppression of the order parameter and the appearance of nonuniversal factors, which directly reflect the spin populations. Furthermore, upon entering a parameter regime where mean-field theory predicts a tricritical phase, we find a first-order phase transition due to the unexpected collapse of superradiance. An accurate and physically transparent description going beyond mean-field theory is established by combining exact numerical simulations, the cumulant expansion, and analytical approximations based on reduced master equations and an effective equilibrium theory. Our findings, compared to the conventional thermodynamic limit of the Dicke model, indicate a general tendency of forming extreme nonequilibrium states in the single-spin system, thus have broad implications for dissipative phase transitions of few-body systems. Published by the American Physical Society 2024