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Modal phase-matching in thin-film lithium niobate waveguides for efficient generation of entangled photon pairs

Jiacheng Liu, Jia-Chen Duan, Pingyu Zhu, Gongyu Xia, Qilin Hong, Kaikai Zhang, Zhihong Zhu, Shiqiao Qin, Ping Xu

Published Oct 13, 2024• 11 citations

Abstract

Thin-film lithium niobate (TFLN) waveguides have emerged as a pivotal platform for on-chip spontaneous parametric down-conversion (SPDC), serving as a crucible for the generation of entangled photon pairs. The periodic poling of TFLN, while capable of generating high-efficiency SPDC, demands intricate fabrication processes that can be onerous in terms of scalability and manufacturability. In this work, we introduce a novel approach to the generation of entangled photon pairs via SPDC within TFLN waveguides, harnessing the principles of modal phase-matching (MPM). To address the challenge of efficiently exciting pump light typically in a higher-order mode, we have engineered a mode converter that couples two asymmetrically dimensioned waveguides. This converter adeptly transforms the fundamental mode into a higher-order mode, demonstrating a conversion loss of 1.55 dB at 785 nm with a 3 dB bandwidth exceeding 30 nm. Subsequently, we have showcased the device's capabilities by characterizing the pair generation rate (PGR), coincidences-to-accidentals ratio (CAR), and spectral profile of the entangled photon source. Our findings present a simplified and versatile method for the on-chip generation of entangled photon sources, which may pave the way for the application in the realms of quantum information processing and communication technologies.

DOI: 10.1364/oe.539105

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Thin-film lithium niobate (TFLN) waveguides have emerged as a pivotal platform for on-chip spontaneous parametric down-conversion (SPDC), serving as a crucible for the generation of entangled photon pairs. The periodic poling of TFLN, while capable of generating high-efficiency SPDC, demands intricate fabrication processes that can be onerous in terms of scalability and manufacturability. In this work, we introduce a novel approach to the generation of entangled photon pairs via SPDC within TFLN waveguides, harnessing the principles of modal phase-matching (MPM). To address the challenge of efficiently exciting pump light typically in a higher-order mode, we have engineered a mode converter that couples two asymmetrically dimensioned waveguides. This converter adeptly transforms the fundamental mode into a higher-order mode, demonstrating a conversion loss of 1.55 dB at 785 nm with a 3 dB bandwidth exceeding 30 nm. Subsequently, we have showcased the device's capabilities by characterizing the pair generation rate (PGR), coincidences-to-accidentals ratio (CAR), and spectral profile of the entangled photon source. Our findings present a simplified and versatile method for the on-chip generation of entangled photon sources, which may pave the way for the application in the realms of quantum information processing and communication technologies.

Spontaneous parametric down-conversion (SPDC) has become a key method for generating entangled photon pairs. Periodically poled thin-film lithium niobate (TFLN) waveguides induce strong SPDC but require complex fabrication processes. In this work, we experimentally demonstrate efficient SPDC and second harmonic generation using modal phase matching methods. This is achieved with inverse-designed optical mode converters and low-loss optical waveguides in a single nanofabrication process. Inverse design methods provide enhanced functionalities and compact footprints for the converter. Despite the extensive achievements in inverse-designed photonic integrated circuits, the potential of inverse-designed TFLN quantum photonic devices has been seldom explored. The device shows an on-chip conversion efficiency of 3.95% W−1 cm−2 in second harmonic generation measurements and a coincidence count rate up to 21.2 kHz in SPDC experiments. This work highlights the potential of the inverse-designed TFLN photonic devices and paves the way for their applications in on-chip nonlinear or quantum optics.

Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.

Polarization-entangled photon pairs are essential sources for photonic quantum information processing. However, generating entangled photon pairs with large detuning via spontaneous parametric down-conversion (SPDC) often requires complex configurations to compensate for phase matching. Here, we propose a simple and efficient scheme to generate polarization-entangled photon pairs based on type-0 SPDC in a thin-film lithium niobate waveguide with a single poling period. By utilizing the strong dispersion engineering capabilities of thin-film waveguides, we can achieve both degenerate and highly detuned entangled photon pairs. Furthermore, we demonstrate on-chip temporal compensation using an integrated waveguide structure. Our approach offers a compact and scalable solution for integrated quantum photonic circuits.

Efficient generation of high-quality photon pairs is essential for modern quantum technologies. Micro-ring resonator is an ideal platform for studying on-chip photon sources due to strong nonlinear effect, resonant-enhanced optical fields, and high integration. Thin-film lithium niobate (TFLN) micro-ring resonators with periodically poled quasi-phase matching have shown high-quality photon pair generation. However, periodic poling technology remains expensive and requires complex fabrication hindering its scalability and capability for practical application in nonlinear photonic devices. To address this, we propose a scalable approach using TFLN micro-ring resonators based on modal phase matching to achieve cost-effective, efficient high-quality photon pair generation, significantly simplifying fabrication. We achieved pair generation rates up to 40.2 MHz/mW through spontaneous parametric down-conversion, with coincidence-to-accidental ratios exceeding 1,200. By combining micro-ring resonance enhancement with modal phase matching, our approach reduces device size and fabrication cost while maintaining high nonlinear efficiency. These results advance the development of compact, efficient on-chip photon sources for next-generation nonlinear and quantum photonic applications.

Spontaneous parametric down conversion in nonlinear material is widely exploited to generate entangled photon pairs in quantum optics experiments and applications, including quantum computing and communication. Periodically poled thin film lithium niobate (PPTFLN) has emerged as a promising platform for efficient entangled photon pair generation, offering enhanced nonlinear interaction through quasi-phase matching (QPM) and tight confinement of light. However, achieving optimal performance requires careful control of the QPM condition since the waveguide in TFLN is highly dispersive to changes in the geometric parameter. In this study, we fabricate PPTFLN rib waveguides to generate entangled photon pairs at telecommunication wavelengths, varying geometric parameters. QPM condition is confirmed with the second harmonic generation experiments and Pair generation rate and coincidence-to-accidental count ratio are also estimated by temporal coincidence measurement. Digital etching process is introduced to control the QPM condition, resulting in incremental peak wavelength shift by discrete etching step. This is expected to contribute to synchronizing wavelength of quantum nodes.