Our research optimized Spherical Bragg Resonators to engineering emissions from Er3+ and Eu3+ emitters, enhancing light-matter interaction. The study achieved significant electromagnetic field and radiative decay rate enhancements, demonstrating the potential for efficient lasing and all-dielectric nanoantenna.
We formulated an analytical model and analyzed the modification of spontaneous emission in Bragg onion resonators. We consider both the case of a single light emitter and a uniformly distributed ensemble of light emitters within the resonator. We obtain an expression for the average radiation rate of the light emitters ensemble and discuss the modification of the average radiation rate as a function of cavity parameters such as the core radius, the number of Bragg cladding layers, the index contrast of the Bragg cladding, and the refractive index of surrounding medium. We also consider the possibility of non-exponential decay of the light emitter ensemble due to the strong dependence of spontaneous emission on the location and polarization of individual light emitter. We conclude that Bragg onion resonators can both enhance and inhibit spontaneous emission by several orders of magnitude. This property can have significant impact in the field of cavity quantum electrodynamics (QED).
Attempting to implement quantum information related applications utilizing atoms and photons, as they naturally form quantum systems supporting superposition states, hybrid quantum plasmonic systems emerged in the past as a platform to study and engineer light-matter interaction. This platform combines the unrivaled electromagnetic field localization of surface plasmon polaritons, boosting the light-matter coupling rate, with the tremendous integration potential of truly nanoscale structures, and both the significant emission rates of nanoantennas and photonic transmission velocities. In this work, a classical description of surface plasmon polaritons is combined with a light-matter interaction model based on a cavity quantum electrodynamical formalism. The resulting composite semi-classical method, introduced and described in this thesis, provides efficient and versatile means to simulate the dynamical behavior of radiative atomic transitions coupled to plasmonic cavity modes in the weak incoherent coupling regime. Both the emission into the far field and various dissipation mechanisms are included by expanding the model to an open quantum system. The variety of light-matter interaction applications that can be modeled with the outlined method is indicated by the four different exemplary scenarios detailed in the application chapter of this thesis. The classical description of localized surface plasmon polaritons is benchmarked by reproducing the experimental measurements of the molecular fluorescence manipulation through optical nanoantennas in a collaborative effort with experimental partners. Furthermore, in the weak light-matter coupling regime, the potential of achieving a higher nanoantenna functionality and simultaneously realizing more elaborate quantum dynamics is revealed by the three remaining applications. Each pivotally involving a bimodal nanoantenna and demonstrating different quantum optical phenomena, the implementation of cavity radiation mode conversion, non-classical cavity emission statistics, and non-classical cavity emission properties is shown and described in the application chapter.
Matter coupled to light can emit photons. In the absence of an external field this process is known as spontaneous emission. The radiation properties depends in detail the nature of the emitter. In this thesis we consider a two level point-source emitter, and examine how the emission is affected by engineering the local environment. We begin by studying analytically how embedding an emitter in a multi-layer cylindrical structure with radius much smaller than the emission wavelength alters the intensity of the emitted light. We find that for carefully chosen metal-dielectric interfaces, the emission can be strongly enhanced by the plasmonic effect. With this intuition, we experimentally study an InGaN semiconductor quantum dot-in-wire structure as our two level emitter, and manipulate the local field environment by coupling to a lossy plasmonic cavity. We find that the strong enhancement of the field around the quantum dot due to the metal more than compensates for the non-radiative losses, leading to order-of-magnitude increases in the radiative spontaneous emission rate, as well as overall brightness. We then examine how the emission of light can be affected by other nearby emitters. The cooperative effects are strongly dependent on the dimension of the system which controls the electromagnetic mode overlap of the emitters. We present a unified formalism capturing how these cooperative effects change from one dimension to the next. Cooperative light scattering between emitters underpins collective effects such as super- and sub-radiance, and we numerically investigate how our previous results give rise to the key experimental signatures that can be used to identify those phenomena. Specifically, we study how the superadiant decay rate scales with the size of a 2-dimensional atomic cloud, and how cooperative effects between a small number of emitters alter the emission spectrum of strongly driven resonance fluorescence.