Quantum sensing based on Rydberg atoms is an emerging technology for electric-field measurement. Theoretical and numerical studies were generally limited by the many-body effect in atomic ensembles. In this work, we initially derived a many-body dynamic equation by incorporating the Rydberg- Rydberg interaction into the four-level optical Bloch equation. Particularly, we proposed a fast steady-state solution as an alternative to the transient one. As a result, we ingeniously replaced the computationally expensive matrix operations with a linearly iterative process, enabling rapid convergence within few steps while considering the Doppler frequency shift. This approach made it possible to simulate the interaction of 7000 atoms in less than a minute. Based on the many-body model, we investigated the phenomenon of electromagnetically induced transparency (EIT) and Autler- Townes (AT) splitting under varying atomic gas densities; and compared the numerical results with experimental data. The comparison revealed a relatively-low error of 4.59% for the EITAT simulation by the many-body model. Moreover, we found that the linear dynamic range of the quantum sensing shrinks when considering the many-body interaction.
Quantum sensing based on Rydberg atoms is an emerging technology for electric-field measurement. Theoretical and numerical studies were generally limited by the many-body effect in atomic ensembles. In this work, we initially derived a many-body dynamic equation by incorporating the Rydberg- Rydberg interaction into the four-level optical Bloch equation. Particularly, we proposed a fast steady-state solution as an alternative to the transient one. As a result, we ingeniously replaced the computationally expensive matrix operations with a linearly iterative process, enabling rapid convergence within few steps while considering the Doppler frequency shift. This approach made it possible to simulate the interaction of 7000 atoms in less than a minute. Based on the many-body model, we investigated the phenomenon of electromagnetically induced transparency (EIT) and Autler- Townes (AT) splitting under varying atomic gas densities; and compared the numerical results with experimental data. The comparison revealed a relatively-low error of 4.59% for the EITAT simulation by the many-body model. Moreover, we found that the linear dynamic range of the quantum sensing shrinks when considering the many-body interaction.
Quantum sensing using Rydberg atoms is an emerging technology for precise measurement of electric fields. However, most existing computational methods are all based on a single-particle model and neglect Rydberg-Rydberg interaction between atoms. In this study, we introduce the interaction term into the conventional four-level optical Bloch equations. By incorporating fast iterations and solving for the steady-state solution efficiently, we avoid the computation of a massive 4 N × 4 N dimensional matrix. Additionally, we apply the Doppler frequency shift to each atom used in the calculation, eliminating the requirement for an additional Doppler iteration. These schemes allow for the calculation of the interaction between 7000 atoms around one minute. Based on the many-body model, we investigate the Rydberg-Rydberg interaction of Rydberg atoms under different atomic densities. Furthermore, we compare our results with the literature data of a three-level system and the experimental results of our own four-level system. The results demonstrate the validity of our model, with an effective error of 4.59% compared to the experimental data. Finally, we discover that the many-body model better predicts the linear range for measuring electric fields than the single-particle model, making it highly applicable in precise electric field measurements.
This thesis investigates the effects of strong Rydberg-Rydberg interactions in the presence of three-level coherent phenomena such as electromagnetically induced transparency (EIT), Autler-Townes splitting (ATS) and coherent population trapping (CPT). As a result of their remarkable properties, highly excited Rydberg atoms have great potential for applications in diverse areas. The interaction-induced dipole blockade between the Rydberg atoms has been proposed as a fundamental tool in quantum information processing with neutral atoms. Yet, they require an increasing level of understanding and control. A many-body theory is developed for the Rydberg excitation dynamics in various atomic systems with different densities and velocity distributions such as for atoms in a vapour cell, ultracold atoms in magneto-optical and optical dipole traps, or a system of optical lattices or dipole trap arrays. The systems were investigated by solving the optical Bloch equations numerically for a two-photon ladder excitation scheme, taking into consideration various experimentally relevant conditions for the emergence of the effects of Rydberg-Rydberg interactions. The lineshape properties of the EIT/ATS/CPT spectra are observed and reviewed while the physical arguments for how the lineshape properties change as a function of various parameters are provided. To account for the differing atomic distributions in the atomic systems, a many-body model based on Monte-Carlo simulation is developed to describe the optical response of the multiatoms systems to two-photon excitation laser lights in the regimes of EIT, ATS and CPT and strong atomic interactions. The study of the lineshape properties allows one to understand possible ways to detect the emergence of interaction-induced excitation suppression, asymmetry, line shift and excitation "antiblockade" enhancement effects. Besides these, the main result of this study is the demonstration that the linewidth properties of the Rydberg EIT/ATS/CPT spectra can reveal collective many-body behaviour associated with the creation of many-body entangled states. The linewidth properties provide compelling evidence of the creation of collective states by confirming the predicted dependence of the generalised Rabi frequency on the square root of the number of atoms in the mesoscopic ensemble. This study could help to quantify and control the conditions necessary for creating many-body entanglement within atomic ensembles. The thesis also describes the step towards experimentally investigating the response of an atomic system to excitation lasers and studying the excitation dynamics of interacting atoms in such systems. Significant work was done to set up the two-photon excitation system for preparing atoms in high-lying Rydberg states and performing Rydberg-based vapour cell experiments. Qualitative analysis of the Rydberg states transparency features allows to obtain laser parameters such as the laser linewidths and Rabi frequencies that are used in the theoretical model to create the similarity between the experimental and theoretical parameters. Further works were carried out towards realising the building blocks for experimentally investigating the interactions between Rydberg atoms in ultracold atom systems. This is by setting-up a trapping system capable of producing a highly dense ultracold atom ensemble within a magneto-optical trap, cold enough to serve as a reservoir from which the optical dipole trap can be loaded efficiently. The optical dipole trap is designed and set up to achieve a micron-size trapping potential capable of producing a sub-micron sized atomic cloud, with a controllable number of atoms, where a full blockade effect can be achieved and exploited to implement a qubit system for quantum gate operations.
We investigate the transient optical response property of an electromagnetically induced transparency (EIT) in a cold Rydberg atomic gas. We show that both the transient behavior and the steady-state EIT spectrum of the system depend strongly on Rydberg interaction. Especially, the response speed of the Rydberg-EIT can be five times faster (and even higher) than the conventional EIT without the Rydberg interaction. For comparison, two different theoretical approaches (i.e., two-atom model and many-atom model) are considered, revealing that Rydberg blockade effect plays a significant role for increasing the response speed of the Rydberg-EIT. The fast-responding Rydberg-EIT by using the strong, tunable Rydberg interaction uncovered here is not only helpful for enhancing the understanding of the many-body dynamics of Rydberg atoms but also useful for practical applications in quantum information processing by using Rydberg atoms.
In recent years, quantum electric field sensing technology based on Rydberg atoms has developed rapidly. Although some studies have begun to focus on the time evolution of two-photon-atom interactions and have conducted preliminary discussions on the transient behavior of EIT systems, most of the work still solves the EIT driving equation under the steady-state assumption and pays insufficient attention to the complete response process of atoms to the external electric field. In order to further fill this research gap, we formulate a density-matrix model for a ladder-type three-level Rydberg system and solve the EIT-driven equations under non-steady-state conditions. Numerical simulations reveal the real-time evolution of the atomic response during two-photon excitation and elucidate how various system parameters shape this response. On this basis, we identify optimal parameter settings that enhance the real-time performance of Rydberg-atom quantum measurements and provide theoretical guidance for future sensor design.
Open quantum system, coupled with an external bath is a key research field of quantum physics. Steady state is the state in which any initial state converges after a long time and is usually of the most interest. However, relatively speaking, the nonequilibrium dynamical processes of quantum many-body systems have been rarely studied. This is mainly due to the fact that quantum many-body systems generally have interactions, and the Hilbert space required for a complete description of their dynamical processes will grow exponentially with the number of particles increasing, and the computational difficulty will increase dramatically as well. Hence, it is a difficult problem to completely describe their dynamical processes completely. With the development of quantum technologies, the interest in the nonequilibrium dynamics of open quantum many-body systems is aroused. A common phenomenon is the metastable state, where the system initially relaxes into a long-lived state and then converges to the final stationary state for a longer time. In this paper, we establish a low-dimensional approximation to describe the metastability dynamics in Markovian open quantum system, based on the spectra of the Liouvillian super-operator. The separation of time scales implies a splitting in the spectrum, and this spectral division allows us to eliminate the fast decay modes by using the perturbation method, and then we establish the effective description in the low-lying eigenmodes subspace. Furthermore, we study the dynamics process of the Rydberg atomic system under electromagnetically induced transparency (EIT) conditions and find that the system can handle metastable dynamics if the atomic interactions are considered. We compare the effective dynamics in the subspace with the actual dynamics in the full space, and the results show that the effective dynamics works well on condition that the perturbation approximation holds. Our work provides a feasible idea and method for establishing an effective and simplified description of the dynamical process of open quantum many-body systems.
The Rydberg-based microwave detection is an all-optical technology that uses the strong coherent interaction between Rydberg atoms and microwave field. Different from the traditional microwave meter, the Rydberg atomic sensing is a new-type microwave detector that transforms the microwave spectrum into a coherent optical spectrum, and arouses increasingly the interests due to its high sensibility. For this kind of sensor, the coherence effect induced by coupling atoms with microwave plays a key role, and the decoherence may reduce the sensitivity. A multi-level Rydberg atomic scheme with optimized quantum coherence, which enhances both the bandwidth and the sensitivity for 4 GHz microwave sensing, is demonstrated experimentally in this work. The enhanced quantum coherence of Rydberg electromagnetically induced transparency (EIT) and microwave induced Autler-Townes (AT) splitting in EIT windows are shown using optical pumping at D1 line. The enhanced sensitivity at 3.4 GHz with 0.3 GHz bandwidth can be realized, based on the enhanced EIT-AT spectrum. The experimental results show that in the stepped Rydberg EIT system, the spectral width of EIT and microwave field EIT-AT can be narrowed by optical pumping (OP), so the sensitivity of microwave electric field measurement can be improved. After optimizing the EIT amplitude and adding single-frequency microwaves, the sensitivity of the microwave electric field measurement observed by the AT splitting interval is improved by 1.3 times. This work provides a reference for utilizing atomic microwave detection.