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Science Advances

Infrared single-photon detection with superconducting magic-angle twisted bilayer graphene

Giorgio Di Battista, Kin Chung Fong, A. Díez-Carlón, Kenji Watanabe, Takashi Taniguchi, Dmitri K. Efetov

Published Sep 18, 2024• 23 citations
Publisher

Abstract

carriers per square centimeter, which is five orders of magnitude lower than traditional superconductors (SCs). This results in an ultralow electronic heat capacity and a large kinetic inductance of this truly two-dimensional SC, providing record-breaking parameters for quantum sensing applications, specifically thermal sensing and single-photon detection. To fully exploit these unique superconducting properties for quantum sensing, here, we demonstrate a proof-of-principle experiment to detect single near-infrared photons by voltage biasing an MATBG device near its superconducting phase transition. We observe complete destruction of the SC state upon absorption of a single infrared photon even in a 16-square micrometer device, showcasing exceptional sensitivity. Our work offers insights into the MATBG-photon interaction and demonstrates pathways to use moiré superconductors as an exciting platform for revolutionary quantum devices and sensors.

DOI
10.1126/sciadv.adp3725

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carriers per square centimeter, which is five orders of magnitude lower than traditional superconductors (SCs). This results in an ultralow electronic heat capacity and a large kinetic inductance of this truly two-dimensional SC, providing record-breaking parameters for quantum sensing applications, specifically thermal sensing and single-photon detection. To fully exploit these unique superconducting properties for quantum sensing, here, we demonstrate a proof-of-principle experiment to detect single near-infrared photons by voltage biasing an MATBG device near its superconducting phase transition. We observe complete destruction of the SC state upon absorption of a single infrared photon even in a 16-square micrometer device, showcasing exceptional sensitivity. Our work offers insights into the MATBG-photon interaction and demonstrates pathways to use moiré superconductors as an exciting platform for revolutionary quantum devices and sensors.
The superconducting (SC) state of magic-angle twisted bilayer graphene (MATBG) shows exceptional properties, as it consists of an unprecedentedly small electron (hole) ensemble of only ~ 10 power 11 carriers per square centimeter, which is five orders of magnitude lower than in traditional superconductors. This results in an ultra-low electronic heat capacity and kinetic inductance of this truly two-dimensional SC, and provides record-breaking key parameters for a variety of quantum sensing applications, in particular in thermal sensing and single photon detection (SPD), which traditionally exploit thermal effects in nanostructured superconducting thin films. In this work, we systematically study the interaction of the superconducting state of MATBG with individual light quanta. We discover full destruction of the SC state upon absorption of a single infrared photon even in a 16 square micrometer sized device, which showcases its exceptional bolometric sensitivity. Upon voltage biasing close to its critical current, we further show that this non-optimized device can be used as a SPD, whose click-rate is proportional to the number of absorbed photons, following Poissonian statistics. Our work offers insights into the MATBG-photon interaction and shows up pathways to use low-carrier density graphene-based superconductors as a new platform for developing revolutionary new quantum devices and sensors.
In this work I present theory, modeling, and experimentation demonstrating that the graphene-based Josephson junction (GJJ) is a capable system for the detection of single photons across the electromagnetic spectrum, from the microwave to the infrared. Two different detection mechanisms are exposed: 1) heating of the graphene weak link in the GJJ and 2) quasiparticle generation in the GJJ superconducting contacts. The first relies on graphene's exceptionally low heat capacity and its decoupled electron and phonon systems. I show in modeling that these thermal properties can lead to a GJJ photon detector for very low energy microwave photons. Experimentally, I show that a GJJ bolometer with its graphene weak link coupled to a microwave resonator can achieve an energy resolution equivalent to a single 32-GHz photon. The second detection mechanism reveals itself in the illumination of a GJJ with near-infrared light. I experimentally demonstrate single-photon detection in this system and show that the data is well fit by a model where photon-induced quasiparticles in the superconducting contacts cause the GJJ phase particle to escape. I give an overview of the single-photon, graphene, and Josephson-junction physics required to arrive at these results before presenting the experimental evidence for single-microwave-photon sensitivity and single-infrared-photon detection with the GJJ.
Josephson junctions are superconducting devices used as high-sensitivity magnetometers and voltage amplifiers as well as the basis of high-performance cryogenic computers and superconducting quantum computers. Although device performance can be degraded by the generation of quasiparticles formed from broken Cooper pairs, this phenomenon also opens opportunities to sensitively detect electromagnetic radiation. We demonstrate single near-infrared photon detection by coupling photons to the localized surface plasmons of a graphene-based Josephson junction. Using the photon-induced switching statistics of the current-biased device, we reveal the critical role of quasiparticles generated by the absorbed photon in the detection mechanism. The photon sensitivity will enable a high-speed, low-power optical interconnect for future superconducting computing architectures.
We propose a novel quantum computing architecture that combines the engineered electromagnetic properties of quantum metamaterials with the strongly correlated electron physics of magic-angle systems. By integrating magic-angle twisted bilayer graphene (MATBG) into superconducting metamaterial waveguides, we demonstrate theoretically that the resulting hybrid system exhibits: (1) enhanced qubit coherence through geometric control of electromagnetic modes, (2) tunable qubit-qubit coupling via metamaterial dispersion engineering, and (3) topologically protected quantum states arising from the interplay of moiré band structure and metamaterial boundary conditions. Our framework provides design equations for a scalable quantum computing platform that leverages both the flat-band physics of magic-angle materials and the controllable photon-matter interactions of quantum metamaterials.
We propose to use graphene-based Josephson junctions (GJJs) to detect single photons in a wide electromagnetic spectrum from visible to radio frequencies. Our approach takes advantage of the exceptionally low electronic heat capacity of monolayer graphene and its constricted thermal conductance to its phonon degrees of freedom. Such a system could provide high-sensitivity photon detection required for research areas including quantum information processing and radio astronomy. As an example, we present our device concepts for GJJ single-photon detectors in both the microwave and infrared regimes. The dark count rate and intrinsic quantum efficiency are computed based on parameters from a measured GJJ, demonstrating feasibility within existing technologies.
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State-of-the-art Superconducting Nanowire Single Photon Detectors based on low-Tc materials reach 100% quantum efficiency. However, the response time is limited to >1-10 ns. Recently, it has been shown that due to a much lower kinetic inductance, a 100 ps response rate can be achieved in 120 μμμm-long MgB2MgB_{2}MgB2​ nanowires. In this work, we demonstrate experimentally that such MgB2MgB_{2}MgB2​ nanowires function as single-photon detectors for both visible (λλλ= 630 nm) and infrared (λλλ= 1550 nm) photons when biased close to the critical current, with a dark count rate of <10 cps. MgB2MgB_{2}MgB2​ photodetectors over-perform NbN SNSPDs in speed by at least an order of magnitude for similar nanowire lengths. Such photodetectors offer a platform for single-photon detectors with a long thought-after combination of a large detector area and a response rate of up to 10 GHz with a single readout line.