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Nature Communications

Storing light near an exceptional point

Yicheng Zhu, Jiankun Hou, Qi Geng, Boyi Xue, Yuping Chen, Xianfeng Chen, Li Ge, Wenjie Wan

Published Sep 16, 2024• 28 citations
Publisher

Abstract

Photons with zero rest mass are impossible to be stopped. However, a pulse of light can be slowed down and even halted through strong light-matter interaction in a dispersive medium in atomic systems. Exceptional point (EP), a non-Hermitian singularity point, can introduce an abrupt transition in dispersion. Here we experimentally observe room-temperature storing light near an exceptional point induced by nonlinear Brillouin scattering in a chip-scale 90-μm-radius optical microcavity, the smallest platform up to date to store light. Through nonlinear coupling, a Parity-Time (PT) symmetry can be constructed in optical-acoustical hybrid modes, where Brillouin scattering-induced absorption (BSIA) can lead to both slow light and fast light of incoming pulses. A subtle transition of slow-to-fast light reveals a critical point for storing a light pulse up to half a millisecond. This compact and room-temperature scheme of storing light paves the way for practical applications in all-optical communications and quantum information processing. Exceptional point introduces the ability to control and tune light propagation. Here the authors demonstrate a 90-μm-radius optical microcavity to store light, induced by nonlinear Brillouin scattering at room temperature.

DOI
10.1038/s41467-024-52064-4

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Photons with zero rest mass are impossible to be stopped. However, a pulse of light can be slowed down and even halted through strong light-matter interaction in a dispersive medium in atomic systems. Exceptional point (EP), a non-Hermitian singularity point, can introduce an abrupt transition in dispersion. Here we experimentally observe room-temperature storing light near an exceptional point induced by nonlinear Brillouin scattering in a chip-scale 90-μm-radius optical microcavity, the smallest platform up to date to store light. Through nonlinear coupling, a Parity-Time (PT) symmetry can be constructed in optical-acoustical hybrid modes, where Brillouin scattering-induced absorption (BSIA) can lead to both slow light and fast light of incoming pulses. A subtle transition of slow-to-fast light reveals a critical point for storing a light pulse up to half a millisecond. This compact and room-temperature scheme of storing light paves the way for practical applications in all-optical communications and quantum information processing. Exceptional point introduces the ability to control and tune light propagation. Here the authors demonstrate a 90-μm-radius optical microcavity to store light, induced by nonlinear Brillouin scattering at room temperature.
Almost twenty years ago, light was slowed down to less than 10^{-7} of its vacuum speed in a cloud of ultracold atoms of sodium. Upon a sudden turn-off of the coupling laser, a slow light pulse can be imprinted on cold atoms such that it can be read out and converted into a photon again. In this process, the light is stopped by absorbing it and storing its shape within the atomic ensemble. Alternatively, the light can be stopped at the band edge in photonic-crystal waveguides, where the group speed vanishes. Here, we extend the phenomenon of stopped light to the new field of parity-time (PT) symmetric systems. We show that zero group speed in PT symmetric optical waveguides can be achieved if the system is prepared at an exceptional point, where two optical modes coalesce. This effect can be tuned for optical pulses in a wide range of frequencies and bandwidths, as we demonstrate in a system of coupled waveguides with gain and loss.
Abstract Storing or delaying optical signals is of key interest for fundamental research and applications in radar, microwave signal processing, quantum information as well as optical communication systems. Delay systems based on stimulated Brillouin scattering (SBS), a coherent interaction between optical and acoustic waves can be implemented in optical fiber or chip-scale platforms, operate at room temperature and can be fully controlled via the optical pump wave. In this article, we review delay and storage techniques based on SBS. We present SBS slow-light, fiber delay lines based on Brillouin dynamic gratings, Brillouin quasi-light storage and Brillouin-based light storage via photon-phonon conversion and compare their performance. In this process, we also include an overview of different platforms used for Brillouin light storage and delay schemes, such as optical fiber, planar soft-glass waveguides, and silica fiber-tip resonators.
The ability to control and manipulate light with light is crucial for optical information and communication technology. However, all-optical information processing is hindered by the absence of interactions between photons in linear materials. Nonlinear materials mediate effective photon-photon interactions, but require large light intensity. Optical resonators store and confine light for many optical cycles, which increases the interaction time and reduces the nonlinearity threshold. However, monolithic optical resonators have limited variability of the intra-cavity medium. Instead, a wide variety of materials can be easily integrated in tunable open-access microcavities, making them an ideal platform for exploring novel materials for nonlinear optics. In this thesis, we present experiments using coherently driven tunable open-access microcavities hosting either oil or a perovskite semiconductor. In Chapter 2 we demonstrate steady-state room-temperature superfluidity of photons in an oil-filled cavity, and reveal how the fluid dynamics are influenced by the nonlocality of the effective interactions mediated by the oil. Chapters 3 and 4 describe experiments using a halide perovskite semiconductor in an open-access microcavity in a closed-cycle cryostat. We demonstrate continuous-wave nonlinearity in the halide perovskite material through optical bistability, and reveal signatures of a phase transition in the temperature dependence of the nonlinearity strength. Next we investigate the emergence of irreversibility in the bistable switching of our perovskite cavity. Finally, we present in Chapter 5 experimental observations of fast nonlinearity-enabled oscillations in the light intensity, that occur despite the slowness of thermal nonlinearity of the oil.
Storing and delaying optical signals is key for signal processing and control in many microwave photonics, quantum and classical communication systems. Hence, scientists proposed and demonstrated a multitude of approaches, from slow-light in photonic crystals, ring resonators, to optomechanical and stimulated Brillouin scattering (SBS) based schemes [1]. Yet, a scheme that offers tunable, long delays in a small form factor is still elusive. Quasi-light storage (QLS) is an optical pulse storage method that has been used to achieve long, dynamically adjustable delay times in optical fibres by utilising SBS to spectrally sample a signal with an optical frequency comb [2]. Relying on long lengths of fibre, however, limits Size, Weight, and Power consumption (SWaP) and induces latency much larger than the storage time. Here, we demonstrate QLS on a photonic chip and achieve delay times an order of magnitude larger than the optical chip transit time. We experimentally show that the SBS interaction between the signal and the pump on the chip creates a single acoustic wave that stores the optical pulse information, and we investigate the temporal dynamics of this storage mechanism. We demonstrate that the repeated interaction of the acoustic wave and optical pump pulses reinforces the acoustic wave, and storage times an order of magnitude larger than the intrinsic acoustic lifetime can be achieved.
The importance of optical signal processing techniques is growing rapidly in recent years due to the exponentially increasing demand for bandwidth, capacity and power efficiency in communications and computing. However, due to their bosonic nature photons do not interact with each other, unless there is a nonlinear medium mediating the interaction. One of the strongest nonlinear effects is the interaction of light waves, photons, with sound-waves, acoustic phonons, which is known as stimulated Brillouin scattering (SBS). This thesis experimentally investigates SBS in photonic chips. It is shown in this thesis that the fundamental interaction strength between light and sound waves can be tailored by using one-dimensional photonic bandgap structures, completely suppressing the effect or alternatively enhancing the interaction to form phase-locked Brillouin frequency combs. It was shown furthermore that efficiently generating SBS on-chip enables the generation of stable RF signals that are widely tunable in frequency. Finally, it is shown in this thesis that SBS enables the storage of light signals on a chip, one of the holy grails of all-optical signal processing. Delaying optical signals is of key importance in optical networks to enable synchronization, buffering, and rerouting. SBS enables large delays by resonantly transferring an optical signal to an acoustic wave, that travels five orders of magnitude slower and retrieving it after a certain storage time. It is demonstrated in this thesis that a Brillouin-based memory (BBM) technique allows storing amplitude and phase of optical data pulses and operate at multiple wavelengths with minimal cross-talk. Replenishing of the acoustic wave to overcome storage time limitations imposed by the lifetime of the acoustic wave as well as non-reciprocal light storage is also shown.
I n 1998, laser pulses were slowed [1] in a Bose-Einstein condensate (BEe) [2] ofsodium to only 17 m/s, more than seven orders of magnitude lower than the speed of light in vacuum. Associated with the dramatic reduction factor for the light speed was a spatial compression of the pulses by the same large factor. A light pulse, which was more than 1 km long in vacuum, was compressed to a size of -50 flm, and at that point was completely contained within the condensate [1]. This allowed the light-slowing experiments to be brought to their ultimate extreme [3]: in the summer of 2000, light pulses were completely stopped, stored, and subsequently revived in an atomic medium, with millisecond storage times [4]. The initial ultra-slow light experiments spurred a flurry of slow light investigations, and slow or partially stopped light has now been observed in limited geometries in warm rubidium vapours [5-7], liquid-nitrogen cooled crystals [8], and recently in room temperature crystals [9]. Here, we begin with a discussion ofultra-slow and stopped light. We describe how cold atoms and Bose-Einstein condensates have been manipulated to generate media with extreme optical properties. While the initial experiments concentrated on the light propagation, we have recently begun a number of investigations of the effects that slow light has on the medium in which it propagates. Effects are profound because both the velocity and length scales associated with propagating light pulses have been brought down to match the characteristic velocity and length scales of the medium. With the most recent extension, the light roadblock [10], we have compressed light pulses to a length ofonly 2 f!ill. Here, we describe the use of ultra-compressed light pulses to probe superfluidity and the creation of quantized vortices in BEes through formation of'superfluid shock. waves'. We also present the observation of an ultra-slow-light-based, pulsed atom laser. Furthermore, we demonstrate the use of slow and stopped light for manipulation of optical information, in particular in Bose-Einstein condensates that allow for phase coherent processing of three-dimensional, compressed patterns of stored optical information.