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Physical Review A

Temperature dependence of optical phase transitions in a system of two-level atoms and photons interacting inside a nonlinear cavity

S. Samimi, Mohammad Mehdi Golshan

Published Sep 17, 2024• 0 citations
Publisher

Abstract

In the present work, the role of temperature in the occurrence of optical phases in a system of a large number of atoms interacting with photons is reported. To this end, it is assumed that the cavity inside which the constituents interact is in equilibrium with a heat reservoir, held at a fixed temperature. To achieve this goal, we start with the conventional density operator to calculate the mean values of electromagnetic quadratures. To make the realization of three distinct optical phases, trivial, electric, and magnetic superradiance, possible, the medium inside the cavity is assumed to be a second-order nonlinear one. The nonlinearity of the medium is further assumed to be activated by an externally applied classical pump field. As a consequence, now there are two external controlling agents, the temperature and nonlinearity strength. We then proceed to calculate the quadrature mean values in the thermodynamical limit and for a large number of atoms as a function of temperature. An analysis of the calculated mean values, along with relevant figures, reveals temperature-dependent conditions for realizing trivial, electric, and magnetic optical phases. Moreover, we shall demonstrate that the atom-field coupling strength gives rise to two distinct regimes where the optical phases behave quite differently. In one of the two regimes it is possible for the phases to coexist, while in the other it is not. As a profound result, it is demonstrated that for such a system there can exist a unique temperature (triple point) at which the three optical phases coexist.

DOI
10.1103/physreva.110.033714

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In this paper, we investigate the finite-temperature properties and phase transition of the Dicke model. Converting the atomic pseudo-spin operator to the two-mode Fermi operators, we obtain the partition function in terms of the imaginary-time path integral. The atomic population and average photon number as analytic functions of the atom-photon coupling strength are found from the thermodynamic equilibrium equation, which leads to the stationary state at a finite temperature and is determined by the variation in an extremum-condition of the Euclidean action with respect to the bosonic field. In particular we study the phase transition from normal to superradiation phase at a fixed low-temperature, in which the phase transition is dominated by quantum fluctuations. The phase transition induced by the variation of the atom-photon coupling strength indeed obeys the Landau continuous phase-transition theory, in which the average photon-number can serve as an order parameter with non-zero value that characterizes the superradiation phase. In the zero temperature limit our results recover exactly all those obtained from the quantum phase transition theory at zero temperature. In addition, we discuss the thermodynamic properties and compare the difference between finite-temperature phase transition and zero-temperature quantum phase transition. It is discovered that the average photon-number and mean energy in the low-temperature stationary state coincide with the corresponding values of zero-temperature in the strong coupling region. The entropy of the superradiation phase decays rapidly to zero with the increase of coupling strength.

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Phase transition and thermodynamic properties of N two-level atoms in an optomechanical cavity at finite temperature

Ni Liu, Shan Huang, Jun‐Qi Li +1 more

Optomechanical cavity is a powerful connection between a nanomechanical oscillator and a quantized electromagnetic field. In this system, a novel photon-phonon nonlinear interaction arising from the nanomechanical oscillation is produced through the radiation pressure. Now this nonlinear photon-phonon interaction has become an important resource for implementing high-precision measurements and processing quantum information. Motivated by T. Esslinger group’s experiment, it is very meaningful to explore the exotic quantum phenomena when a ultra-cold BEC is trapped in an optomechanical cavity. In this paper, we mainly investigate phase transition and the finite-temperature thermodynamic properties of a Bose-Einstein condensate in an optomechanical cavity. It’s worth mentioning that at zero temperature many different mean-field approximate methods have been used to analyze the ground state properties of a Bose-Einstein condensate in an optomechanical cavity. Two common methods are Holstein-Primakoff transformation and spin coherent state variation. In this paper, an interesting imaginary-time path integral approach has been introduced to study finite temperature thermodynamic properties and phase transition of a Bose-Einstein condensate in an optomechanical cavity. First, we obtained system's partition function by taking imaginary-time path integration. Meanwhile, an effective action has been obtained by means of this method, which is the basic of the variation to get the numerical solution of photon number and the expression of the atomic number. At zero temperature, these results are consistent with what we have obtained by Holstein-Primakoff transformation or spin coherent state variational method. By adjusting the atom-field coupling strength and other parameters the second-order phase transition from the normal phase to the superradiant phase has been revealed. Meanwhile, a new unstable superradiant state was also found. And we found that in addition to the normal phase and superradiation phase, there exists an un-solution region of the mean photon number. Meanwhile, we find that the nonlinear photon-phonon interaction does not affect the normal phase. However, in the superradiant phase, the nonlinear photon-phonon interaction can enhance the macroscopic collective excitations. At the same time, the thermodynamic properties of the system are also discussed. According to the obtained distribution function, we can derive the analytical expression of the average energy and the free energy. Furthermore, the expression of entropy at finite temperature can also be obtained. we find the nonlinear photon-phonon interaction does not affect the average energy in the normal phase, but the average energy in the superradiant phase can deeply deviate in the large nonlinear photon-phonon interaction. It’s worth mentioning that the mean photon number and average energy in the finite-temperature tend to be consistent with the case in absolute zero temperature in the strong coupling region, while the entropy in the superradiant phase is rapidly reduced to zero as the atom-field coupling strength increases. In other words, strongly coupled collective excited states are highly ordered and are not affected by thermal fluctuations in the temperature range we are considering. The thermodynamic properties, such as the entropy and corresponding specific heat, characterize the Dicke phase transition.

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Ultracold Atoms in Optical Cavities

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This thesis summarizes the research work we did in the past years, which focuses on the theoretical study of quantum effects of ordered atomic structures interacting with the quantum electric field of an optical resonator. Within this work we investigated the quantum properties of the light at the cavity output, emitted by this kind of system, and the quantum state of the atoms confined by the light fields of the cavity mode. Following one possible partition, we have organized the thesis in two parts. The first part of the thesis is devoted to the quantum properties of the light at the output of optical cavities, in which atoms are confined. After a brief introduction on the basics of atom-photon interactions, we show theoretically, that two atomic dipoles in a resonator can behave as a quantum non-linear medium, whose response can be controlled through the interactomic distance of the atoms inside the resonator. We identify the parameter regime, for which the system operates as a parametric amplifier, based on the atoms' collective dipole cascade emission. Moreover we also determine the corresponding field squeezing spectrum at the cavity output. These dynamics could be observed as a result of self-organization processes of laser-cooled atoms in resonators. The second part of the thesis studies the quantum ground state of an ultracold atomic gas trapped inside an optical resonator by the mechanical effects of atom-photon interactions. Due to the strong coupling regime, the ultracold atomic gas feels a quantum potential, where the fluctuations at the single photon level may be relevant in determining the trapping conditions. This potential depends on the atomic distribution, which at the same time determines the intracavity field amplitude. Here, after a brief introduction on ultracold atoms in optical lattices, we study the low temperature physics of an ultracold atomic gas in the quantum potential formed inside a pumped cavity, by mapping the dynamics to an effective Bose-Hubbard model. We predict the existence of non-compressible states of the atomic gas, and determine a phase diagram as a function of the cavity parameters. Novel effects are encountered, such as the existence of overlapping stability regions corresponding to competing insulator-like states when the laser pumps the cavity, to provide one example out of many. At the end of the thesis a concluding chapter presents some general outlooks to this thesis work.

•Jan 1, 2010•0 citations
In the present work, the role of temperature in the occurrence of optical phases in a system of a large number of atoms interacting with photons is reported. To this end, it is assumed that the cavity inside which the constituents interact is in equilibrium with a heat reservoir, held at a fixed temperature. To achieve this goal, we start with the conventional density operator to calculate the mean values of electromagnetic quadratures. To make the realization of three distinct optical phases, trivial, electric, and magnetic superradiance, possible, the medium inside the cavity is assumed to be a second-order nonlinear one. The nonlinearity of the medium is further assumed to be activated by an externally applied classical pump field. As a consequence, now there are two external controlling agents, the temperature and nonlinearity strength. We then proceed to calculate the quadrature mean values in the thermodynamical limit and for a large number of atoms as a function of temperature. An analysis of the calculated mean values, along with relevant figures, reveals temperature-dependent conditions for realizing trivial, electric, and magnetic optical phases. Moreover, we shall demonstrate that the atom-field coupling strength gives rise to two distinct regimes where the optical phases behave quite differently. In one of the two regimes it is possible for the phases to coexist, while in the other it is not. As a profound result, it is demonstrated that for such a system there can exist a unique temperature (triple point) at which the three optical phases coexist.
In the present article, we investigate the behavior of a large collection of three-level $\mathrm{\ensuremath{\Lambda}}$ atoms interacting with two quantized electromagnetic fields inside a second-order nonlinear quantum cavity. The nonlinearity of the cavity is supposed to be activated by the application of two classical pump fields. The total Hamiltonian of the combination, with due attention to the nonlinearity effects, is diagonalized. The corresponding ground-state energy then follows from minimizing the total Hamiltonian. The structure of the ground state indicates that four distinct optical phases can occur in such a system. These possible phases turn out to be trivial, dark, left-arm and right-arm superradiant ones. Conditions under which any of the four optical phases can actually occur are also analyzed and discussed. The analysis of the conditions, accompanied by several figures, then reveals that with a suitable choice of the pump field amplitudes and/or geometrical phases, one can intensify the two superradiant phases drastically. Moreover, we demonstrate that the dark optical phase cannot occur at all, while the trivial and superradiant ones can, in fact, coexist. Our calculations also show that transition from the trivial phase to left-arm (right-arm) superradiant one is continuous (discrete) and second (first) order in nature. Another important result of our investigation is that by adjusting the pump field strength, one can switch from the left-arm superradiant phase to the right-arm one and vice versa. This point, in turn, provides an alternative mechanism for the development of quantum optical switching devices.
In the present report, the question of U(1) symmetry breaking in a system of atoms and electromagnetic fields, interacting inside a leaky cavity, filled with a nonlinear medium, is addressed. In particular, the Z2{Z}_{2}Z2​ discrete symmetry of the system and the emergence of optical phases are fully discussed. For the nonlinearity of a general order, with an electromagnetic field of any number of modes, conditions under which the resulting field-field interactions destroy the U(1) (and Z2{Z}_{2}Z2​) symmetry are determined. We then apply the theory to the case of a collection of two-level atoms and three electromagnetic modes. Taking one of the fields as a classically adjustable pumping one, it is demonstrated that the quantized field-field coupling profoundly depends upon the pump field strength. The presence of two competing phenomena, namely, the cavity photonic dissipation and nonlinearity, is shown to lead the system towards steady behavior. The steady-state solutions to the atomic population and field quadratures exhibit the normal and superradiant phases, depending on the strengths of pumping field and atom-field couplings. The conditions for the stability of such steady-state solutions are also discussed in detail. A notable result of the present article is that by adjusting the parameters involved in the system one can switch from the normal to electric and/or magnetic superradiant phases.
In this paper, we investigate the finite-temperature properties and phase transition of the Dicke model. Converting the atomic pseudo-spin operator to the two-mode Fermi operators, we obtain the partition function in terms of the imaginary-time path integral. The atomic population and average photon number as analytic functions of the atom-photon coupling strength are found from the thermodynamic equilibrium equation, which leads to the stationary state at a finite temperature and is determined by the variation in an extremum-condition of the Euclidean action with respect to the bosonic field. In particular we study the phase transition from normal to superradiation phase at a fixed low-temperature, in which the phase transition is dominated by quantum fluctuations. The phase transition induced by the variation of the atom-photon coupling strength indeed obeys the Landau continuous phase-transition theory, in which the average photon-number can serve as an order parameter with non-zero value that characterizes the superradiation phase. In the zero temperature limit our results recover exactly all those obtained from the quantum phase transition theory at zero temperature. In addition, we discuss the thermodynamic properties and compare the difference between finite-temperature phase transition and zero-temperature quantum phase transition. It is discovered that the average photon-number and mean energy in the low-temperature stationary state coincide with the corresponding values of zero-temperature in the strong coupling region. The entropy of the superradiation phase decays rapidly to zero with the increase of coupling strength.
The authors consider a system comprised of a collection of identical two-level atoms interacting with the electromagnetic field in the dipole approximation and with an externally applied steady-state coherent driving field. The atoms are considered to interact with each other only via the electromagnetic field and are assumed to be contained within a volume much smaller than a resonance wavelength. The system is treated as a quantum-statistical ensemble in the rotating frame, rotating at the carrier frequency of the externally applied coherent field. The Hamiltonian in this frame is explicitly time independent and the exact analog of a spin temperature is defined. The thermodynamic-Green's-function method is used to determine the thermodynamic equilibrium properties of the system in the rotating frame. This results in a nonlinear relation between the applied field and the field in the volume containing the atoms. The expression is a nonlinear function of the effective or "spin" temperature as well, and has the form of a first-order phase transition with the macroscopic atomic polarization as order parameter. In the low-"spin"-temperature limit, and for perfect tuning, the expression reduces to the exact form of the nonlinear relation for optical bistability derived by Bonifacio and Lugiato and relating the incident and transmitted fields for atoms in a ring cavity in the mean-field approximation. The results contain absorptive as well as dispersive contributions. These results predict essentially different behavior as a function of off tuning compared with behavior predicted by others using statistical steady-state models far from thermodynamic equilibrium. In the limit of zero value for the applied field amplitude, the results reduce to the conditions for the well-known second-order superradiant" phase transition. The condition for the existence of the second-order phase transition is shown to depend on the cavity tuning and the photon escape rate. The authors also show why, in light of the experiments in optical bistability, this second-order phase is difficult to observe.
Optomechanical cavity is a powerful connection between a nanomechanical oscillator and a quantized electromagnetic field. In this system, a novel photon-phonon nonlinear interaction arising from the nanomechanical oscillation is produced through the radiation pressure. Now this nonlinear photon-phonon interaction has become an important resource for implementing high-precision measurements and processing quantum information. Motivated by T. Esslinger group’s experiment, it is very meaningful to explore the exotic quantum phenomena when a ultra-cold BEC is trapped in an optomechanical cavity. In this paper, we mainly investigate phase transition and the finite-temperature thermodynamic properties of a Bose-Einstein condensate in an optomechanical cavity. It’s worth mentioning that at zero temperature many different mean-field approximate methods have been used to analyze the ground state properties of a Bose-Einstein condensate in an optomechanical cavity. Two common methods are Holstein-Primakoff transformation and spin coherent state variation. In this paper, an interesting imaginary-time path integral approach has been introduced to study finite temperature thermodynamic properties and phase transition of a Bose-Einstein condensate in an optomechanical cavity. First, we obtained system's partition function by taking imaginary-time path integration. Meanwhile, an effective action has been obtained by means of this method, which is the basic of the variation to get the numerical solution of photon number and the expression of the atomic number. At zero temperature, these results are consistent with what we have obtained by Holstein-Primakoff transformation or spin coherent state variational method. By adjusting the atom-field coupling strength and other parameters the second-order phase transition from the normal phase to the superradiant phase has been revealed. Meanwhile, a new unstable superradiant state was also found. And we found that in addition to the normal phase and superradiation phase, there exists an un-solution region of the mean photon number. Meanwhile, we find that the nonlinear photon-phonon interaction does not affect the normal phase. However, in the superradiant phase, the nonlinear photon-phonon interaction can enhance the macroscopic collective excitations. At the same time, the thermodynamic properties of the system are also discussed. According to the obtained distribution function, we can derive the analytical expression of the average energy and the free energy. Furthermore, the expression of entropy at finite temperature can also be obtained. we find the nonlinear photon-phonon interaction does not affect the average energy in the normal phase, but the average energy in the superradiant phase can deeply deviate in the large nonlinear photon-phonon interaction. It’s worth mentioning that the mean photon number and average energy in the finite-temperature tend to be consistent with the case in absolute zero temperature in the strong coupling region, while the entropy in the superradiant phase is rapidly reduced to zero as the atom-field coupling strength increases. In other words, strongly coupled collective excited states are highly ordered and are not affected by thermal fluctuations in the temperature range we are considering. The thermodynamic properties, such as the entropy and corresponding specific heat, characterize the Dicke phase transition.
This thesis summarizes the research work we did in the past years, which focuses on the theoretical study of quantum effects of ordered atomic structures interacting with the quantum electric field of an optical resonator. Within this work we investigated the quantum properties of the light at the cavity output, emitted by this kind of system, and the quantum state of the atoms confined by the light fields of the cavity mode. Following one possible partition, we have organized the thesis in two parts. The first part of the thesis is devoted to the quantum properties of the light at the output of optical cavities, in which atoms are confined. After a brief introduction on the basics of atom-photon interactions, we show theoretically, that two atomic dipoles in a resonator can behave as a quantum non-linear medium, whose response can be controlled through the interactomic distance of the atoms inside the resonator. We identify the parameter regime, for which the system operates as a parametric amplifier, based on the atoms' collective dipole cascade emission. Moreover we also determine the corresponding field squeezing spectrum at the cavity output. These dynamics could be observed as a result of self-organization processes of laser-cooled atoms in resonators. The second part of the thesis studies the quantum ground state of an ultracold atomic gas trapped inside an optical resonator by the mechanical effects of atom-photon interactions. Due to the strong coupling regime, the ultracold atomic gas feels a quantum potential, where the fluctuations at the single photon level may be relevant in determining the trapping conditions. This potential depends on the atomic distribution, which at the same time determines the intracavity field amplitude. Here, after a brief introduction on ultracold atoms in optical lattices, we study the low temperature physics of an ultracold atomic gas in the quantum potential formed inside a pumped cavity, by mapping the dynamics to an effective Bose-Hubbard model. We predict the existence of non-compressible states of the atomic gas, and determine a phase diagram as a function of the cavity parameters. Novel effects are encountered, such as the existence of overlapping stability regions corresponding to competing insulator-like states when the laser pumps the cavity, to provide one example out of many. At the end of the thesis a concluding chapter presents some general outlooks to this thesis work.