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Physical Review A

Optical coherence transfer in atom arrays

P. R. Berman, A. Kuzmich

Published Sep 5, 2024• 0 citations
Publisher

Abstract

A $J=0$ to $J=1$ to $J=0$ ladder scheme can be used as a prototype for probing optical coherence transfer in an atom array. Two incident ${\ensuremath{\sigma}}_{\ensuremath{-}}$ polarized fields drive transitions from the ground state to the intermediate state and the intermediate state to the uppermost state in the atoms. The uppermost state is taken to be a long-lived Rydberg level. In the absence of any atom-atom interactions, excitation to the Rydberg level is not allowed, owing to the selection rules. However, dipole-dipole interactions can provide a transfer of the state amplitude associated with the $m=\ensuremath{-}1$ sublevel in one atom to the $m=+1$ sublevel in another atom. The overall process of field excitation and optical coherence transfer can then lead to an excitation of the Rydberg level. One can then apply a readout pulse to obtain phase-matched emission from the array. For a linear array of atoms, the phase-matched signal can increase more rapidly than ${N}^{2}$, where $N$ is the number of atoms in the array. For arrays that are invariant under a rotation $\ensuremath{\delta}\ensuremath{\phi}<\ensuremath{\pi}$ about the $z$ axis, however, it turns out that the total field intensity vanishes identically in the phase-matched direction. For such arrays, the Rydberg state population can serve as a measure of the optical coherence transfer.

DOI
10.1103/physreva.110.033703

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A J=0J=0J=0 to J=1J=1J=1 to J=0J=0J=0 ladder scheme can be used as a prototype for probing optical coherence transfer in an atom array. Two incident \ensuremathσ\ensuremath−{\ensuremath{\sigma}}_{\ensuremath{-}}\ensuremathσ\ensuremath−​ polarized fields drive transitions from the ground state to the intermediate state and the intermediate state to the uppermost state in the atoms. The uppermost state is taken to be a long-lived Rydberg level. In the absence of any atom-atom interactions, excitation to the Rydberg level is not allowed, owing to the selection rules. However, dipole-dipole interactions can provide a transfer of the state amplitude associated with the m=\ensuremath−1m=\ensuremath{-}1m=\ensuremath−1 sublevel in one atom to the m=+1m=+1m=+1 sublevel in another atom. The overall process of field excitation and optical coherence transfer can then lead to an excitation of the Rydberg level. One can then apply a readout pulse to obtain phase-matched emission from the array. For a linear array of atoms, the phase-matched signal can increase more rapidly than N2{N}^{2}N2, where NNN is the number of atoms in the array. For arrays that are invariant under a rotation \ensuremathδ\ensuremathϕ<\ensuremathπ\ensuremath{\delta}\ensuremath{\phi}<\ensuremath{\pi}\ensuremathδ\ensuremathϕ<\ensuremathπ about the zzz axis, however, it turns out that the total field intensity vanishes identically in the phase-matched direction. For such arrays, the Rydberg state population can serve as a measure of the optical coherence transfer.
Abstract We demonstrate a synthetic gauge phase in Rydberg electromagnetically induced transparency (EIT) using room-temperature rubidium vapor. By utilizing the polarization selection rules in a ladder-type system involving ground, intermediate, and Rydberg states, multiple Zeeman sublevels form closed-loop transitions that acquire a gauge phase. We show that the relative polarization angle between the linearly polarized probe and coupling lasers directly controls the gauge phase, which modulates the EIT transmission and Rydberg state population, consequently controlling the linewidth of EIT owing to Rydberg dipole–dipole interactions between atoms. Our approach provides a simple polarization-based method for realizing synthetic gauge physics and manipulating many-body interactions in atomic ensembles without requiring laser cooling or dipole traps.
Quantum nonlinear optics by Rydberg polaritons can enable single-photon transistor and switch, single-photon source, and deterministic quantum information processing. A major hindrance in this study is the fast motional decoherence. Here, we devise a scheme to significantly enhance the coherence of Rydberg polariton by letting the atoms {\it remember} their velocities, or, alternatively, by {\it changing} the phase of Rydberg polariton according to its storage time. After the Rydberg polariton is prepared with a Rydberg state ∣r1⟩|r_1\rangle∣r1​⟩, i.e., during the storage time, two laser fields induce a transition between ∣r1⟩|r_1\rangle∣r1​⟩ and a nearby Rydberg state ∣r2⟩|r_2\rangle∣r2​⟩ via a low-lying intermediate state ∣f⟩\lvert f\rangle∣f⟩ which is largely detuned. In particular, we find that either a 2πN2π\mathbb{N}2πN protocol, a πππ-wait-πππ protocol, or a wait-πππ protocol, along with an appropriate choice of ∣f⟩\lvert f\rangle∣f⟩ can lead to a phase-coherent Rydberg polariton upon its retrieval. Importantly, the coherent transition between ∣r1⟩|r_1\rangle∣r1​⟩ and ∣r2⟩|r_2\rangle∣r2​⟩ ensures that the Rydberg polariton can block the Rydberg excitation of nearby atoms as in usual applications of Rydberg polaritons. Numerics show that the theory can nearly completely eliminate the motional dephasing, leaving Rydberg-state decay as the only fundamental channel of decoherence. This sheds light on a broad application of Rydberg-mediated quantum nonlinear optics.
We present a theory of cascade emission from an array of NNN fixed, ``three-level'' atoms. The total angular momentum of the ground state of each atom is J=0J=0J=0, that of the intermediate state is J=1J=1J=1, and that of the upper state is J=0J=0J=0. The atoms are prepared in a spatially phased superposition of their ground and upper states, collectively sharing a single excitation. We calculate the time-integrated, joint probability distribution for radiation to be emitted in a given direction with a given polarization on each transition and use this joint probability distribution to calculate the time-integrated intensity emitted on each transition. The dipole-dipole interaction between the atoms is taken into account. Analytic expressions are obtained for two atoms and the calculation is then extended formally to an ensemble of NNN atoms at arbitrary positions. As expected, the radiation emitted on the upper transition is unpolarized and isotropic. However, somewhat surprisingly, we find that for excitation by counterpropagating fields and for nearly equal ground to intermediate and intermediate to upper level transition frequencies, the radiation on the lower transition is also isotropic and unpolarized, provided the atoms are prepared in a fully symmetric state. We also establish conditions for which there can be a phase-matched enhancement of the joint probability density for specific directions of emissions on the upper and lower transitions.
We demonstrate a synthetic gauge phase in Rydberg electromagnetically induced transparency (EIT) using room-temperature rubidium vapor. By exploiting polarization selection rules in a ladder-type system involving ground, intermediate, and Rydberg states, multiple Zeeman sublevels form closed-loop transitions that acquire a gauge phase. We show that the relative polarization angle between the linearly polarized probe and coupling lasers directly controls this gauge phase, which modulates the EIT transmission and Rydberg state population, consequently controlling the linewidth of EIT due to Rydberg dipole-dipole interactions between atoms. Our approach provides a simple polarization-based method for realizing synthetic gauge physics and manipulating many-body interactions in atomic ensembles without requiring laser cooling and dipole traps.