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Quantum 2.0 Conference and Exhibition

Cavity-Quantum Electrodynamics with Single Diamond Tin-Vacancy Centers

Yanik Herrmann, Julius Fischer, Julia M. Brevoord, Colin Sauerzapf, Leonardo G. C. Wienhoven, Laurens J. Feije, Matteo Pasini, Martin Eschen, Maximilian Ruf, Matthew J. Weaver, Ronald Hanson

Published Jan 1, 2024• 0 citations
Publisher

Abstract

We show diamond Tin-Vacancy centers, coherently-coupled to a tunable microcavity. The exceptional optical properties of this emitter in combination with a stable, high quality cavity enables a cavity transmission signal modulated by a single emitter.
DOI
10.1364/quantum.2024.qm2b.4

Related papers

Coherent Coupling of a Diamond Tin-Vacancy Center to a Tunable Open Microcavity

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Efficient coupling of optically active qubits to optical cavities is a key challenge for solid-state-based quantum optics experiments and future quantum technologies. Here we present a quantum photonic interface based on a single tin-vacancy center in a micrometer-thin diamond membrane coupled to a tunable open microcavity. We use the full tunability of the microcavity to selectively address individual tin-vacancy centers within the cavity mode volume. Purcell enhancement of the tin-vacancy center optical transition is evidenced both by optical excited state lifetime reduction and by optical linewidth broadening. As the emitter selectively reflects the single-photon component of the incident light, the coupled emitter-cavity system exhibits strong quantum nonlinear behavior. On resonance, we observe a transmission dip of 50% for low incident photon number per Purcell-reduced excited state lifetime, while the dip disappears as the emitter is saturated with higher photon number. Moreover, we demonstrate that the emitter strongly modifies the photon statistics of the transmitted light by observing photon bunching. This work establishes a versatile and tunable platform for advanced quantum optics experiments and proof-of-principle demonstrations on quantum networking with solid-state qubits. Published by the American Physical Society 2024

arXiv:2311.08456•Physical Review X•Oct 15, 2024•23 citations

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Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR)•Jan 1, 2022•0 citations
Efficient coupling of optically active qubits to optical cavities is a key challenge for solid-state-based quantum optics experiments and future quantum technologies. Here we present a quantum photonic interface based on a single tin-vacancy center in a micrometer-thin diamond membrane coupled to a tunable open microcavity. We use the full tunability of the microcavity to selectively address individual tin-vacancy centers within the cavity mode volume. Purcell enhancement of the tin-vacancy center optical transition is evidenced both by optical excited state lifetime reduction and by optical linewidth broadening. As the emitter selectively reflects the single-photon component of the incident light, the coupled emitter-cavity system exhibits strong quantum nonlinear behavior. On resonance, we observe a transmission dip of 50% for low incident photon number per Purcell-reduced excited state lifetime, while the dip disappears as the emitter is saturated with higher photon number. Moreover, we demonstrate that the emitter strongly modifies the photon statistics of the transmitted light by observing photon bunching. This work establishes a versatile and tunable platform for advanced quantum optics experiments and proof-of-principle demonstrations on quantum networking with solid-state qubits. Published by the American Physical Society 2024
The tin-vacancy center in diamond (SnV) has emerged as a compelling building block for realizing next-generation quantum networks thanks to its excellent optical and spin properties. Coupling to photonic crystal cavities (PCCs) promises to further enhance the SnV light-matter interface and unlock a diverse range of entanglement generation protocols. Recent pioneering experiments showing Purcell enhancement of SnV centers in PCCs underscore this potential. However, optical coupling that is coherent - the key ingredient for use in quantum protocols - has so far remained elusive. Here, we demonstrate above-unity coherent cooperativity of SnV centers embedded in photonic crystal cavities. We fabricate free-standing PCCs using a quasi-isotropic undercut. Across two samples, we conduct room-temperature characterizations, measuring resonances for 327 cavities, with an average quality factor exceeding Q=1.0(3)×104Q = 1.0(3) \times 10^4Q=1.0(3)×104. Two cavity-coupled emitters are examined in detail, exhibiting quality factors up to Q=25.4(4)×103Q = 25.4(4) \times 10^3Q=25.4(4)×103 and Purcell-reduced lifetimes corresponding to cooperativities up to C=20.6(11)C = 20.6(11)C=20.6(11). Furthermore, the single SnVs are observed to strongly modulate the cavity transmission with an extinction contrast up to 98.8(4)%98.8(4) \%98.8(4)% on resonance. Finally, SnV linewidth measurements reveal above-unity coherent cooperativities in both devices, with the highest value being Ccoh=8.3(12)C_\mathrm{coh} = 8.3(12)Ccoh​=8.3(12). These results open the door to using cavity-coupled SnV centers as efficient, coherent light-matter interfaces for future quantum networks.
Efficient coupling between quantum emitters and optical cavities is essential for scalable quantum photonic technologies. Group-IV vacancy centers in diamond, particularly the negatively charged tin-vacancy center, have emerged as promising candidates due to their spectral stability, high Debye-Waller factor, and large orbital splitting in ground states. Here, we demonstrate controlled coupling of a single negatively charged tin-vacancy center hosted in a nanodiamond to a fully tunable Fabry-Pérot microcavity. At cryogenic temperatures, we access the weak-coupling regime and observe a transition from the bad-emitter regime to the bad-cavity regime as the optical transition of the color center narrows. At 4 K, a Purcell factor exceeding 1.7 is measured, confirming cavity-enhanced emission. The obtained results demonstrate the potential of Sn − V − centers in nanodiamonds as a coherent single-photon source for quantum networks.