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Optics Letters

Spontaneous parametric downconversion photon pair generation in small footprint X-cut periodically poled lithium niobate micro-resonator

Hyeon Hwang, Woojin Noh, Mohamad Reza Nurrahman, Guhwan Kim, Kiwon Moon, Jung Jin Ju, Hansuek Lee, Min‐Kyo Seo

Published Aug 29, 2024• 14 citations
Publisher

Abstract

Spontaneous parametric downconversion (SPDC) has been crucial for producing non-classical light, such as correlated photon pairs and squeezed states, essential for optical quantum technologies. Recently, thin-film lithium niobate (TFLN)-based devices have enabled high-performance SPDC in on-chip integrated photonic platforms. Here, we developed an X-cut periodically poled lithium niobate (PPLN) racetrack micro-resonator with a compact footprint and demonstrated bright SPDC photon pair generation characterized by distinct resonances and high extraction efficiency. We separately assessed the internal and loaded photon pair generation rates, measuring them at 4.525 MHz/µW and 62.73 kHz/µW, respectively. Our platform is integrated with maturing electro-/thermo-optic TFLN circuit elements and has meaningful potential for advancing active quantum photonic applications.

DOI
10.1364/ol.533039

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Spontaneous parametric down-conversion (SPDC) has been utilized in generating non-classical light, such as correlated photon pairs and squeezed light, significantly influencing optical quantum information research. Advances in thinfilm lithium niobate (TFLN) technologies have brought the benefits of χ(2)nonlinearity from bulk optics to integrated photonics. Targeting fully exploitation of high Electro-optic (EO) controllability and the periodic poled lithium niobate (PPLN), enabling quasi-phase matching (QPM), offer the realization especially under the X-cut based platform [1]–[3]. Moreover, the small footprint is also key figure of merit for efficient processing of SPDC spectrum. In this work, we demonstrate SPDC photon pair generation in a small footprint size with a 0.614 nm FSR at the IR wavelength, based on X-cut PPLN racetrack resonator.

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Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.

arXiv:2405.10943•Light Science & Applications•Oct 3, 2024•69 citations
Spontaneous parametric downconversion (SPDC) has been crucial for producing non-classical light, such as correlated photon pairs and squeezed states, essential for optical quantum technologies. Recently, thin-film lithium niobate (TFLN)-based devices have enabled high-performance SPDC in on-chip integrated photonic platforms. Here, we developed an X-cut periodically poled lithium niobate (PPLN) racetrack micro-resonator with a compact footprint and demonstrated bright SPDC photon pair generation characterized by distinct resonances and high extraction efficiency. We separately assessed the internal and loaded photon pair generation rates, measuring them at 4.525 MHz/µW and 62.73 kHz/µW, respectively. Our platform is integrated with maturing electro-/thermo-optic TFLN circuit elements and has meaningful potential for advancing active quantum photonic applications.
Spontaneous parametric down-conversion (SPDC) has been utilized in generating non-classical light, such as correlated photon pairs and squeezed light, significantly influencing optical quantum information research. Advances in thinfilm lithium niobate (TFLN) technologies have brought the benefits of χ(2)nonlinearity from bulk optics to integrated photonics. Targeting fully exploitation of high Electro-optic (EO) controllability and the periodic poled lithium niobate (PPLN), enabling quasi-phase matching (QPM), offer the realization especially under the X-cut based platform [1]–[3]. Moreover, the small footprint is also key figure of merit for efficient processing of SPDC spectrum. In this work, we demonstrate SPDC photon pair generation in a small footprint size with a 0.614 nm FSR at the IR wavelength, based on X-cut PPLN racetrack resonator.
Spontaneous parametric down-conversion (SPDC) has become a key method for generating entangled photon pairs. Periodically poled thin-film lithium niobate (TFLN) waveguides induce strong SPDC but require complex fabrication processes. In this work, we experimentally demonstrate efficient SPDC and second harmonic generation using modal phase matching methods. This is achieved with inverse-designed optical mode converters and low-loss optical waveguides in a single nanofabrication process. Inverse design methods provide enhanced functionalities and compact footprints for the converter. Despite the extensive achievements in inverse-designed photonic integrated circuits, the potential of inverse-designed TFLN quantum photonic devices has been seldom explored. The device shows an on-chip conversion efficiency of 3.95% W−1 cm−2 in second harmonic generation measurements and a coincidence count rate up to 21.2 kHz in SPDC experiments. This work highlights the potential of the inverse-designed TFLN photonic devices and paves the way for their applications in on-chip nonlinear or quantum optics.
Nanophotonic platforms have multiple properties and features desirable for producing correlated photon pairs. In these platforms, spontaneous parametric down-conversion (SPDC) and spontaneous four-wave-mixing (SFWM) have been used to achieve photon pair production. By placing the nonlinear region in a resonant cavity, the source obtains an enhanced nonlinear interaction and naturally filters out photons by frequency according to the cavity linewidth. Among various platforms, X-cut thin-film lithium niobate (TFLN) stands out for its strong second-order optical nonlinearity (χ(2)χ^{(2)}χ(2)) and access to a strong platform for modulating light. Although previously demonstrated, present sources are limited in their photon pair channel availability, limiting the potential of quantum applications in quantum information processing, communication, and sensing that can scale in robustness by having access to multiple photon pair channels. To this end, we demonstrate a photon pair source on X-cut TFLN with 80 measured photon pair channels spanning the C and L optical bands with a frequency spacing of 49.5 GHz between photons. We characterize the second-order correlation function and pair generation rate (PGR) of 80 channels, the highest number of channels demonstrated to date, and achieve a pair generation of 125.7 kHz / μW after accounting for the cavity's escape efficiency. We also demonstrate heralded single photon operation by calculating a heralded auto-correlation dip of 0.0544 ±\pm± 0.0054 with 2.2 mW of on-chip pump power. These findings demonstrate the promise of X-cut TFLN as a strong platform for quantum optical applications.
In this Letter, we theoretically study spontaneous parametric downconversion (SPDC) in a periodically poled structure composed of two linearly uncoupled resonators that are nonlinearly coupled via a Mach-Zehnder interferometer. The device does not require dispersion engineering to achieve efficient doubly resonant SPDC, and, unlike the case of a single resonator, one can reconfigure the system to generate photon pairs over a bandwidth of hundreds of nm. We consider the case of SPDC pumped at 775 nm in a periodically poled lithium niobate (PPLN) device compatible with up-to-date technological platforms. We calculated pair generation rates of up to 250 MHz/mW pump power for a single resonance and integrated pair generation rates of up to 100 THz/mW pump power over 170 nm. When properly reconfigured, a single device can efficiently generate over a bandwidth of some 300 nm, covering the S, C, L, and U infrared bands.
Chip-integrated photon-pair sources based on spontaneous parametric down-conversion (SPDC) have emerged as a promising solution for scalable quantum light generation. Thin-film lithium tantalate (TFLT) is a compelling χ(2)χ^{(2)}χ(2) platform, combining strong nonlinearity with a high optical-damage threshold, weak photorefractive response, and ferroelectricity that enables quasi-phase matching. However, SPDC-based photon-pair generation on TFLT has not yet been demonstrated. Here, we combine high-quality periodic poling with low-loss nanophotonic waveguides to realize photon-pair sources on TFLT in both traveling-wave and resonant configurations. In periodically poled straight waveguides, we achieve broadband photon-pair generation with high efficiency (2.1 GHz mW−12.1~\mathrm{GHz}~\mathrm{mW}^{-1}2.1 GHz mW−1) and coincidence-to-accidental ratio (up to 3.8×1053.8\times10^{5}3.8×105). We further confirm high-purity single-photon operation via heralded second-order correlation (gH(2)(0)=0.0018±0.0002g^{(2)}_\mathrm{H}(0) = 0.0018 \pm 0.0002gH(2)​(0)=0.0018±0.0002) and high-fidelity time-energy entanglement through Franson interference (visibility of 98.9±0.5%98.9 \pm 0.5\%98.9±0.5%). In periodically poled racetrack resonators, we map out a broad quantum frequency comb spanning the telecom C- and L-bands. By isolating individual frequency-correlated pairs, we measure a high spectral brightness of 11 GHz mW−1 GHz−111~\mathrm{GHz}~\mathrm{mW}^{-1}~\mathrm{GHz}^{-1}11 GHz mW−1 GHz−1. These results are competitive with the state of the art across χ(2)χ^{(2)}χ(2) integrated platforms, positioning TFLT as a strong contender for integrated quantum light sources, with applications in wavelength-multiplexed quantum communications and photonic quantum information processing.
Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.