Array-form ultrahigh sensitivity single-beam atomic magnetometers are ideal for high-resolution biomagnetic imaging applications, such as magnetocardiography and magnetoence-phalography. In the low-frequency range of interest for biomagnetism, an essential reason for the deterioration of atomic magnetometer low-frequency sensitivity is the light shift noise caused by temperature fluctuations of the pump laser. Accordingly, this article proposes a new frequency response model of the atomic magnetometer sensitivity, treating light shift as a time-dependent variable. The model reveals the frequency relationship between the deterioration of atomic magnetometer sensitivity and the low-frequency light shift. A new method for suppressing the low-frequency light shift noise based on precise laser temperature control is deduced from the frequency response model, significantly improving the average sensitivity of atomic magnetometers by over 30%. This study presents a theoretical foundation for investigating the low-frequency light shift in atomic magnetometers from a novel perspective and contributes to the optimization of biomagnetic imaging systems composed of single-beam atomic magnetometers.
Array-form ultrahigh sensitivity single-beam atomic magnetometers are ideal for high-resolution biomagnetic imaging applications, such as magnetocardiography and magnetoence-phalography. In the low-frequency range of interest for biomagnetism, an essential reason for the deterioration of atomic magnetometer low-frequency sensitivity is the light shift noise caused by temperature fluctuations of the pump laser. Accordingly, this article proposes a new frequency response model of the atomic magnetometer sensitivity, treating light shift as a time-dependent variable. The model reveals the frequency relationship between the deterioration of atomic magnetometer sensitivity and the low-frequency light shift. A new method for suppressing the low-frequency light shift noise based on precise laser temperature control is deduced from the frequency response model, significantly improving the average sensitivity of atomic magnetometers by over 30%. This study presents a theoretical foundation for investigating the low-frequency light shift in atomic magnetometers from a novel perspective and contributes to the optimization of biomagnetic imaging systems composed of single-beam atomic magnetometers.
Quantum manipulation technology and photoelectric detection technology have jointly facilitated the rapid development of ultra-sensitive atomic spin magnetometers. To improve the output signal and sensitivity of the spin-exchange-relaxation-free (SERF) atomic spin magnetometer, the noises influencing on the output signal and the sensitivity were analyzed, and the corresponding noise suppression methods were presented. The magnetic field noises, including the residual magnetic field noise and the light shift noise, were reduced to approximately zero by employing the magnetic field compensation method and by adjusting the frequency of the pump beam, respectively. With respect to the operation temperature, the simulation results showed that the temperature of the potassium atomic spin magnetometer realizing the spin-exchange relaxation-free regime was 180 °C. Moreover, the fluctuation noises of the frequency and the power were suppressed by using the frequency and the power stable systems. The experimental power stability results showed that the light intensity stability was enhanced 10%. Contrast experiments on the sensitivity were carried out to demonstrate the validity of the suppression methods. Finally, a sensitivity of 13 fT/Hz(1/2) was successfully achieved by suppressing noises and optimizing parameters.
The light shift represents a major source of measurement error and system noise in optically pumped atomic magnetometers (OPAMs). Tuning the laser frequency to a specific value is a common and effective approach to suppressing light shift in many optical-pumping systems. However, when this method is applied to OPAMs, a significant issue arises: at the zero-light-shift frequency, the magnetometer’s sensitivity decreases markedly. Consequently, it is not possible to optimize simultaneously both the measurement accuracy affected by the light shift and the overall sensitivity of the magnetometer. To address this contradiction, the underlying mechanism was analyzed using the theory of light absorption and the principles governing light–atom interactions, leading to the proposal of a dual-frequency optical-pumping scheme. Experimental results demonstrate that this approach can suppress the light shift by more than 95% while maintaining the optimal sensitivity of the OPAM. The proposed dual-frequency scheme can also be extended to other circularly polarized optical-pumping systems, thereby facilitating both the enhancement of OPAM performance and its practical deployment in real-world applications.
We demonstrate a single-beam atomic magnetometer (AM) capable of measuring a three-axis magnetic field with high-sensitivity, achieved by applying a small DC offset field and a high frequency modulation field. To satisfy the miniaturization demand of AMs, an elliptically polarized light detuned by 50 GHz from the resonance transition center is employed. The circularly polarized component is used to polarize the alkali-metal atoms, while the linearly polarized light is used to detect the dynamics of the polarized spin under a magnetic field. Based on theoretical analysis, parameters that significantly affect the performance are optimized, and a sensitivity of 20 fT/Hz 1/2 in x -axis, 25 fT/Hz 1/2 in y -axis, 30 fT/Hz 1/2 in z -axis is achieved with a miniature 4 × 4 × 4 mm 87 Rb vapor cell. Moreover, we also verify that the operation principle of AMs can be used to null background magnetic fields in-situ with isotropic compensation resolution of 6.7 pT, which provides an effectively precise method for zeroing ambient magnetic field. The high-sensitivity operating of an elliptically-polarized-laser-based magnetometer provides prospective futures for constructing a compact, low-cost AM, which is particularly applicable for non-invasive bio-magnetic imaging such as array-based magnetoencephalography (MEG) and magnetocardiography (MCG).
Single-beam optically pumped atomic magnetometers (OPAMs) represent promising candidates for applications in geomagnetic field monitoring, biomedicine, and various other precision sensing domains owing to their exceptional sensitivity, high measurement accuracy, and cost-effectiveness. However, in orientation-based OPAMs utilizing circularly polarized light (CPL) pumping, the off-resonant light introduces light shift. The light shift acts as an additional magnetic field, reducing the measurement accuracy of OPAMs. Moreover, the dependence of the light shift on light intensity and frequency facilitates the conversion of light noise into magnetic noise, thereby degrading the sensitivity of OPAMs. In this study, we propose an optical pumping scheme based on space division multiplexing light (SDML) to suppress the light shift in OPAM. The approach employs two orthogonally polarized linearly polarized beams with a controlled phase difference to generate a spatially periodic distribution of left- and right-handed CPL. Optical pumping with the SDML induces oppositely directed light shifts in distinct spatial regions that effectively cancel each other. Finally, it is verified by experiments that the light shift is greatly suppressed based on SDML. Under detuned SDML pumping, both the light shift and light intensity noise are suppressed by over 50%, while maintaining a sensitivity comparable to that achieved with conventional CPL pumping. The proposed method demonstrates significant potential for magnetometers in light-noise-prone environments, and it can be generalized to other orientation-based magnetometers that rely on CPL pumping.
Atomic magnetometers operated in spin-exchange relaxation-free (SERF) have the potential to replace superconducting quantum interference devices (SQUIDs) in the field of biomagnetism. Here, we demonstrate the dual-axis closed-loop control of a single-beam SERF magnetometer that allows sensing of two orthogonal magnetic fields simultaneously and independently with suppressed cross-talk effect, achieved by applying a rotating modulation field and using of the negative feedback. Operating in the dual-axis closed-loop mode with a miniature 4 × 4 × 4 mm 87Rb cell, we achieve magnetic field sensitivity of 20 fT/Hz1/2 and a bandwidth of 1.8 kHz. In addition to the experimental study of the sensitivity and bandwidth, we perform a theoretical analysis to the dual-axis response and develop an effective decoupling method. The implementation of closed-loop control enables the magnetometer to be robust against the disturbance of the ambient field, which could enlarge the dynamic range, enhance the systematic stability, and suppress the cross-talk effect. Such a simple, yet high-performance SERF magnetometer could be suitable as a promising candidate in the field of biomagnetism, allowing for a denser sensor array and opening up new possibilities for the noninvasive biomagnetic imaging.
The light shift in a spin-exchange relaxation-free (SERF) atomic magnetometer (AM) generated by detuning of circularly polarized pump light, results in deviations of orthogonality measurement and attenuation of magnetometer response. In this paper, we propose and systematically investigate a dual-axis method to suppress light shift based on a self-developed single-beam compact SERF AM capable of measuring magnetic field components along two orthogonal sensitive axes. By sequentially observing the non-sensitive axis response and applying a magnetic field along the pump light direction, the virtual magnetic field induced by light shift is compensated and is rigorously demonstrated as a dominant component in this direction. Experimental results show a significant reduction in crosstalk between the dual sensitive axes, improving accuracy in resonant frequency determination of87Rb atoms and orthogonality evaluation of triaxial coils. Furthermore, the performance of dual-axis measurement in the SERF AM is tested, showing a more notable enhancement than that of single-axis measurement.