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Frontiers in Quantum Science and Technology

Quantum entanglement of optical photons: the first experiment, 1964–67

Carl A. Kocher

Published Aug 22, 2024• 4 citations
Publisher

Abstract

The first experimental observation of entangled visible light was achieved by optically exciting free atoms of calcium and detecting pairs of photons emitted in a two-stage cascade. The polarizations of the entangled photons were observed to be correlated, in agreement with quantum theory. This review describes the rationale, methodology, challenges, and results, including experimental details not previously published.

DOI
10.3389/frqst.2024.1451239

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The first experimental observation of entangled visible light was achieved by optically exciting free atoms of calcium and detecting pairs of photons emitted in a two-stage cascade. The polarizations of the entangled photons were observed to be correlated, in agreement with quantum theory. This review describes the rationale, methodology, challenges, and results, including experimental details not previously published.
The first two-photon entanglement experiment performed 50 years ago by Kocher and Commins (KC) provided isolated pairs of entangled photons from an atomic three-state fluorescence cascade. In view of questioning of Bell’s theorem, data from these experiments are re-analyzed and shown sufficiently precise to confirm quantum mechanical and dismiss semi-classical theory without need for Bell’s inequalities. Polarization photon correlation anisotropy (A) is useful: A is near unity as predicted quantum mechanically and well above the semi-classic range, 0⩽A⩽1/2. Although yet to be found, one may envisage a three-state molecule emitting entangled photon pairs, in analogy with the KC atomic system. Antibunching in fluorescence from single molecules in matrix and entangled photons from quantum dots promise it be possible. Molecules can have advantages to parametric down-conversion as the latter photon distribution is Poissonian and unsuitable for producing isolated pairs of entangled photons. Analytical molecular applications of entangled light are also envisaged.
We report an experimental demonstration of entanglement swapping over two quantum stages. By successful realizations of two cascaded photonic entanglement swapping processes, entanglement is generated and distributed between two photons, that originate from independent sources and do not share any common past. In the experiment we use three pairs of polarization entangled photons and conduct two Bell-state measurements: one between the first and second pair, and one between the second and third pair. This results in projecting the remaining two outgoing photons from pair 1 and 3 into an entangled state, as characterized by an entanglement witness. The experiment represents an important step towards a full quantum repeater where multiple entanglement swapping is a key ingredient.
Non-classical states of light are of fundamental importance for emerging quantum technologies. All optics experiments producing multi-qubit entangled states have until now relied on outcome post-selection, a procedure where only the measurement results corresponding to the desired state are considered. This method severely limits the usefulness of the resulting entangled states. fiere, we show the direct production of polarization- entangled photon triplets by cascading two entangled down-conversion processes[1]. First, a Sagnac source [2] produces non-degenerate entangled photon pairs at 776 nm and 842 nm in a Bell state. The 776 nm photon is sent through a polarizing Mach-Zehnder interferometer with a down-conversion crystal in each arm. If it is down-converted, a photon pair is created in modes 2 and 3 with a polarization state depending on the pump photon. The quantum stete describing the photon triplets is:
We study, experimentally and theoretically, temporal correlations between the polarization of photon pairs emitted during the biexciton-exciton radiative cascade from a single semiconductor quantum dot, optically excited by a continuous-wave light source. The system is modeled by a Lindbladian coupled to two Markovian baths: One bath represents the continuous light source, and a second represents the emitted radiation. Very good agreement is obtained between the theoretical model that we constructed and a set of 36 different time-resolved, polarization correlation measurements between cascading photon pairs.