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npj Nanophotonics

Analysis, recent challenges and capabilities of spin-photon interfaces in Silicon carbide-on-insulator

Joshua Bader, Hamed Arianfard, Alberto Peruzzo, Stefania Castelletto

Published Aug 2, 2024• 9 citations
Publisher

Abstract

Abstract Silicon-carbide (SiC) is a promising platform for long-distance quantum information transmission via single photons, offering long spin coherence qubits, excellent electronic and optical characteristics and CMOS-compatibility. We review key properties of spin-photon interface components for future deployment on the SiC-on-insulator platform with detailed insights provided for available color centers as well as integrated photonic circuits. The associated challenges to achieve high-fidelity multi-qubit control and photon-mediated entanglement on-chip are elaborated, perspectively.

DOI
10.1038/s44310-024-00031-8

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Abstract Silicon carbide (SiC) is an excellent industrially compatible material, which has been widely used in high power electronic devices. Recently, spin defects in SiC have been found to be a high-quality spin-to-photon interface with long spin coherence time and high spin-selective optical transition. Spin states can be initialized and readout with extremely high fidelity. The infrared and even telecom fluorescence is suited for fiber communication with less scatting loss. The bandwidth of intrinsic zero-phonon-line emission can be manipulated by classical electrical devices. The achieved near lifetime-limited optical linewidths greatly increase the indistinguishability of photon emission and facilitate the connection with other narrowband absorption quantum systems, such as cold atoms, trapped ions, and rare-earth dopants in crystals. Moreover, spin defects coupled with photonic nanocavities have been demonstrated, which can greatly enhance the photon emission in the zero-phonon-line. The realization of controllable electron-nuclear spin entanglement further extends the memory-based quantum applications. In this perspective, we will briefly discuss the most recent development of spin defects in SiC. These results show that spin defects in SiC are desirable quantum platforms for quantum networking applications. We also discuss some of the current challenges and possible future development.
Quantum communication promises unprecedented capabilities enabled by the transmission of quantum states of light. However, current implementations face severe distance limitations due to photon loss. Silicon carbide (SiC) defects have emerged as a promising quantum device platform, offering strong optical transitions, long spin coherence lifetimes and the opportunity for integration with semiconductor devices. Some defects with optical transitions in the telecom range have been identified, allowing to interface with fiber networks without the need for wavelength conversion. These unique properties make SiC an attractive platform for the implementation of quantum nodes for quantum communication networks. We provide an overview of the most prominent defects in SiC and their implementation in spin-photon interfaces. Furthermore, we model an exemplary, memory-enhanced quantum communication protocol in order to extract the parameters required to surpass a direct point-to-point link performance. Based on these insights, we summarize the key steps required towards the deployment of SiC devices in large-scale quantum communication networks.
The PL6 color center in silicon carbide has recently emerged as a promising platform for quantum information processing, yet its coherent spin--photon interface has remained largely unexplored. Here we present a comprehensive investigation of single PL6 centers, combining spectroscopy with theoretical analysis. The excited-state fine structure is fully resolved using group-theoretical modeling and strain-dependent measurements. Under resonant excitation, we achieve a spin initialization fidelity of 99.69±0.03%99.69 \pm 0.03\%99.69±0.03% and a readout contrast of 98.31±1.03%98.31 \pm 1.03\%98.31±1.03%. The spin--photon--entangled A2A_2A2​ transition exhibits narrow optical linewidths (∼180\sim 180∼180~MHz) and a polarization visibility of ∼82%\sim 82\%∼82%. Coherent optical driving enables Rabi frequencies up to 2.8952.8952.895~GHz, while dynamical decoupling extends the spin coherence time from 0.50.50.5~ms to 5.705.705.70~ms. Our results establish PL6 as a competitive solid-state spin--photon interface hosted in a commercially available semiconductor platform.
Color centers in wide bandgap semiconductors are prominent candidates for solid-state quantum technologies due to their attractive properties including optical interfacing, long coherence times, and spin–photon and spin–spin entanglement, as well as the potential for scalability. Silicon carbide color centers integrated into photonic devices span a wide range of applications in quantum information processing in a material platform with quantum-grade wafer availability and advanced processing capabilities. Recent progress in emitter generation and characterization, nanofabrication, device design, and quantum optical studies has amplified the scientific interest in this platform. We provide a conceptual and quantitative analysis of the role of silicon carbide integrated photonics in three key application areas: quantum networking, simulation, and computing.
Optically addressable solid-state spin defects are promising candidates for storing and manipulating quantum information using their long coherence ground-state manifold; individual defects can be entangled using photon-photon interactions, offering a path toward large-scale quantum photonic networks.Quantum computing protocols place strict limits on the acceptable photon losses in the system.These lowloss requirements cannot be achieved without photonic engineering, but are attainable if combined with state-of-the-art nanophotonic technologies.However, most materials that host spin defects are challenging to process: as a result, the performance of quantum photonic devices is orders of magnitude behind that of their classical counterparts.Silicon carbide (SiC) is well suited to bridge the classical-quantum photonics gap, since it hosts promising optically addressable spin defects and can be processed into SiC-on-insulator for scalable, integrated photonics.In this paper, we discuss recent progress toward the development of scalable quantum photonic technologies based on solid-state spins in silicon carbide, and discuss current challenges and future directions.