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Photonics for Quantum (PfQ)

Quantum dot coherent control for quantum communication

Gregor Weihs

Published Aug 2, 2024• 0 citations
Publisher

Abstract

Temporal encodings of quantum information are prevalent in applications because of their suitability for long-distance quantum communication and their compatibility with optical fiber communication networks. Perhaps the simplest temporal encoding is time-bin encoding, i. e. in superpositions of two (or more) temporally separated optical pulses. Early attempts at generating time-bin entanglement from single quantum emitters was not able to avoid the problem of re-excitation or was converted probabilistically from polarization entangled photon pairs from a quantum dot. Direct generation requires a metastable level to carry the coherence and avoid double pair emission into the desired time bins. In order to use dark exciton states as metastable states we have worked on their efficient creation and coherent control in the presence of in-plane magnetic fields. Much of this is based on our recent work on advanced excitation schemes using chirped pulses. With chirped pulses we are now able to deterministically populate a dark exciton state and to transfer this population to the biexciton, which can then emit a photon pair.

DOI
10.1117/12.3028913

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Temporal encodings of quantum information are prevalent in applications because of their suitability for long-distance quantum communication and their compatibility with optical fiber communication networks. Perhaps the simplest temporal encoding is time-bin encoding, i. e. in superpositions of two (or more) temporally separated optical pulses. Early attempts at generating time-bin entanglement from single quantum emitters was not able to avoid the problem of re-excitation or was converted probabilistically from polarization entangled photon pairs from a quantum dot. Direct generation requires a metastable level to carry the coherence and avoid double pair emission into the desired time bins. In order to use dark exciton states as metastable states we have worked on their efficient creation and coherent control in the presence of in-plane magnetic fields. Much of this is based on our recent work on advanced excitation schemes using chirped pulses. With chirped pulses we are now able to deterministically populate a dark exciton state and to transfer this population to the biexciton, which can then emit a photon pair.
Summary form only given. A realization of time-bin entanglement obtained from quantum dots would join the strength of long distance transmission that characterizes this type of entanglement with the single photon state purity of the quantum dot emission. Compared with polarization entanglement from quantum dots this scheme does not require elimination of the fine structure splitting responsible for partial distinguishability of the quantum dot cascades [1].Here, we present our results on coherent and resonant excitation of quantum dots, creation of photon pairs, scattering free emission and measurement of the high purity of the emitted photons [2, 3]. In addition, we will show our measurements of the generated time-bin entanglement. To excite a single quantum dot we performed two-photon resonant excitation of the biexciton state. Here, we exploited the biexciton binding energy in order to use the laser light which was not resonant to any photon emitted from the quantum dot (Fig. 1a). Our measurements were performed on a single self-assembled InAs/GaAs quantum dot. We confirmed the resonant nature of the excitation by observing Rabi oscillations (Fig. 1b). Additionally, we performed Ramsey interference measurement and determined the coherence time of the ground-biexciton state superposition. These measurements show that we can coherently transfer the phase of the excitation laser onto the quantum dot system, a necessary requirement to obtain time-bin entanglement.To test the statistics of the emitted state we measured the auto-correlation of the emitted photons (Fig. 3c). Here, the auto-correlation parameter at zero delay was measured to be 0.012(1) without and 0.0073(8) with background subtraction. In addition, we performed a measurement to characterize the state emitted from a quantum dot using a witness-based criterion described in [4]. With this measurement we experimentally confirmed that the resonantly excited quantum dot emits a non-Gaussian state of light (Fig. 1d). This measurement is the first of this nature ever performed on a semiconductor single photon emitter.
We report a study on coherence of excitation of single quantum dots. We address the coherent excitation of biexcitons, the process that is indispensable for deterministic photon pair generation in quantum dots. Based on theoretical modeling we optimized the duration of the excitation pulse in our experiment to minimize the laser-induced dephasing and increase the biexciton-to-background single-exciton occupation probability. An additional effect of this approach is a high degree of time-bin entanglement with a concurrence of up to 0.78(6) and a 0.88(3) overlap with a maximally entangled state.
The strong confinement of semiconductor excitons in a quantum dot gives rise to atomlike behavior. The full benefit of such a structure is best observed in resonant excitation where the excited state can be deterministically populated and coherently manipulated. Because of the large refractive index and device geometry it remains challenging to observe resonantly excited emission that is free from laser scattering in III/V self-assembled quantum dots. Here we exploit the biexciton binding energy to create an extremely clean single photon source via two-photon resonant excitation of an InAs/GaAs quantum dot. We observe complete suppression of the excitation laser and multiphoton emissions. Additionally, we perform full coherent control of the ground-biexciton state qubit and observe an extended coherence time using an all-optical echo technique. The deterministic coherent photon pair creation makes this system suitable for the generation of time-bin entanglement and experiments on the interaction of photons from dissimilar sources.
Semiconductor Quantum dots are potentially an attractive source of non-classical light. They can confine bound electron-hole pairs, excitons, in all three spatial dimensions giving them discrete optical emission energies, much like the electronic states in atomic systems. The semiconductor nature of the system allows quantum dots to be integrated into complicated device structures including optical cavities [1] and electrical injection [2]. The radiative exciton emission from a semiconductor quantum dot can provide the simplest form of quantum light, a single photon source [2]. The finite re-excitation time following the radiative decay of an exciton in a quantum dot prevents the dot from emitting more than one photon if excited with a short optical or electronic pulse. In a similar fashion excitation of the biexciton state, consisting of two electrons and holes, in the quantum dot results in the emission of a pair of photons at the energy of the biexciton and exciton transitions. The biexciton state was, in fact, proposed as a possible source of polarisation-entangled photons in 2000 by Benson et al. [3] as it consists of two polarisation-correlated decay paths which could potentially be indistinguishable. The condition of indistinguishability is fundamental to the generation of entangled photons and is, in general, not true of the two decay paths from the biexciton state in a quantum dot; physical anisotropy causes the intermediate exciton states to hybridise and separate in energy providing ‘which-path’ information about the route taken through the biexciton decay. We demonstrate how the splitting between the intermediate exciton states in a single InAs quantum dot can be controlled by growth [4], rapid thermal annealing [5] and the application of an external magnetic field [6]. Each of these three techniques can be used to make the intermediate exciton states degenerate allowing the biexciton decay to produce singe pairs of entangled photons triggered by short laser pulses [7,8]. Entangled photon pair sources are essential for applications such as entanglement based quantum key distribution, and optical quantum computing. For these applications it is important that no more than one entangled photon pair is generated in a cycle, a requirement met by our quantum dot source which is not possible with traditional methods for generating entangled pairs of photons. Entanglement also enables quantum interferometry and metrology, the basis of image resolution beyond that possible with equivalent classical light. Biphoton interferometry using entangled emission from the biexciton decay reveals fringes with half the period of classical light [9], and less that that of the laser. In addition, interferometry suggests that this type of entangled light source is not limited by decoherence, we fine the biphoton is surprising robust against dephasing, in stark contrast to the devastating effect of decoherence upon single photons emitted by similar structures.
The next generation of telecommunication networks will rely on the transmission of complex quantum states to enable secure and transformative information processing, utilizing entanglement and superposition. Cluster states - multipartite entangled states that retain entanglement under local measurements - are a vital resource for quantum networking applications such as blind photonic quantum computing, quantum state teleportation and all-photonic quantum repeaters. However, the transmission of cluster states over optical fiber has remained elusive with previous approaches. Here, we demonstrate the first transmission of a four-qubit cluster state over 25 km of single-mode fiber by using a two-photon multi-level time-bin encoding. We directly generate the state by exploiting coherent control of a parametric generation process, rendering a resource-intensive controlled-phase gate obsolete. To enable efficient and reconfigurable projective measurements on the multi-level time-bin encoded state, we introduce chirped-pulse modulation and implement the first time-bin beam splitter, allowing us to certify genuine multipartite entanglement and to demonstrate one-way computing operations. Our approach enables the transmission of complex quantum states over long-distance fibers, permitting the implementation of multipartite protocols and laying the foundation for large-scale quantum resource networks.