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Europhysics Letters (EPL)

Enhanced optical pumping using mutually orthogonal magnetic fields for quantum sensing

Sudip Mandal, Raghwinder Singh Grewal, Swarupananda Pradhan

Published Jul 2, 2024• 0 citations
Publisher

Abstract

Abstract The atomic population trapped in irrelevant atomic states is a limiting factor for sensors based on laser-atom interaction. Using a bi-chromatic light field along with a specific combination of magnetic fields, we show a significant increase in the amplitude ( i.e. , more than seven times) of a two-photon coherent population trapping (CPT) resonance, which can be effectively used for atomic magnetometry. This increase in amplitude can be explained through enhanced optical pumping via the transfer of population to the relevant Zeeman states. Our experimental observations are consistent with the theoretical calculations carried out for a realistic three-level atomic system using density matrix formalism. We further discuss the optimum condition for enhanced optical pumping by adjusting the ground-state decoherence rate. Enhanced optical pumping through the manipulation of the magnetic field is quite important and is of great interest in the field of quantum technology.

DOI
10.1209/0295-5075/ad5e1c

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Abstract The atomic population trapped in irrelevant atomic states is a limiting factor for sensors based on laser-atom interaction. Using a bi-chromatic light field along with a specific combination of magnetic fields, we show a significant increase in the amplitude ( i.e. , more than seven times) of a two-photon coherent population trapping (CPT) resonance, which can be effectively used for atomic magnetometry. This increase in amplitude can be explained through enhanced optical pumping via the transfer of population to the relevant Zeeman states. Our experimental observations are consistent with the theoretical calculations carried out for a realistic three-level atomic system using density matrix formalism. We further discuss the optimum condition for enhanced optical pumping by adjusting the ground-state decoherence rate. Enhanced optical pumping through the manipulation of the magnetic field is quite important and is of great interest in the field of quantum technology.
The atomic population trapped in uncoupled atomic states is a limiting factor for processes based on laser-atom interaction. The use of repump laser, bi-chromatic field, and vector magnetic field are explored in degenerate as well as non-degenerate atomic system to overcome the limitation. The magnetic resonance of 85Rb atoms under these complementary conditions are investigated in a buffer gas filled cell. The most suitable condition is achieved by the combined action of a bi-chromatic light with a specific combination of magnetic fields for non-degenerate levels where the relevant magnetic resonance shows more than 7-fold increase in its amplitude. The phenomenon is consistently observed through RF as well as magnetic field de-modulation technique. It will lead to similar improvement in the sensitivity of the atomic magnetometers. The optical pumping of the atomic population to the stretch state by manipulation of magnetic field will be of general interest involving quantum technology.
In the Λ three-level system, we will make use of semi-classical density matrix method to analyze cesium (Cs) hyperfine structure of coherent population trapping (CPT) phenomenon. Coherent population trapping has been widely used in electromagnetically induced transparency, non-inversion laser, optical storage and ultra-slow speed of light fields, then strong-coupling light and weak detecting light form coherent laser light to change the hyperfine structure energy levels of particles number distribution, which impacts on laser pumping magnetic resonance. In this paper, we will discuss the theoretical analysis and system design of laser pumping cesium magnetometer, cesium atomic energy level formed hyperfine structure with the I-J coupling, the hyperfine structure has been further split into Zeeman sublevels for the effects of magnetic field. To use laser pump and RF magnetic field make electrons transition in the Zeeman sublevels to produce the results of magneto-optical double resonance and on this basis we analyze the influence of laser pumping magnetic resonance based on coherent population trapping.
We report our study on coherent population trapping (CPT) in a $\ensuremath{\Lambda}$ configuration coupled by magnetic dipole interactions. The $\ensuremath{\Lambda}$ configuration is formed by bichromatic radio-frequency fields coupling a pair of Zeeman sublevels in one hyperfine level of an alkali-metal atom to another sublevel in the other hyperfine level. The Zeeman sublevel at the apex is coupled to a state in the nPnPnP manifold via an optical transition on one of the spectroscopic DDD lines to induce optical pumping to a dark state. The configuration is closed without leakage to other Zeeman sublevels. We use lithium atoms in an optical trap for our experimental study. The system allows independent control of the main parameters characterizing CPT, which include the upper-state decay rate and the decoherence rate as well as the Rabi frequencies. By turning off the applied fields, the system is frozen so that its quantum state can be measured precisely. We studied the line shapes and dynamics of the CPT system, and measured the phase relation of the dark superposition state to find excellent agreement with theory. The possible application of the scheme as a method to cool optically trapped atoms below the recoil limit in a manner analogous to velocity-selective coherent population trapping is discussed.
This work is concerned with the temporal evolution of the coherent population trapping (CPT) process in the case of additional optical pumping to states not contributing to the CPT superposition states. Special attention is paid to the influence of weak external magnetic fields that can change the laser-atom interaction considerably. The theoretical analysis is completed by experimental observations on a sodium atomic beam, which show good agreement with our theory. The results obtained are of importance for a realistic picture of CPT schemes in practical applications.
We report the observation of enhanced magneto-optic rotation as the coherent superposition of different hyperfine states is established in an atomic sample. The polarization rotation near the two-photon Raman resonance condition appears to have an analogous characteristic to the well established Faraday rotation observed in the vicinity of a single-photon resonance; however, it contains sharp features arising from coherent population trapping states. The profile of the two-photon rotation signal exhibits interesting features for a slightly imbalanced circular polarization component of the laser field as well as for on and away from the single-photon resonance. The investigation can be used to explore the effect of superposition states generated by coherent population trapping on optical activity. A complete density matrix based numerical simulation that consistently captures all the relevant features of the experiment is presented. The experimental and theoretical investigation can be useful for magnetometry using polarization rotation near two-photon Raman resonance.
This paper reports experimental investigations of the spectral response of synchronous coherent population trapping (CPT) for magnetometry applications. Synchronous CPT is demonstrated using resonant two-photon excitation with a modulated bichromatic laser field in the 87RbD1^{87}\mathrm{Rb} {D}_{1}87RbD1​ manifold. Spectra containing multiple magnetic resonances are produced due to two-photon excitations created by various frequency components of the modulated beam. Theoretical modeling based on the atomic density-matrix equations is used to simulate the spectral response of synchronous CPT. Our results show potential advantages of synchronous CPT over synchronous optical pumping for magnetic field measurement. Magnetic resonance signals produced by synchronous CPT can be used in eliminating the dead-zone problem and also in determining the magnetic field direction.