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Journal of the Optical Society of America B

Jaynes–Cummings model breaks down when the cavity geometry significantly reduces free-space emission

Martin Blaha, Arno Rauschenbeutel, Jürgen Volz

Published Jun 17, 2024• 2 citations
Publisher

Abstract

Strong coupling between a single resonator mode and a single quantum emitter is key to a plethora of experiments and applications in quantum science and technology and is commonly described by means of the Jaynes–Cummings model. Here, we show that the Jaynes–Cummings model only applies when the cavity does not significantly change the emitter’s decay rate into free-space. Most notably, the predictions made by the Jaynes–Cummings model become increasingly wrong when approaching the ideal emitter-resonator systems with no free-space decay channels. We present a Hamiltonian that provides, within the validity range of the rotating wave approximation, a correct theoretical description that applies to all regimes. As minimizing the coupling to free-space modes is paramount for many cavity-based applications, a correct description of strong light-matter interaction is therefore crucial for developing and optimizing quantum protocols.

DOI
10.1364/josab.522498

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Strong coupling between a single resonator mode and a single quantum emitter is key to a plethora of experiments and applications in quantum science and technology and is commonly described by means of the Jaynes–Cummings model. Here, we show that the Jaynes–Cummings model only applies when the cavity does not significantly change the emitter’s decay rate into free-space. Most notably, the predictions made by the Jaynes–Cummings model become increasingly wrong when approaching the ideal emitter-resonator systems with no free-space decay channels. We present a Hamiltonian that provides, within the validity range of the rotating wave approximation, a correct theoretical description that applies to all regimes. As minimizing the coupling to free-space modes is paramount for many cavity-based applications, a correct description of strong light-matter interaction is therefore crucial for developing and optimizing quantum protocols.
Strong coupling between a single resonator mode and a single quantum emitter is key to a plethora of experiments and applications in quantum science and technology and is commonly described by means of the Jaynes-Cummings model. Here, we show that the Jaynes-Cummings model only applies when the cavity does not significantly change the emitter's emission rate into free-space. Most notably, the predictions made by the Jaynes-Cummings model become increasingly wrong when approaching the ideal emitter-resonator systems with no free-space decay channels. We present a Hamiltonian that provides, within the validity range of the rotating wave approximation, a correct theoretical description that applies to all regimes. As minimizing the coupling to free-space modes is paramount for many cavity-based applications, a correct description of strong light-matter interaction is therefore crucial for developing and optimizing quantum protocols.
As atom-cavity systems are becoming more sophisticated, the limitations of the Jaynes-Cummings model are becoming more apparent. In this paper, we therefore take a more dynamical approach to the modelling of atom-cavity systems and do not reduce the electromagnetic field inside the resonator to a single mode. Our approach shows that the decay rate Gamma_cav of an emitter inside a subwavelength cavity with metallic mirrors can be much larger than its free space decay rate Gamma_free due to constructive interference effects of the emitted light. In general, however, we find that Gamma_cav = Gamma_free to a very good approximation which might explain why atom-cavity experiments with planar mirrors have not been able to operate in the so-called strong coupling regime.
As atom-cavity systems are becoming more sophisticated, the limitations of the Jaynes-Cummings model are becoming more apparent. In this paper, we therefore take a more dynamical approach to the modelling of atom-cavity systems and do not reduce the electromagnetic field inside the resonator to a single mode. Our approach shows that the decay rate [Formula: see text] of an emitter inside a subwavelength cavity with metallic mirrors can be much larger than its free space decay rate [Formula: see text] due to constructive interference effects of the emitted light. In general, however, we find that [Formula: see text] to a very good approximation which might explain why atom-cavity experiments with planar mirrors have not been able to operate in the so-called strong coupling regime.
The interaction of an ensemble of NNN two-level quantum emitters with a single-mode electromagnetic field is described by the Tavis-Cummings model. There, the collectively enhanced light-matter coupling strength is given by gN=Ng‾1{g}_{N}=\sqrt{N}{\overline{g}}_{1}gN​=N​g​1​, where g‾1{\overline{g}}_{1}g​1​ is the ensemble-averaged single-emitter coupling strength. This model has been employed to describe and to analyze numerous cavity-based experiments. Here, we show that this is only justified if the effective scattering rate into noncavity modes is negligible compared to the cavity's free-spectral range. In terms of experimental parameters, this requires that the optical depth of the ensemble is low, a condition that is violated in several state-of-the-art experiments. We give quantitative conditions for the validity of the Tavis-Cummings model and derive a more general Hamiltonian description that takes into account the cascaded interaction of the photons with all consecutive emitters. We show that the predictions of our cascaded model can differ quantitatively and even qualitatively from those obtained with the Tavis-Cummings model. Finally, we present experimental data, for which the deviation from the predictions of the Tavis-Cummings model is apparent. Our findings are relevant for all experiments in which optically dense ensembles of quantum emitters are coupled to an optical resonator.
The Jaynes-Cummings Hamiltonian is at the core of cavity quantum electrodynamics; however, it relies on bound-electron emitters fundamentally limited by the binding Coulomb potential. In this work, we propose theoretically a new approach to realizing the Jaynes-Cummings model using low-energy free electrons coupled to dielectric microcavities and exemplify several quantum technologies made possible by this approach. Using quantum recoil, a large detuning inhibits the emission of multiple consecutive photons, effectively transforming the free electron into a few-level system coupled to the cavity mode. We show that this approach can be used for generation of single photons, photon pairs, and even a quantum SWAP gate between a photon and a free electron, with unity efficiency and high fidelity. Tunable by their kinetic energy, quantum free electrons are inherently versatile emitters with an engineerable emission wavelength. Hence, they pave the way toward new possibilities for quantum interconnects between photonic platforms at disparate spectral regimes.
We revisit the mathematical formulation of the famous Jaynes–Cummings–Paul Hamiltonian, which describes the interaction of a two-level atom with a single mode of an electromagnetic cavity reservoir. We rigorously show that under the condition of ultrastrong coupling between the atom and cavity in which the transition frequency is comparable to the coupling frequency, the bosonic field operators undergo non-sinusoidal time variations. As a result, the well-known solutions to the Jaynes–Cummings–Paul model are no longer valid, even when the rotating wave approximation is not used. We show how a correct mathematical solution could be found instead.