The parametric generation of quantum states of light holds a central position across various fields of quantum technologies. Starting from the seminal experiments in the 1970’s, we retrace the history of this powerful approach for creating and tailoring entangled photon pairs or squeezed states of light from the interaction of strong laser fields with optically nonlinear media. From its inception to its latest applications, this technique not only continues to play a pivotal role in the burgeoning fields of quantum computation, communication, and metrology, but shares also fundamental links with general concepts of quantum field theories in curved space-times.
The parametric generation of quantum states of light holds a central position across various fields of quantum technologies. Starting from the seminal experiments in the 1970’s, we retrace the history of this powerful approach for creating and tailoring entangled photon pairs or squeezed states of light from the interaction of strong laser fields with optically nonlinear media. From its inception to its latest applications, this technique not only continues to play a pivotal role in the burgeoning fields of quantum computation, communication, and metrology, but shares also fundamental links with general concepts of quantum field theories in curved space-times.
This presentation first reviews the historical development of the field of nonlinear optics, starting from its inception in 1961. It then reviews some of its more recent developments, including especially how nonlinear optics has become a crucial tool for the developing field of quantum technologies. Fundamental quantum processes enabled by nonlinear optics, such as the creation of squeezed and entangled light states, are reviewed. We then illustrate these concepts by means of specific applications, such as the development of secure communication systems based on the quantum states of light.
Two photons in a pair generated in the nonlinear optical process of spontaneous parametric down-conversion are, in general, strongly quantum entangled. Accordingly, they contain extremely strong energy, time, polarization and momentum quantum correlations. This entanglement involves more than one quantum variable and has served as a powerful tool in fundamental studies of quantum theory. It is now playing a large role in the development of novel information processing techniques and new optical measurement technologies. Here we review some of these technologies and their origins.
This presentation first reviews the historical development of the field of nonlinear optics, starting from its inception in 1961. It then reviews some of its more recent developments, including especially how nonlinear optics has become a crucial tool for the developing field of quantum technologies. Fundamental quantum processes enabled by nonlinear optics, such as the creation of squeezed and entangled light states, are reviewed. We then illustrate these concepts by means of specific applications, such as the development of secure communication systems based on the quantum states of light. We are also interested in studying the properties of structured light fields. These structured light beams have recently been shown to possess exotic properties of their own, such as vacuum propagation velocities differing from the light velocity c for plane waves. These beams can also be tailored in such a way that they carry orbital angular momentum, which can be used to apply a torque to mechanical objects and as a carrier of information in a classical and quantum telecommunication system. Light can carry angular momentum both by means of its spin angular momentum (as manifested for example in circular polarization) and by means of its orbital angular momentum (OAM), whose origin is a helical structure of its wavefront. The orbital angular momentum of light has recently been recognized to constitute a crucial attribute for many photonic technologies, including the trapping and manipulation of small particles and for multiplexing in optical telecommunication. In this presentation we review some of the fundamental properties of OAM including its quantum features such as entanglement. We then go on to describe a secure telecommunication system in which information is encoded in OAM, and which can carry more than one bit of information per photon.
Engineering non-classical states of the electromagnetic field is a central quest for quantum optics1,2. Beyond their fundamental significance, such states are indeed the resources for implementing various protocols, ranging from enhanced metrology to quantum communication and computing. A variety of devices can be used to generate non-classical states, such as single emitters, light-matter interfaces or non-linear systems3. We focus here on the use of a continuous-wave optical parametric oscillator3,4. This system is based on a non-linear χ2 crystal inserted inside an optical cavity and it is now well-known as a very efficient source of non-classical light, such as single-mode or two-mode squeezed vacuum depending on the crystal phase matching. Squeezed vacuum is a Gaussian state as its quadrature distributions follow a Gaussian statistics. However, it has been shown that number of protocols require non-Gaussian states5. Generating directly such states is a difficult task and would require strong χ3 non-linearities. Another procedure, probabilistic but heralded, consists in using a measurement-induced non-linearity via a conditional preparation technique operated on Gaussian states. Here, we detail this generation protocol for two non-Gaussian states, the single-photon state and a superposition of coherent states, using two differently phase-matched parametric oscillators as primary resources. This technique enables achievement of a high fidelity with the targeted state and generation of the state in a well-controlled spatiotemporal mode.
The fields of quantum and nonlinear optics have given rise to a variety of nonclassical states of light that have been proven to surpass certain limitations set by classical physics. Namely, certain squeezed and entangled states have been shown to beat the shot-noise limit when making precision phase measurements in interferometry, as well as write lithographic patterns that are smaller than classically allowed by the Rayleigh diffraction limit. Additionally, single-photon sources and entangled photon pairs have given rise to provably secure quantum key distribution for cryptography. Producing these quantum states of light has proven a difficult task. Nonlinear crystals, when pumped by a laser, produce pairs of single photons via the process of spontaneous parametric down conversion (SPDC). This process is mediated by the second order nonlinear susceptibility of the material. When pumped in a high gain regime, these crystals give rise to optical parametric amplification, which is a viable source of squeezed light. The vast majority of research in this area has focused on crystals that are seeded by vacuum in their two modes. This dissertation concerns the field of quantum nonlinear optics. It is an investigation into the processes that occur when nonlinear materials interact with the electromagnetic field on the single photon level. I have focused on seeding nonlinear crystals with quantum states of light, including single photons and entangled states. This process results in various states directly applicable to interferometry, imaging, and cryptography. Another application investigated is an absolute radiance measurement via stimulated parametric down conversion resulting from non-vacuum seeding of a nonlinear crystal. Additionally, other nonlinear processes, including four-wave mixing, nonlinear magneto-optical effects and coherent population trapping in warm atomic vapor involving quantum states of light are investigated. The process of seeding third-order nonlinear interactions, such as in atomic vapors, gives rise to a variety of interesting, nonclassical phenomena such as entangled image transfer and nonlocal imaging. Strong analogies between SPDC and four-wave mixing are drawn. I also experimentally show an all optical pi-only phase shift of one light beam via another in warm Cesium vapor.
Light has provided both fundamental phenomenology and enabling technology for scientific discovery for many years, and today it continues to play a central role in fundamental explorations and innovative applications. The ability to manipulate light beams and pulses with the quantum degrees of freedom of optical radiation will add to those advances. The future of quantum optics, which encompasses both the generation and manipulation of nonclassical radiation, as well as its interaction with matter, lies in the rich variety of quantum states that is now becoming feasible to prepare, together with the numerous applications in sensing, imaging, metrology, communications, and information processing that such states enable.