Abstract Advances in quantum information processing can open a way for numerous applications of the processing in various fields of science and technology: communication, precision measurement, computing, nano-scale detectors, and sensors. Classical and various quantum correlations have been studied in real spin 1/2 systems. The nonlocality measures provide a novel classification scheme for bipartite states, highlighting that nonlocality is a quantum resource distinct from other types of quantum correlations. We first studied the temperature and field dependencies of nonlocality measure in the three fictitious spin 1/2 system, which represents a nuclear spin-7/2 placed in magnetic and inhomogeneous electric fields. The relationship between nonlocality and other quantum correlations (entanglement and geometric discord) was studied. The Hamiltonian and spin operators for a spin 7/2 are represented in the basis formed by the Kronecker products of the Pauli matrices. This transformation allows us to represent a spin 7/2 as a system of three coupled fictitious spins 1/2 and, from the quantum information point of view, as an equivalent system of three coupling qubits. Well-developed methods were used to calculate measures of quantum correlations. For example, we consider 59Co (spin 7/2) in the compounds [Co(NH3)5Cl]Cl2 and Ca3Co2O6. The interaction between the fictitious spins of 59Co nuclei depends on the magnitude and direction of the external magnetic field. Other potential cases of quantum correlations can be realized based on nuclear spins 7/2 in solid-state systems, for instance, such as 51V, 165Ho, or 123Sb.
Abstract Advances in quantum information processing can open a way for numerous applications of the processing in various fields of science and technology: communication, precision measurement, computing, nano-scale detectors, and sensors. Classical and various quantum correlations have been studied in real spin 1/2 systems. The nonlocality measures provide a novel classification scheme for bipartite states, highlighting that nonlocality is a quantum resource distinct from other types of quantum correlations. We first studied the temperature and field dependencies of nonlocality measure in the three fictitious spin 1/2 system, which represents a nuclear spin-7/2 placed in magnetic and inhomogeneous electric fields. The relationship between nonlocality and other quantum correlations (entanglement and geometric discord) was studied. The Hamiltonian and spin operators for a spin 7/2 are represented in the basis formed by the Kronecker products of the Pauli matrices. This transformation allows us to represent a spin 7/2 as a system of three coupled fictitious spins 1/2 and, from the quantum information point of view, as an equivalent system of three coupling qubits. Well-developed methods were used to calculate measures of quantum correlations. For example, we consider 59Co (spin 7/2) in the compounds [Co(NH3)5Cl]Cl2 and Ca3Co2O6. The interaction between the fictitious spins of 59Co nuclei depends on the magnitude and direction of the external magnetic field. Other potential cases of quantum correlations can be realized based on nuclear spins 7/2 in solid-state systems, for instance, such as 51V, 165Ho, or 123Sb.
The Hamiltonian and the spin operators for a spin 3/2 are represented in the basis formed by the Kronecker productions of the [Formula: see text] Pauli matrices. This reformulation allows us to represent a spin 3/2 as a system of two coupled fictitious spins 1/2. Correlations between these fictitious spins are studied using well-developed methods. We investigate the temperature and field dependences of correlations, such as mutual information, classical correlations, entanglement, and geometric and quantum discords in the fictitious spin-1/2 system describing a nuclear spin 3/2 which is placed in magnetic and inhomogeneous electric fields. It is shown that the correlations between the fictitious spins demonstrate properties which differ from those of real two-spin systems. In contrast to real systems all the correlations between the fictitious spins do not vanish with increasing external magnetic field; at a high magnetic field the correlations tend to their limiting values. Classical correlations, quantum and geometric discords reveal a pronounced asymmetry relative to the measurements on subsystems (fictitious spins) even in a uniform magnetic field and at symmetrical EFG, [Formula: see text]. The correlations depend also on the distribution of external charges, on the parameter of symmetry [Formula: see text]. At [Formula: see text] quantum and geometric discords have finite values in a zero magnetic field. The proposed approach may be useful in analysis of properties of particles with larger angular momentum, can provide the way to discover new physical phenomenon of quantum correlations, and can be a useful tool for similar definitions of other physical quantities of complex systems.
Non-classical correlations arise in various quantum mechanical systems. Characterization and quantification of these correlations is an important and active branch of research in the field of quantum information theory. Investigation of non-classical correlations in condensed matter systems gives important insights about the characteristics of these systems. In particular, systems possessing a quantum critical point in their phase diagrams have attracted much attention due to the peculiar behavior of correlations near these points. In this thesis, we have investigated two distinct quantum spin models from the perspective of correlations and, we have discussed the correlation content of an important subclass of bipartite states. We start by an analytical calculation of the quantum discord for a system composed of spin-j and spin-1/2 subsystems possessing rotational symmetry. We have compared our results with the quantum discord of states having similar symmetries and seen that in rotationally invariant states the amount of quantum discord is much higher. Moreover, using the well known entanglement properties of these states, we have compared their quantum discord with entanglement and seen that quantum discord is higher than the entanglement. Next, we have investigated the thermal quantum correlations and entanglement in spin-1 Bose-Hubbard model with two and three particles. We have demonstrated that the energy level crossings in the ground state of the system are signalled by both the behavior of thermal quantum correlations and entanglement. Finally, we have investigated various thermal quantum and total correlations in the anisotropic XY spin-chain with transverse magnetic field. We have shown that the ability of the considered measures to estimate the critical points of this system at finite temperature strongly depends on the anisotropy parameter of the Hamiltonian. Furthermore, we have studied the effect of temperature on long-range correlations of the XY chain.
Despite the success of quantum mechanics in predicting the outcomes of experiments in many branches of physics, the foundations of the theory have remained subject of research and dispute. At the basis of this struggle with the theory lie the phenomena of nonlocality and entanglement. Since it was first predicted by Bell in 1964, nonlocality was not only verified in numerous experiments, but also identified as a useful resource for quantum information processing. Thus, the study of nonlocality is important both from a fundamental point of view and with respect to new applications in quantum information theory, such as secure cryptography and randomness generation. The identification of entanglement as a resource for quantum information led to a strong theoretical effort devoted to its characterisation and detection. Many of the resulting mathematical tools find application in several domains of physics. Although the only known way to create nonlocal correlations is to measure entangled quantum systems, it has been shown that entanglement and nonlocality constitute two inequivalent properties. Therefore, in the light of the success of entanglement theory, it is of interest to also devise a resource theory of nonlocality. The task of this thesis is to develop such a theoretical framework for the characterisation of nonlocality as a resource. To gain a better understanding of nonlocal correlations it will be necessary to investigate correlation scenarios that go beyond the situation originally considered by Bell. In doing so, this thesis provides new description of nonlocality that also have implications for the characterisation of quantum correlations and the detection of new forms of nonlocality. The first question we address is how nonlocality can consistently be defined in a scenario of arbitrarily many parties that may collaborate among each other. To this end we recognise which are the allowed physical operations in this situation and then define nonlocality as the resource that cannot be created by these operations. Our approach shows that the conventional definition of multipartite nonlocality, adopted by the community so far, is inconsistent with this operational definition; we further propose and analyse new models that do not suffer from these inconsistencies. Furthermore, we show that our findings have implications for the characterisation of quantum correlations. A recent approach to describe the set of quantum correlation consists in using principles inspired from information theory. By using a special instance of the models we defined earlier we show a fundamental limitation of this approach: no bipartite information principle is sufficient to single out the set of quantum correlations from the set of nonsignalling correlations. We then developed a description of nonlocality in an even more generalised scenario of several parties. Motivated by a result of Popescu we study scenarios where the parties are allowed to perform not only a single but sequences of measurements on their systems. Characterising nonlocality also in this scenario in operational terms and defining local models compatible with this definition, we show that a new form of nonlocality can be detected Lastly, we examine the problem of detecting the presence of nonlocality in a multipartite scenario when one is given only partial access to the global system. We find that one can verify that the total system must display nonlocality, even though the accessible subsystems only exhibit local correlations.
Quantum mechanics is nonlocal, which makes it different from classical mechanics. Quantum information and quantum computation is a promising frontier science which is based on quantum mechanics. The nonlocality of quantum mechanics is the fundamental reason that many quantum information processing tasks have significant advantages over their classical counterparts.
In this dissertation, we study three aspects of quantum nonlocality, which include the quantitative relationship between entanglement and nonlocality, the quantification of genuine tripartite nonlocality and the distribution of nonlocal quantum resources. To be specific,
• We investigate the quantitative relationship between entanglement and nonlocality of bipartite quantum systems. We start by exploiting the condition that the nonlocality of two different two-qubit states can be optimally examined by a same nonlocality test setting. Via numerical simulation, we find that the nonlocality of a generic two-qubit state is upper bounded by a function of the corresponding entanglement. Further, we give an analytical proof for the upper bound and find the class of two-qubit states that can reach the upper bound.
• We analyze the quantification of genuine tripartite nonlocality of a generic three-qubit state. We find a method to solve the problem for a special class of three-qubit states which include not only pure states but also mixed states. Applying the method, we drive analytical results for the genuine tripartite nonlocality of generalized GHZ states, generalized Werner states and two class of mixed states with special correlation matrices.
• We investigate the distribution of nonlocal quantum resources. To distribute bipartite nonlocal quantum resources, we design an efficient quantum repeater scheme, which not only achieves the optimal transmission rate but also consumes less resources of local operations and classical communication, for the case of general pure states of two-qubit system. We also analyze the case of bipartite pure states of arbitrary dimensional quantum system and get an upper bound on the probability of a successful projection operation to produce a maximally nonlocal state. To distribute tripartite nonlocal resources, we propose a simple scenario to generate tripartite nonlocal resources from bipartite nonlocal resources. As examples, we examine the cases that two-qubit Werner states and general two-qubit pure states are prepared as resources, respectively. We get the upper bounds on the genuine tripartite nonlocality that can be generated in the scenario. We also provide the optimal measurement settings to achieve the upper bounds.
It has been proven that the quantum discord is a more general tool to capture non-classical correlation than quantum entanglement, because there is a non-zero quantum discord in several mixed states that could not be measured by quantum entanglement. But because of optimization part in formulating quantum discord, it is very difficult and nearly impossible to find quantum discord for some quantum states. So people proposed geometric quantum discord, which in a bipartite state could be describe as the distance of the states from the closest zero-discord state. To understand better geometric quantum discord, this paper is devoted to compare it with quantum discord and measurement induced non-locality that is in some sense dual to the geometric quantum discord. As studying the quantum correlation experimentally is one of the important thing in quantum information processing, so as our example for illustrating the difference of geometric quantum discord, quantum discord and measurement induced non-locality, our quantum system is a dimer (two spin-1/2 particles) in multiple quantum nuclear magnetic resonance.
A formalism is presented that describes the time behavior of the spin density matrix of a nuclear spin system with arbitrary spin in terms of fictitious spin −(1/2) operators. This formalism is an extension of that used earlier for nuclei with spin I=1. For a spin system with n eigenstates we define for every pair of eigenstates ‖i〉 and ‖j〉 three operators Ii−jp, with p=x, y, and z, according to the three 2×2 Pauli matrices σx, σy, and σz. These operators together constitute a complete set of n2−1 independent Hermitian operators, and we can write the n×n density matrix and the spin Hamiltonian of the system in terms of the Ii−jp operators. The commutation relations among the operators make it possible in many cases to solve the equation of motion of the density matrix analytically. Three examples of the use of the Ii−jp operators are presented. Firstly a system of noninteracting spins with I=1 is considered. The Ii−jp operators for this case are compared with the Iq,k operator defined earlier. The cw signal intensities of the single and double quantum transitions for the I=1 spin system are derived. Secondly a spin system with I=3/2 is described as a simple extension of the use of the Ii−jp operators. The excitation and the detection of the triple quantum coherence are discussed for noninteracting nuclei in solids. Finally the double quantum effects in a system of two interacting spins with I=1/2 are discussed.