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International Journal of Modern Physics C

Dynamics of graphene as an open quantum system

M. Showkat, Mayank Shah

Published May 17, 2024• 0 citations
Publisher

Abstract

We examine the imbalance thermodynamics of uncontaminated decoherence in graphene. In a uncontaminated decoherence process, no exchange of energy takes place directly between graphene and the surroundings. It is seen that due to decoherence heat dissolution takes place due to which energy of the environment cannot remain conserved. In this paper, we find out the energy eigenvalues and wave function in the graphene from the perturbed Hamiltonian to find out the density matrix and entropy of the system and their unique relation between the density matrix, momentum of the graphene and entropy where the graphene is taken as an open system. In graphene, the behavior of electrons is controlled by the massless Hamiltonian and ([Formula: see text]) Dirac equation.

DOI
10.1142/s0129183124501663

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We examine the imbalance thermodynamics of uncontaminated decoherence in graphene. In a uncontaminated decoherence process, no exchange of energy takes place directly between graphene and the surroundings. It is seen that due to decoherence heat dissolution takes place due to which energy of the environment cannot remain conserved. In this paper, we find out the energy eigenvalues and wave function in the graphene from the perturbed Hamiltonian to find out the density matrix and entropy of the system and their unique relation between the density matrix, momentum of the graphene and entropy where the graphene is taken as an open system. In graphene, the behavior of electrons is controlled by the massless Hamiltonian and ([Formula: see text]) Dirac equation.
We investigate the non-equilibrium thermodynamics of pure decoherence. In a pure decoherence process, the system Hamiltonian is a constant of motion and there is no direct energy exchange between the system and its surroundings. Nevertheless, the environment’s energy is not generally conserved and in this work we show that this leads to non-trivial heat dissipation as a result of decoherence alone. This heat has some very distinctive properties: it obeys an integral fluctuation relation and can be interpreted in terms of the entropy production associated with populations in the energy eigenbasis of the initial state. We show that the heat distribution for a pure decoherence process is different from the distribution of work done by the initial system–bath interaction quench. Instead, it corresponds to a mixture of work distributions of cyclical processes, each conditioned on a state of the open system. Inspired by recent experiments on impurities in ultracold gases, we demonstrate our general results by studying the heat generated by the decoherence of a qubit immersed within a degenerate Fermi gas in the lowest band of a species-selective optical lattice.
Thermodynamics coupled quantum features on electron and hole dynamics in Dirac materials is quite interesting and crucial for real device applications such as electronic, thermoelectric, energy devices, and quantum circuits. The correlation between the formation of electron-hole puddles near the charge neutrality point (CNP) and the role of disorder in terms of differential entropy is fundamentally important for the Dirac transport mechanism in graphene systems, but not yet well-established. With this motivation, we map the energy quantization for Dirac materials through the empirical relation of voltage-driven charge density in monolayer graphene, using the differential entropy (h)-ruled wavevector (k) mechanics. For this work, we propose the four postulates which are the key observable descriptions of earlier research reports, to study the precise electronic transport via an entropy-guided wavevector propagation approach, along with the Klein paradox, which pertains to the ultrafast dynamics in the Dirac or quasi-Dirac systems. The introduced h-ruled k and h-ruled N relations generalize the electron dynamics in both the unbounded and potentially bounded Dirac systems. Through the quantization mapping procedure under different voltage-driven potential (U=eV) boundary conditions, the observed energy shift from lower to excited quantum state obeys the relation of N(k)=N(U)^3; here, N(U) is the voltage-driven potential energy contribution factor for the quantum state existence. In such a way, the mapped electron density, diffusion coefficient, and mobility for bounded Dirac materials are increased by orders of N^3, N^2, and N, respectively. This study reveals information about the interaction potential-DOS relationship in the Dirac materials.
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Abstract We investigate the dynamics of entanglement and quantum coherence between the pseudospin and valley indices of individual electrons in two-dimensional graphene, thermalized at an equilibrium temperature T . The system is modeled by an effective Dirac-like Hamiltonian describing a graphene valley-pseudospin qubit under polarized laser driving, including sublattice-dependent scattering process, while the thermal fluctuations are accounted through the standard Gibbs thermal state. Entanglement between the two degrees of liberty of electrons is quantified using concurrence, and coherence with the system is measured employing the relative entropy of coherence. The findings demonstrate that the behavior of entanglement and coherence under thermal noise strongly depends on the scattering strength, wavevector components, and electromagnetic field. Additionally, our results indicate that the strong polarized fields ( ξ 0 = 8 meV 2 ) with low-frequency ( ω = 0.06 eV ) can be employed to enhance the robustness of thermal entanglement and coherence of the system at intermediate temperatures. We also explore the impact of the other system parameters, like scattering strength and wavevector components, in enhancing and preserving quantum resources within graphene-based systems, noting particularly that the relative entropy of coherence is more resilient than concurrence against thermal decoherence.
This research delves into the influence of intrinsic decoherence on the behavior of quantum correlations and coherence between two interacting qubits in a graphene-based system. To evaluate the amount of nonclassical correlations in the system, we employ local quantum uncertainty (LQU), and to assess quantum coherence we use the relative entropy of coherence [Formula: see text] and [Formula: see text]-norm [Formula: see text]. We assume that the system is initially prepared in an extended-Werner-like (EWL) state, and we investigate how these quantifiers evolve over time and examine their sensitivity to various graphene layer system parameters, mixture parameter of the initial state and the intrinsic decoherence rate. Our results indicate that by adjusting the wave number operators, decreasing the intrinsic decoherence rate, and increasing the initial state mixing parameter, it is possible to enhance both quantum correlations and coherence within the two-dimensional honeycomb lattice system. In addition, we found that quantum coherence is more resilient to intrinsic decoherence than LQU, moreover, the [Formula: see text]-norm is more robust than the relative entropy of coherence.
We study the nonequilibrium thermodynamics of pure decoherence processes in open quantum systems coupled to a thermal reservoir. We review various definitions of central quantities, such as internal energy, work, heat, and entropy production, developed within local and global approaches to quantum thermodynamics. Within local approaches, thermodynamic quantities only refer to the open system's degrees of freedom, while in the global approaches, certain quantities are defined by referring explicitly to the reservoir degrees of freedom. Employing a microscopic, analytically solvable model, we perform a comparison of these two perspectives, revealing substantial differences in the thermodynamic quantities and in the formulations of the first and second laws. The main reason for these discrepancies is the fact that the global approaches involve the system-reservoir interaction which exchanges a large amount of energy with the environment, while the average open system energy is constant in time because the dynamics represents pure decoherence and does not affect the open system populations.