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New Journal of Physics

Effect of relaxation on the transfer of orbital angular momentum via four-wave mixing process in the four-level double lambda atomic system

Rohit Kumar, Dixith Manchaiah, Mobassir Ahmad, Raghavan K. Easwaran

Published May 1, 2024• 5 citations
Publisher

Abstract

Abstract In this work, we have theoretically studied the resonant four-wave mixing (FWM) in a four-level double Lambda (Λ) atomic system in connection with orbital angular momentum (OAM) transfer from probe to generated signal beam. The effect of the relaxation process is studied in the forward as well as backward FWM. Based on the semiclassical model, our analysis shows a strong dependence of conversion efficiency on spontaneous decay and decoherence rates. From the intensity and phase profile, we have confirmed the OAM nature of the generated signal beam. The physical explanation is given for the dependence of efficiency on the decay rate of the excited atomic state. We have shown that decoherence present in the system always leads to a deleterious effect on conversion efficiency. Our presentation treats forward and backward FWM in a unified way in the context of OAM transfer and sheds light on the parameter dependence of conversion efficiency.

DOI
10.1088/1367-2630/ad4b59

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Abstract In this work, we have theoretically studied the resonant four-wave mixing (FWM) in a four-level double Lambda (Λ) atomic system in connection with orbital angular momentum (OAM) transfer from probe to generated signal beam. The effect of the relaxation process is studied in the forward as well as backward FWM. Based on the semiclassical model, our analysis shows a strong dependence of conversion efficiency on spontaneous decay and decoherence rates. From the intensity and phase profile, we have confirmed the OAM nature of the generated signal beam. The physical explanation is given for the dependence of efficiency on the decay rate of the excited atomic state. We have shown that decoherence present in the system always leads to a deleterious effect on conversion efficiency. Our presentation treats forward and backward FWM in a unified way in the context of OAM transfer and sheds light on the parameter dependence of conversion efficiency.
Vortex light, a unique optical field that carries orbital angular momentum (OAM), has attracted considerable attention in recent years. In this paper, we present a detailed theoretical analysis of OAM transfer from the input field to the generated signal field in a four-level double-Lambda system via the four-wave mixing (FWM) process, showing that their OAMs follow a specific algebraic relationship. We identify the optimal conditions for efficient vortex light transmission, analyze the influence of detuning on transmission efficiency and phase distortion, and specifically examine the scenario where the control field carries OAM the latter being essential for a complete characterization of OAM conservation in the FWM process, while all three aspects have been largely overlooked in the existing literature. Furthermore, we investigated the tunability of the group velocity between the probe and signal fields by modulating the Rabi frequencies of the two control fields and the relative phase between the probe and signal fields during the FWM process. We demonstrate that the conversion between matched vortex slow and fast light can be realized an effect that has not been widely explored in dual-Lambda-type systems. These results may hold promise for applications in quantum information storage and processing, quantum computing, and ultrasensitive detection.
We propose and analyze an efficient scheme for the coherent transfer of optical vortices in a cold atomic ensemble with four-level double-$\mathrm{\ensuremath{\Lambda}}$ configuration. The orbital angular-momentum (OAM) information can be transferred from the incident vortex fields to the generated backward signal field via resonant backward four-wave mixing (FWM). Considering the single vortex probe field initially acting on one transition of the atomic ensemble and using experimentally achievable parameters, we identify the conditions under which the resonant backward FWM allows us to greatly improve the conversion efficiency of optical vortices beyond what is achievable in the resonant forward OAM transfers. It is found that the complete energy conversion of optical vortices originates from the perfect competition between linear absorption and parametric gain. We also demonstrate that the phase mismatching would be detrimental to the high-efficiency transfer of optical vortices. Furthermore, we show that the generated backward signal field develops a new pure or mixing OAM state when the control field is also a vortex beam. Finally, we investigate the composite vortex beam generated by collinear superposition of the incident vortex probe and signal fields, which can controlled via adjusting the intensity of the control field. Our scheme may have potential applications in OAM-based optical communication and optical information processing.
Abstract In this paper, we suggest a theoretical model for the exchange of the orbital angular momentum (OAM) state of laser fields in a real cold atomic system for realization in an experimental setup. By using four-wave mixing (FWM) processes, we study the spatial dependence of the new weak generated signal light under electromagnetically induced transparency conditions when one of the laser lights becomes an optical vortex. We discuss the spatial dependence of FWM processes via experimental parameters for different conditions of the OAM of vortex light. We have found that the intensity and phase distributions of the new generated light depends strongly on the OAM number of the optical vortex light. Moreover, we investigate the absorption spectrum of the new generated signal light for different OAM of the optical vortex light. Our obtained results may have potential applications in quantum information science.
We explore the conservation of orbital angular momentum (OAM) in the four-wave mixing (FWM) process in hot rubidium vapor. Since most modern communication systems send data in pulses corresponding to bits, we can use OAM to encode more information in each pulse by assigning structure to each signal. Furthermore, because FWM can be used to generate entangled photon pairs, we can use this process to bring enhanced signal security. We experimentally studied FWM with a wide range of Laguerre-Gaussian modes and their superpositions and observed OAM transfer from the probe field to a generated Stokes field. By studying the output Stokes intensity and phase distributions, we confirm l mode (OAM) conservation for pure l and p modes, as well as for the superpositions of l and -l for the mode numbers up to l = 4, p = 4. We also found that p index is generally not conserved and its conservation is highly dependent on the relative sizes of the probe and pump beams in the Rb cell. We also identify parameters to improve FWM gain with OAM transfer and propose an analytical method for determining OAM p number.
Electromagnetically-induced-transparency-based four-wave mixing (FWM) in a resonant four-level double-Λ system has a maximum conversion efficiency (CE) of 25% due to spontaneous emission. Herein, we demonstrate that spontaneous emission can be considerably suppressed by arranging the applied laser beams in a backward configuration. With the backward double-Λ FWM scheme, we observe a CE of 63% in cold rubidium atoms with an optical depth (OD) of 48. To the best of our knowledge, this is the first observation of a CE exceeding the conversion limit in resonant FWM processes. Furthermore, we present a theoretical model that includes the phase-mismatch effect in the backward double-Λ FWM system. According to the theoretical model, the present scheme can achieve 96% CE using a medium with a large OD of 200 under ideal conditions. Such an efficient frequency conversion scheme has potential applications in optical quantum information technology.
A scheme for high-efficiency transfer of optical vortices is proposed by an inelastic two-wave mixing (ITWM) process in an inverted-Y four-level atomic medium, which is originally prepared in a coherent superposition of two ground states. The orbital angular momentum (OAM) information in the incident vortex probe field can be transferred to the generated signal field through the ITWM process. Choosing reasonable experimentally realizable parameters, we find that the presence of the off-resonance control field can greatly improve the conversion efficiency of optical vortices, rather than in the absence of a control field. This is caused by the broken of the destructive interference between two one-photon excitation pathways. Furthermore, we also extend our model to an inelastic multi-wave mixing process and demonstrate that the transfer efficiency between multiple optical vortices strongly depends on the superposition of the ground states. Finally, we explore the composite vortex beam generated by collinear superposition of the incident vortex probe and signal fields. It is obvious that the intensity and phase profiles of the composite vortex can be effectively controlled via adjusting the intensity of the control field. Potential applications of our scheme may exist in OAM-based optical communications and optical information processing.