The sensitivity of electric field sensors based on two-photon electromagnetically induced transparency (EIT) involving highly excited Rydberg states in thermal atoms is often limited by the residual Doppler effect and optical power broadening. Here, we propose a method to reduce the EIT spectral linewidth using a Ramsey interrogation approach, allowing multiple interrogations of atomic coherence, using either temporally or spatially separated laser beams. Our theoretical calculations predict that the linewidth of such Raman-Ramsey spectral features can be substantially reduced compare to a standard Doppler-broadened EIT, opening a possibility to improved sensitivity of Rydberg atomic vapor-based sensors. We also discuss some preliminary experimental efforts toward observing Raman-Ramsey resonances for both spatially and temporally separated interrogation approaches and associated technical challenges.The sensitivity of electric field sensors based on two-photon electromagnetically induced transparency (EIT) involving highly excited Rydberg states in thermal atoms is often limited by the residual Doppler effect and optical power broadening. Here, we propose a method to reduce the EIT spectral linewidth using a Ramsey interrogation approach, allowing multiple interrogations of atomic coherence, using either temporally or spatially separated laser beams. Our theoretical calculations predict that the linewidth of such Raman-Ramsey spectral features can be substantially reduced compare to a standard Doppler-broadened EIT, opening a possibility to improved sensitivity of Rydberg atomic vapor-based sensors. We also discuss some preliminary experimental efforts toward observing Raman-Ramsey resonances for both spatially and temporally separated interrogation approaches and associated technical challenges.

arXiv:2310.10615Oct 16, 20230 citations

Fundamental linewidth limit of electromagnetically induced transparency in a thermal Rydberg ladder

Anonymous, Nikunjkumar Prajapati, Alexandra B. Artusio‐Glimpse +2 more

Spectroscopy of Rydberg states has become a popular platform for quantum sensing, with the most common readout scheme being two-photon electromagnetically induced transparency (EIT) using counterpropagating laser beams. In this scheme, the energy resolution of the Rydberg state is set by the spectral linewidth of the EIT feature. While selection criteria for the two-photon resonance can narrow the linewidth to the order of the Rydberg state decay rate for a single atom, the Doppler shift from thermal velocity of the atoms broadens the ensemble linewidth to the order of the decay rate of the intermediate state. Here, we derive an analytic expression for the Doppler residual line shape in the low-power limit and corroborate the results with experiment. For Rb, we find the full-width-at-half-maximum linewidth limit to be 1.84 MHz when scanning the coupling laser and measure an experimental linewidth of 2.04 MHz. These linewidths are around a factor of 2 narrower than previous theoretical estimates as well as previously reported measured linewidths. With this, we demonstrate the most precise two-photon energy resolution of a Rydberg state in thermal vapor to date. We then map out broadening mechanisms near this limit.Spectroscopy of Rydberg states has become a popular platform for quantum sensing, with the most common readout scheme being two-photon electromagnetically induced transparency (EIT) using counterpropagating laser beams. In this scheme, the energy resolution of the Rydberg state is set by the spectral linewidth of the EIT feature. While selection criteria for the two-photon resonance can narrow the linewidth to the order of the Rydberg state decay rate for a single atom, the Doppler shift from thermal velocity of the atoms broadens the ensemble linewidth to the order of the decay rate of the intermediate state. Here, we derive an analytic expression for the Doppler residual line shape in the low-power limit and corroborate the results with experiment. For Rb, we find the full-width-at-half-maximum linewidth limit to be 1.84 MHz when scanning the coupling laser and measure an experimental linewidth of 2.04 MHz. These linewidths are around a factor of 2 narrower than previous theoretical estimates as well as previously reported measured linewidths. With this, we demonstrate the most precise two-photon energy resolution of a Rydberg state in thermal vapor to date. We then map out broadening mechanisms near this limit.

arXiv:2603.04596Physical Review ResearchAug 26, 20260 citations

Photon shot-noise-limited Rydberg-EIT electrometry

Gyeongmin Ju, Ye Jin Yu, Heewoo Kim +4 more

Rydberg-atom electrometry is a core technique in the development of highly sensitive quantum electric-field sensors. Its sensitivity based on atom-photon interaction is typically limited by photon shot-noise (PSN) and spectral broadenings. Here, we experimentally demonstrate a near PSN-limited Rydberg electrometry from a 85Rb atomic vapor cell. By engineering atomic coherence through control of residual magnetic fields and laser frequency noise, we achieve the Rydberg electromagnetically induced transparency (EIT) with the narrow linewidth of 1.6 MHz, yielding an enhanced spectral slope for high-sensitivity Rydberg-EIT electrometry. Under optimized superheterodyne detection conditions, we obtain an electric-field sensitivity of 12.5(8) nV cm^-1 Hz^-1/2 at 37 GHz, in close agreement with the calculated PSN limit. These results provide direct experimental evidence of the high-sensitive quantum electrometry and establish a practical route toward quantum-noise-limited Rydberg electrometry.Rydberg-atom electrometry is a core technique in the development of highly sensitive quantum electric-field sensors. Its sensitivity based on atom-photon interaction is typically limited by photon shot-noise (PSN) and spectral broadenings. Here, we experimentally demonstrate a near PSN-limited Rydberg electrometry from a 85Rb atomic vapor cell. By engineering atomic coherence through control of residual magnetic fields and laser frequency noise, we achieve the Rydberg electromagnetically induced transparency (EIT) with the narrow linewidth of 1.6 MHz, yielding an enhanced spectral slope for high-sensitivity Rydberg-EIT electrometry. Under optimized superheterodyne detection conditions, we obtain an electric-field sensitivity of 12.5(8) nV cm^-1 Hz^-1/2 at 37 GHz, in close agreement with the calculated PSN limit. These results provide direct experimental evidence of the high-sensitive quantum electrometry and establish a practical route toward quantum-noise-limited Rydberg electrometry.

physics.atom-phCross-listedarXiv:2606.04354Jun 4, 20260 citations

Improving Spectral Resolution of Rydberg Atom-Based Electrometry by 2 × 2 Laser Arrays

Fengting Zhao, Qiang An, Jinhao Zhang +1 more

Rydberg atom-based electrometry based on electromagnetic induced transparency (EIT) and Autler–Townes splitting (EIT-AT) could achieve ultra-high sensitivity measurements. The amplitude and linewidth of EIT spectra significantly impact the accuracy of electric field measurements. This research utilizes cascade diffraction gratings to generate 2×2 probe laser arrays for the excitation of Rydberg atoms, thereby enhancing spectral resolution under the power broadening. Compared with one laser, the laser array boosts EIT amplitude, narrowing the linewidth from 23.53 MHz to 12.66 MHz, making EIT-AT more distinguishable under identical fields and achieving an enhancement of the sensitivity of 77.96 nV/cm/Hz. These results indicate that laser arrays can optimize the sensitivity of measurement systems based on the Rydberg EIT effect.Rydberg atom-based electrometry based on electromagnetic induced transparency (EIT) and Autler–Townes splitting (EIT-AT) could achieve ultra-high sensitivity measurements. The amplitude and linewidth of EIT spectra significantly impact the accuracy of electric field measurements. This research utilizes cascade diffraction gratings to generate 2×2 probe laser arrays for the excitation of Rydberg atoms, thereby enhancing spectral resolution under the power broadening. Compared with one laser, the laser array boosts EIT amplitude, narrowing the linewidth from 23.53 MHz to 12.66 MHz, making EIT-AT more distinguishable under identical fields and achieving an enhancement of the sensitivity of 77.96 nV/cm/Hz. These results indicate that laser arrays can optimize the sensitivity of measurement systems based on the Rydberg EIT effect.

PhotonicsDec 3, 20252 citations

Rydberg-atom-based radio-frequency sensors: amplitude-regime sensing

Matthias Schmidt, Stephanie M. Bohaichuk, Vijin Venu +5 more

Rydberg atom-based radio frequency electromagnetic field sensors are drawing wide-spread interest because of their unique properties, such as small size, dielectric construction, and self-calibration. These photonic sensors use lasers to prepare atoms and read out the atomic response to a radio frequency electromagnetic field based on electromagnetically induced transparency, or related phenomena. Much of the theoretical work has focused on the Autler-Townes splitting induced by the radio frequency wave. The amplitude regime, where the change in transmission observed on resonance is measured to determine electric field strength, has received less attention. In this paper, we deliver analytic expressions that are useful for calculating the absorption coefficient in the amplitude regime. Our main goal is to describe the analytic expressions for the absorption coefficient and demonstrate their validity over a large range of the interesting parameter space. The effect of the thermal motion of the atoms is explicitly addressed. The analytic formulas for the absorption coefficient for different types of Doppler broadening are compared to estimate the sensitivity under conditions where it is limited by the laser shot noise. Residual Doppler shifts are shown to limit sensitivity. The expressions, approximations and descriptions presented in the paper are important for understanding the absorption of Rydberg atom-based sensors in the amplitude regime. This provides insight into the physics of multi-level interference phenomena.Rydberg atom-based radio frequency electromagnetic field sensors are drawing wide-spread interest because of their unique properties, such as small size, dielectric construction, and self-calibration. These photonic sensors use lasers to prepare atoms and read out the atomic response to a radio frequency electromagnetic field based on electromagnetically induced transparency, or related phenomena. Much of the theoretical work has focused on the Autler-Townes splitting induced by the radio frequency wave. The amplitude regime, where the change in transmission observed on resonance is measured to determine electric field strength, has received less attention. In this paper, we deliver analytic expressions that are useful for calculating the absorption coefficient in the amplitude regime. Our main goal is to describe the analytic expressions for the absorption coefficient and demonstrate their validity over a large range of the interesting parameter space. The effect of the thermal motion of the atoms is explicitly addressed. The analytic formulas for the absorption coefficient for different types of Doppler broadening are compared to estimate the sensitivity under conditions where it is limited by the laser shot noise. Residual Doppler shifts are shown to limit sensitivity. The expressions, approximations and descriptions presented in the paper are important for understanding the absorption of Rydberg atom-based sensors in the amplitude regime. This provides insight into the physics of multi-level interference phenomena.

arXiv:2307.00121Optics ExpressJun 13, 202422 citations

SPECTRAL LINE NARROWING IN ELECTROMAGNETICALLY INDUCED TRANSPARENCY

Yanhong Xiao

Electromagnetically induced transparency (EIT) can make an otherwise opaque medium transparent by utilizing quantum coherence. EIT has attracted great interest since the 1990s for its wide applications in metrology, nonlinear and quantum optics, and quantum information science. We present a review on spectral line narrowing mechanisms in EIT-related systems, accounting for linewidths much narrower than expected from the standard mechanisms of Doppler broadening, transit time broadening, magnetic field inhomogeneity and power broadening. Topics covered include Dicke narrowing, atomic-motion-induced Ramsey narrowing, motional narrowing, density narrowing, laser induced narrowing and power-broadening-free resonance. Intuitive pictures are provided to describe the essential physics of each mechanism.Electromagnetically induced transparency (EIT) can make an otherwise opaque medium transparent by utilizing quantum coherence. EIT has attracted great interest since the 1990s for its wide applications in metrology, nonlinear and quantum optics, and quantum information science. We present a review on spectral line narrowing mechanisms in EIT-related systems, accounting for linewidths much narrower than expected from the standard mechanisms of Doppler broadening, transit time broadening, magnetic field inhomogeneity and power broadening. Topics covered include Dicke narrowing, atomic-motion-induced Ramsey narrowing, motional narrowing, density narrowing, laser induced narrowing and power-broadening-free resonance. Intuitive pictures are provided to describe the essential physics of each mechanism.

Modern Physics Letters BFeb 20, 200923 citations

Rydberg Raman-Ramsey (R

{}^3

) resonances in atomic vapor