We study a generalization of a recently introduced Dicke trimer model [Phys. Rev. Lett. 128, 163601 (2022); Phys. Rev. Res. 5, L042016 (2023)], which allows for cavity losses and unbalanced light-matter interactions (in which rotating and counter-rotating terms can be tuned independently). In the original description of a Dicke trimer, three Dicke models are coupled in a ring topology via a complex photon hopping whose complex phase describes a synthetic magnetic field threading the loop. This original model features several intriguing equilibrium phases and critical phenomena such as frustrated superradiance, two-critical scalings in the frustrated superradiant phase, and finite critical fluctuations in the anomalous normal phase. Here, we find that in the extreme unbalanced limit, where only rotating terms are present, the U(1) symmetry of the Tavis-Cummings model is restored, qualitatively altering the critical phenomena in the superradiant phase due to the presence of a zero-energy mode. To analyze this general regime, we develop a semiclassical theory based on a requantization technique. This theory also provides further physical insight on recently reported anomalous finite critical fluctuations in the time-reversal broken regime. Moving to the open-Dicke case, by introducing local dissipation to the cavities, we observe the emergence of a rich range of nonequilibrium phases characterized by trivial and nontrivial dynamical signatures. In the former case, we identify, when time-reversal symmetry is present, a new stationary phase that features superradiant states in two of the three cavities and a normal state in the other cavity. In the latter case, we observe the emergence of dynamical phases in which the system exhibits superradiant oscillations, characterized by periodic or chaotic phase space patterns. The landscape of transitions associated with these dynamical phases features a wide range of qualitatively different behaviors such as Hopf bifurcations (followed by period-doubling cascades or quasiperiodic oscillations), anomalous Hopf bifurcations (with burst-oscillation-like post-bifurcation dynamics), collisions between basins of attraction (associated with different symmetry-broken equilibria), and exterior crises (featuring transient chaotic dynamics). We highlight how the two-critical-scalings feature of the closed model is robust under dissipation (with doubled critical exponents) while the phenomenon of anomalous finite critical fluctuations becomes a mean-field scaling (as a consequence of Hopf bifurcations of the equilibria featuring the normal state) in the open model.
We study a generalization of a recently introduced Dicke trimer model [Phys. Rev. Lett. 128, 163601 (2022); Phys. Rev. Res. 5, L042016 (2023)], which allows for cavity losses and unbalanced light-matter interactions (in which rotating and counter-rotating terms can be tuned independently). In the original description of a Dicke trimer, three Dicke models are coupled in a ring topology via a complex photon hopping whose complex phase describes a synthetic magnetic field threading the loop. This original model features several intriguing equilibrium phases and critical phenomena such as frustrated superradiance, two-critical scalings in the frustrated superradiant phase, and finite critical fluctuations in the anomalous normal phase. Here, we find that in the extreme unbalanced limit, where only rotating terms are present, the U(1) symmetry of the Tavis-Cummings model is restored, qualitatively altering the critical phenomena in the superradiant phase due to the presence of a zero-energy mode. To analyze this general regime, we develop a semiclassical theory based on a requantization technique. This theory also provides further physical insight on recently reported anomalous finite critical fluctuations in the time-reversal broken regime. Moving to the open-Dicke case, by introducing local dissipation to the cavities, we observe the emergence of a rich range of nonequilibrium phases characterized by trivial and nontrivial dynamical signatures. In the former case, we identify, when time-reversal symmetry is present, a new stationary phase that features superradiant states in two of the three cavities and a normal state in the other cavity. In the latter case, we observe the emergence of dynamical phases in which the system exhibits superradiant oscillations, characterized by periodic or chaotic phase space patterns. The landscape of transitions associated with these dynamical phases features a wide range of qualitatively different behaviors such as Hopf bifurcations (followed by period-doubling cascades or quasiperiodic oscillations), anomalous Hopf bifurcations (with burst-oscillation-like post-bifurcation dynamics), collisions between basins of attraction (associated with different symmetry-broken equilibria), and exterior crises (featuring transient chaotic dynamics). We highlight how the two-critical-scalings feature of the closed model is robust under dissipation (with doubled critical exponents) while the phenomenon of anomalous finite critical fluctuations becomes a mean-field scaling (as a consequence of Hopf bifurcations of the equilibria featuring the normal state) in the open model.
We study a generalization of a recently introduced Dicke trimer model [Phys. Rev. Lett. 128, 163601, Phys. Rev. Research 5, L042016], which allows for cavity losses and unbalanced light-matter interactions (in which rotating and counter-rotating terms can be tuned independently). We find that in the extreme unbalanced limit, the U(1) symmetry of the Tavis-Cummings model is restored, qualitatively altering the critical phenomena in the superradiant phase due to the presence of a zero-energy mode. To analyze this general regime, we develop a semiclassical theory based on a re-quantization technique. This theory also provides further physical insight on a recently reported anomalous finite critical fluctuations in the time-reversal broken regime. Moving to the open-Dicke case, by introducing local dissipation to the cavities, we observe the emergence of a rich range of nonequilibrium phases characterized by trivial and non-trivial dynamical signatures. In the former case, we identify, when time-reversal symmetry is present, a new stationary phase that features superradiant states in two of the three cavities and a normal state in the other cavity. In the latter case, we observe the emergence of dynamical phases in which the system exhibits superradiant oscillations, characterized by periodic or chaotic phase space patterns. The landscape of transitions associated with these dynamical phases features a wide range of qualitatively different behaviours such as Hopf bifurcations, anomalous Hopf bifurcations, collisions between basins of attraction, and exterior crises. We highlight how the two-critical-scalings feature of the closed model is robust under dissipation while the phenomenon of anomalous finite critical fluctuations becomes a mean-field scaling in the open model.
In recent years there have been significant advances in the study of many-body interactions between atoms and light confined to optical cavities.One model that has received widespread attention of late is the Dicke model, which under certain conditions exhibits a quantum phase transition to a state in which the atoms collectively emit light into the cavity mode, known as superradiance.We consider a generalization of this model that features independently controllable strengths of the corotating and counter-rotating terms of the interaction Hamiltonian.We study this system in the semiclassical (mean field) limit, i.e., neglecting the role of quantum fluctuations.Under this approximation, the model is described by a set of nonlinear differential equations, which determine the system's semiclassical evolution.By taking a dynamical systems approach, we perform a comprehensive analysis of these equations to reveal an abundance of complex dynamics.Examples of the phenomena that we observe are the emergence of superradiant oscillations arising due to Hopf bifurcations, and the appearance of a pair of chaotic attractors arising from period-doubling cascades, followed by their collision to form a single, larger chaotic attractor via a sequence of infinitely many homoclinic bifurcations.Moreover, we find that a flip of the collective spin can result in the sudden emergence of chaotic dynamics.Overall, we provide a comprehensive road map of the possible dynamics that arise in the unbalanced, open Dicke model in the form of a phase diagram in the plane of the two interaction strengths.Hence, we lay out the foundations to make further advances in the study of the fingerprint of semiclassical chaos when considering the master equation of the unbalanced Dicke model, thus, providing the possibility of studying a manifestation of quantum chaos in a specific, experimentally realizable system.
We study the nonequilibrium steady states of an open anisotropic quantum Rabi trimer. Combining semiclassical and quantum mechanical treatments, we map out the system's phase diagram and elucidate the critical phenomena induced by anisotropic light-matter coupling, cavity dissipation, and complex photon hopping, which give rise to abundant multistable phases. Counterintuitively, the frustrated superradiant phase (FSP) can be stabilized by both positive and negative photon hopping, a feature absent in closed Rabi and Dicke trimers. We further uncover two independent dissipation thresholds for the normal superradiant phase and the FSP. Unlike isotropic open quantum Rabi trimers, both phases are suppressed once the dissipation exceeds their respective critical values. The rotating and counter-rotating interaction terms exhibit mutually reciprocal effects on the quantum phase transitions. By analyzing universal scaling behaviors with quantum fluctuations incorporated, we reveal an unprecedented finite-fluctuation critical exponent for the FSP. Moreover, the critical exponents of individual phases are coupling-strength dependent. The multistability and FSP can be tuned by anisotropy and dissipation. Our results broaden the scope of nonequilibrium quantum phase physics in few-body systems and hold promising applications for quantum state engineering and cavity/circuit quantum electrodynamics.
In 1973 Klaus Hepp and Elliott Lieb showed that a tightly confined ensemble of atoms placed in a quantised single-mode optical cavity will have their emission of light enhanced by constructive interference of emission events if the photons emitted are indistinguishable. This effect, known as superradiance, has proven difficult to realise experimentally due to the strong light-matter coupling required to produce such behaviour. However, over the last decade there have been several successful realisations which engineer superradiance by driving Raman transitions between atomic ground states of multilevel atoms. In this case, superradiance emerges via a quantum phase transition mediated by the laser driving power. In this work, we consider a generalisation of this model referred to as the unbalanced Dicke model. It has recently been implemented experimentally and is characterised by two lasers driving two distinct Raman transitions. We show that, in the semiclassical limit of a large number of atoms, the unbalanced Dicke model exhibits a wealth of nonlinear dynamics which describe novel dynamical phases of matter. Examples of nonlinear behaviour observed are pitchfork, saddle-node, and Hopf bifurcations, as well as two types of chaos. We explore the quantum mechanical manifestations of these bifurcations and additional physical effects which appear in the presence of quantum fluctuations. In this way, the model creates a playground in which to explore the onset of classical nonlinear dynamics from an open quantum system.
We study the complex nonlinear dynamics of the two-photon Dicke model in the semiclassical limit by considering cavity and qubit dissipation. In addition to the normal and super-radiant phases, another phase that contains abundant chaos-related phenomena is found under balanced rotating and counter-rotating couplings. In particular, chaos may manifest itself through period-doubling bifurcation, intermittent chaos, or quasi-periodic oscillation, depending on the value of qubit frequency. Transition mechanisms that exist in these three distinct routes are investigated through the system's long-time evolution and bifurcation diagram. Additionally, we provide a comprehensive phase diagram detailing both the existence of stable fixed points and the aforementioned chaos-related dynamics.
Quantum optics is the field of physics that studies the interaction between light and matter under a fully quantum mechanical treatment. In recent decades, relentless advances in the technologies used for trapping, cooling, and controlling atoms and molecules have allowed us to finally start exploring experimentally the physics displayed by different cornerstone models of quantum optics originally proposed in the second half of the 20th century. In this thesis, we propose multiple extensions to those fundamental models, expanding the already interesting physics displayed by them into new and exciting directions. More specficially, we study these generalized models in the context of quantum phase transitions both in and out of equilibrium and show how new phases of matter can be unlocked in these extended models. In Chapters 1 and 2 we briefly introduce the reader to the realms of quantum phase transitions and quantum optics. Once the fundamental aspects of both of these fields are covered, we present the superradiant phase transition displayed in the Dicke and Rabi models in Chapter 3. This phase transition will be the central topic we will be orbiting around in the subsequent chapters. In Chapter 4 we propose a generalization of the quantum Rabi model, where N cavities, instead of one, are connected to each other through photon hopping. In this system, named the quantum Rabi ring, interesting chiral superradiant phases can develop as a function of the hopping phase and the geometry of the ring. In particular, we find that geometrical frustration plays a key role in determining the stable phases in equilibrium. Moreover, frustration manifests itself in the quantum Rabi ring through unconventional non-symmetric critical exponents, a phenomenon reported before, but hardly observed in condensed matter materials. Finally, in Chapter 5, we introduce a different extension to the Dicke model where instead of two-level atoms, three-level atoms are considered. In this system, which we have named the tricritical Dicke model, the superradiant phase transition can occur through first-order, second-order, and third-order critical points. We study the critical properties of the system in and out of equilibrium and find that in the open-system description, the tricritical points are still present but are now accompanied by regions of bistability where the final fate depends highly on the initial conditions. These regions of bistability represent potentially interesting environments to investigate dynamical features and steady-state preparation schemes. The critical phenomena displayed by the extended models proposed here, such as multicriticality, geometrically frustrated quantum phases, and chiral phases breaking time-reversal symmetry, are all features that have been observed, although not abundantly, or proposed in condensed matter physics. However, the unmatched tunability and control of atomic and molecular experimental platforms, where the models presented in this thesis are proposed to be realized, causes these extended models to become promising candidates for investigating these features in parameter regimes and conditions never explored before.