Collective light scattering in dense atomic ensembles: sub and super-radiance

Charlie-Ray Mann, Francesco Andreoli, Vladimir I. Protsenko +2 more

A novel way to create efficient atom-light interfaces is to engineer collective atomic states that selectively radiate into a target optical mode by suppressing emission into undesired modes through destructive interference. While it is generally assumed that this approach requires dense atomic arrays with sub-wavelength lattice constants, here we show that selective radiance can also be achieved in arrays with super-wavelength spacing. By stacking multiple two-dimensional arrays we find super-wavelength mirror configurations where one can eliminate emission into unwanted diffraction orders while enhancing emission into the desired specular mode, leading to near-perfect reflection of weak resonant light. These super-wavelength arrays can also be functionalized into efficient quantum memories, with error probabilities on the order of ~1 for a trilayer with only around ~100 atoms per layer. Relaxing the previous constraint of sub-wavelength spacing could potentially ease the technical requirements for realizing efficient atom-light interfaces, such as enabling the use of tweezer arrays.

Antoine Browaeys

James Keaveney

Stefan Richter, Sebastian Wolf, Joachim von Zanthier +1 more

Modification of spontaneous decay in space and time is a central topic of quantum physics. It has been predominantly investigated in the context of cavity quantum electrodynamics (QED), gaining new interest recently in the domain of nano-optics. Beyond cavity-QED, spontaneous emission may be modified also in free space due to correlations among the photon emitters, a phenomenon known as super- and sub-radiance. Correlations may stem either from direct interactions between the particles, from long-range exchange of photons, or by measuring single photons in a common mode. Yet, the genuine spatial spontaneous emission pattern of an atomic ensemble in an entangled quantum state has not been observed so far, due to the lack of ultra-fast cameras with high spatial resolution suited for recording single photons from single atoms. Preparing two trapped ions in free space in entangled Dicke states via photon detection, we study the resulting collective spontaneous emission patterns. Depending on the symmetry of the Dicke states, associated with the direction of detection of the first state-determining photon, we observe fundamentally different emission patterns for the subsequently scattered photon, including super- and sub-radiance. Our results demonstrate that the detection of a single photon can profoundly modify the collective emission of an atomic array, here represented by its most elementary building block of two atoms in free space.

J. H. Macek

Laszlo Rassaert, Tommaso Roscilde

Super-radiance is a striking phenomenon resulting from the collective interaction of emitters with light, and it is fundamentally related to the appearance of long-range correlations between the dipole moments of the emitters. As such, it represents a distinct phase of dissipative many-body systems compared to the case of independent emitters, similarly to how ferromagnetism stands out in magnetic materials in contrast to paramagnetism. In this work we address the conditions under which the transition to super-radiance can occur in ensembles of emitters subject to dephasing and individual decay -- a situation which is particularly relevant to the case of emitters in the solid state. The simplifying assumption of an ensemble of permutationally invariant emitters allows for the efficient solution of both the dissipative dynamics after a pulsed excitation, as well as of the steady state under incoherent pumping. This exact solution allows us to benchmark a truncated cumulant expansion approach, which can give predictions for arbitrarily big system sizes. We show that super-radiance is fundamentally robust to sizable dephasing and non-radiative decay rates, both under a pulsed excitation, as well as under continuous pumping. This robustness is the result of the collective acceleration effect of super-radiant emission with respect to the individual coupling to a local environment. We establish the universal critical scaling laws at the transition between normal radiance and super-radiance; and we show that, in the super-radiant phase, significant finite-size crossovers can be observed before reaching the asymptotic scaling regime. Our results pave the way for future experiments to provide a quantitative characterization of the scaling properties of super-radiance, seen as a distinct non-equilibrium many-body phase in ensembles of incoherently pumped emitters.