The superconducting nanowire single photon detector (SNSPD) is currently one of the best detectors with comprehensive performance in the mid-infrared wavelength, which has been widely used in quantum optics, LiDAR, and biological fluorescence detection. To develop new devices with excellent performance, the photon detection mechanism of SNSPD still needs further research. Here we find that the single quantum phase slip is the dominating mechanism leading to dark-count and photon-response events in SNSPD below the quantum temperature. We fabricate the nanowire with a length of 7.5 μm and a width of 25 nm using niobium nitride film with a thickness of 5 nm. The distribution of the superconducting switching current is measured as a function of temperature at temperatures ranging from 0.3 to 7 K. We observe single quantum phase slips in the nanowire at the temperature below 1.2 K, and we further investigate the quantitative relationship between the single quantum phase slip rate and the superconducting switching rate of the nanowire under the laser illumination. Experimental results show that the single quantum phase slip is a significant factor leading to photon response and dark counts in the nanowire below the quantum temperature. Our research helps to further reveal the photon detection mechanism of the SNSPD, laying a theoretical foundation for the development of high-performance SNSPD.
The superconducting nanowire single photon detector (SNSPD) is currently one of the best detectors with comprehensive performance in the mid-infrared wavelength, which has been widely used in quantum optics, LiDAR, and biological fluorescence detection. To develop new devices with excellent performance, the photon detection mechanism of SNSPD still needs further research. Here we find that the single quantum phase slip is the dominating mechanism leading to dark-count and photon-response events in SNSPD below the quantum temperature. We fabricate the nanowire with a length of 7.5 μm and a width of 25 nm using niobium nitride film with a thickness of 5 nm. The distribution of the superconducting switching current is measured as a function of temperature at temperatures ranging from 0.3 to 7 K. We observe single quantum phase slips in the nanowire at the temperature below 1.2 K, and we further investigate the quantitative relationship between the single quantum phase slip rate and the superconducting switching rate of the nanowire under the laser illumination. Experimental results show that the single quantum phase slip is a significant factor leading to photon response and dark counts in the nanowire below the quantum temperature. Our research helps to further reveal the photon detection mechanism of the SNSPD, laying a theoretical foundation for the development of high-performance SNSPD.
Single photon detection advanced rapidly in the last decade. The superconducting nanowire single-photon detector (SNSPD) is an emerging technology, which offers low dark count rates, broadband sensitivity from visible to mid-infrared wavelengths and very high quantum efficiency. All these features are appealing for future emerging applications in remote gas sensing, quantum key distribution and quantum information processing. By enclosing the detector in an optical cavity, tuned to the operating wavelength, the total system detection of the SNSPD is improved. Based on the cavity design, the detector absorption is boosted at the desired experimental wavelength. Devices have been fabricated and tested, in this thesis, with enhanced detection efficiency at near-infrared, infrared and mid-infrared wavelengths. NbTiN detectors fabricated on Ta2O5 / SiO2 distributed Bragg reflectors (DBR) for front-side coupling exhibit a system detection efficiency of ≈ 90% at λ = 940 nm for the best device measured. SNSPDs were also fabricated in NbTiN on metallic mirrors for back-side coupling for 1550 and 2333 nm experimental wavelengths. The first design exhibited a system detection efficiency of ≈ 84.5%, at λ = 1550 nm for the best device measured. The second exhibited low system detection efficiency since the device suffered from unexpectedly high dark count rate mainly due to blackbody radiation at 2.2 K. However, it was possible to measure the timing jitter of this device at 350 mK indicating a FWHM of 84 ps. Another technique to improve the total system detection efficiency of the SNSPD, is by fabricating a hairpin-shaped nanowire atop a single mode waveguide. In this design, photons travel through the waveguide and via evanescent coupling are absorbed in the nanowire. These SNSPD devices have been designed to thread along single mode Si ridge waveguides using a hairpin-shaped nanowire structure, which offers enhanced coupling and absorption efficiency via evanescent coupling. These ultra-thin superconducting MoSi detectors are precisely patterned on top of a single mode Si waveguide (600 nm) with alignment error less than 40 nm. Low temperature electrical and nano-optical characterization was carried out using a two-stage pulse tube (PT) coldhead, using an additional 4He / 3He sorption pump, low vibration characterization of SNSPD devices at 350 mK was carried out. Characterised devices exhibit low dark count rate <5 counts per second and timing jitter of ≈ 83 ps full width half maximum (FWHM) at wavelength (λ) = 1550 nm and at critical current ≈ 30 µA.
Superconducting nanowire single photon detector (SNSPD) plays a significant role in plenty of fields such as quantum information, deep space laser communication and lidar, while the mechanism of the photon response process still lacks a recognized theory. It is prerequisite and essential for fabricating high-performance SNSPD to understand in depth and clarify the photon response mechanism of the SNSPD. As mature theories on the SNSPD response progress, hot-spot model and vortex-based model both have their disadvantages: in the former there exists the cut-off wavelength and in the later there is the size effect, so they both need further improving. The Cut-off wavelength means that the detection efficiency of the SNSPD drops to zero with the increase of light wavelength, which is indicated by the hot-spot model but not yet observed in experiment. The size effect implies that the vortex does not exist in the weak link with the width less than 4.41ξ, where ξ is the GL coherence length. Phase slip is responsible for the intrinsic dissipation of superconductors, which promises to expound the SNSPD photon response progress and to establish a complete theory. This paper reviews and discusses the fundamental conception, the development history and the research progress of the hot-spot models, i.e. the vortex-based model and the superconductor phase slips, providing a reference for studying the SNSPD photon response mechanism.
The realization of an ultralow-dark-count rate (DCR) along with the conservation of high detection efficiency (DE) is critical for many applications using single photon detectors in quantum information technologies, material sciences, and biological sensing. For this purpose, a fiber-coupled superconducting nanowire single-photon detector (SNSPD) with a meander-type niobium nitride nanowire (width: 50 nm) is studied. Precise measurements of the bias current dependence of DE are carried out for a wide spectral range (from 500 to 1650 nm in steps of 50 nm) using a white light source and a laser line Bragg tunable band-pass filter. An ultralow DCR (0.0015 cps) and high DE (32%) are simultaneously achieved by the SNSPD at a wavelength of 500 nm.
The intrinsic mechanism of absorbing photons in superconductors reveals the interaction between photons and Cooper pairs, which is of great significance for developing new superconducting nanowire single photon detectors (SNSPDs). Here we propose a photon-assisted phase slip model to describe the interaction mechanism between photons and superconductors. In this model, incident photons destroy large quantities of Cooper pairs and reduce the free-energy barrier of the phase slip, resulting in proliferation in the phase slip events and leading to superconducting transition. The switching rates from the superconducting state of a niobium nitride nanowire under various photon irradiation and temperatures are calculated through the distribution of switching currents in the experiment. The experimental data can be well fitted by our deduced expression of phase slip rate after eliminating the influence of external noise.
Abstract Superconducting Nanowire Single-Photon Detectors (SNSPDs) are key building blocks for photonic quantum technologies due to their ability to detect single photons with ultra-high efficiency, low dark counts and fast temporal resolution. Superconducting materials exhibiting high uniformity, large absorption cross-section and atomic-scale thickness are desirable to extend single-photon detection from the near-infrared up to the terahertz regime, where existing material choices are especially constrained. Substrate independence would further open the way to integrating detectors onto functional materials and heterostructures, enhancing performance and enabling proximal readout of a wide range of individual excitations. Here, we pattern the prototypical two-dimensional superconductor niobium diselenide (NbSe 2 ) into few-layer nanowires less than 100 nm wide and demonstrate single-photon detection at 780 nm and 1550 nm. At the same time, the dark-count rate remains below 1 Hz up to the switching current and we achieve a timing jitter below 50 ps. We estimate via a diffusive hot-spot model that materials and geometric parameters would allow a theoretical cut-off wavelength in the millimetre range, assuming state-of-the-art device parameters. Our results open up routes toward quantum-limited detectors integrated into quantum-photonic circuits and quantum devices, with the potential for novel detection capabilities and unprecedented energy sensitivity.
Superconducting nanowire single photon detectors (SNSPD) offer excellent performance for infrared single photon detection, combining high efficiency, low timing jitter, low dark count rates and high photon counting rates. Promising application areas for SNSPDs include quantum key distribution, space-to-ground communications and single photon remote sensing [1]. SNSPDs are typically made with ultrathin niobium nitride (NbN) films with thickness 4 nm and a superconducting transition temperature above 9 K. NbN offers high performance in the near infrared but their sensitivity drops at wavelengths beyond 2 um. There is growing interest in potential photon counting applications in the mid infrared domain (for example remote sensing of greenhouse gases in the atmosphere [2]). One way to overcome the wavelength limit in NbN SNSPDs is to use films with a lower superconducting energy gap [3]. Here we report on the study of SNSPDs fabricated with thin films of titanium nitride (TiN). We compare TiN films deposited by atomic layer deposition (ALD) and by magnetron sputtering. The TiN films range in thickness from 5 to 60 nm, with superconducting transition temperatures from ~1 K to 3.5 K. We have analyzed the films via transmission electron microscopy and variable angle spectroscopic ellipsometry. We characterize TiN SNSPDs performance from near to mid-infrared at wavelengths (1-4 um) with fast optical parametric oscillator (OPO) source. We compare the performance of TiN SNSPDs to devices based on other lower gap materials: MoSi, NbTiN, WSi. [1] Natarajan et al Superconductor Science and Technology 25 063001 (2012) [2] Abshire et al Laser Applications to Chemical, Security and Environmental Analysis, (Optical Society of America, 2008) paper LMA4 [3] Verma et al Applied Physics Letters 105 022602 (2014)