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MATSUS Spring Conference

Cooperative emission from solid-state quantum emitters

Moritz Cygorek

Published Dec 18, 2023• 0 citations
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Abstract

Cooperative emission from solid-state quantum emittersMoritz Cygorek aa 1Open Quantum Systems Group, Technical University of Dortmund, 44227 Dortmund, GermanyMaterials for Sustainable Development Conference (MATSUS)Proceedings of MATSUS Spring 2024 Conference (MATSUS24)#PeroQuant24 - Halide perovskites for quantum technologiesBarcelona, Spain, 2024 March 4th - 8thOrganizers: Simon Boehme, Sascha Feldmann and Maksym KovalenkoInvited Speaker, Moritz Cygorek, presentation 555DOI: https://doi.org/10.29363/nanoge.matsus.2024.555Publication date: 18th December 2023Novel growth and fabrication technologies allow for an unprecedented level of control over nanoscale semiconductor quantum devices. Recently, several groups have demonstrated samples where multiple quantum dots can be tuned into resonance [1,2]. When multiple quantum emitters become indistinguishable, collective quantum effects like superradiance and measurement-induced cooperative emission [2] emerge due to entanglement between the emitters. A detailed understanding of the signatures of cooperative emission is challenging for several reasons: First, close-to-identical emitters operate in a regime where non-degerate perturbation theory breaks down. Second, real-world quantum devices typically strongly interact with local phonon baths as well as with a global photonic environment, and the different environments generally influence each other. Moreover, the presence of ad- ditional imperfections like spectral wandering further obfuscates the physical picture. Nevertheless, for few emitters, the problem of cooperative emission in the presence of multiple environments can be solved numerically exactly using the process tensor (PT) formalism [3,4]. Here, I report on recent theoretical and experimental findings and summarize the current understanding of cooperative emission in semiconductor nanostructures. This in- cludes the discussion of how genuine superradiance can be distinguished from measurement- induced cooperative emission, how to interpret peaks in g(2) photon correlation experi- ments, and why inter-emitter correlations remain strong for long times despite strong interactions with phonons. References:[1] J.-H. Kim, S. Aghaeimeibodi, C. J. K. Richardson, R. P. Leavitt, E. Waks, Nano Lett. 18, 4734 (2018).[2] Z.X. Koong, M. Cygorek, E. Scerri, T. S. Santana, S. I. Park, J. D. Song, E. M. Gauger, B. D. Gerardot, Sci. Adv. 8, abm8171 (2022).[3] M. Cygorek, M. Cosacchi, A. Vagov, V. M. Axt, B. W. Lovett, J. Keeling, E. M. Gauger, Nature Physics 18, 662 (2022).[4] J. Wiercinski, E. M. Gauger, M. Cygorek, Phys. Rev. Research 5, 013176 (2023)© FUNDACIO DE LA COMUNITAT VALENCIANA SCITOnanoGe is a prestigious brand of successful science conferences that are developed along the year in different areas of the world since 2009. Our worldwide conferences cover cutting-edge materials topics like perovskite solar cells, photovoltaics, optoelectronics, solar fuel conversion, surface science, catalysis and two-dimensional materials, among many others.nanoGe Fall MeetingnanoGe Fall Meeting (NFM) is a multiple symposia conference celebrated yearly and focused on a broad set of topics of advanced materials preparation, their fundamental properties, and their applications, in fields such as renewable energy, photovoltaics, lighting, semiconductor quantum dots, 2-D materials synthesis, charge carriers dynamics, microscopy and spectroscopy semiconductors fundamentals, etc.nanoGe Spring MeetingThis conference is a unique series of symposia focused on advanced materials preparation and fundamental properties and their applications, in fields such as renewable energy (photovoltaics, batteries), lighting, semiconductor quantum dots, 2-D materials synthesis and semiconductors fundamentals, bioimaging, etc.International Conference on Hybrid and Organic PhotovoltaicsInternational Conference on Hybrid and Organic Photovoltaics (HOPV) is celebrated yearly in May. The main topics are the development, function and modeling of materials and devices for hybrid and organic solar cells. The field is now dominated by perovskite solar cells but also other hybrid technologies, as organic solar cells, quantum dot solar cells, and dye-sensitized solar cells and their integration into devices for photoelectrochemical solar fuel production.Asia-Pacific International Conference on Perovskite, Organic Photovoltaics and OptoelectronicsThe main topics of the Asia-Pacific International Conference on Perovskite, Organic Photovoltaics and Optoelectronics (IPEROP) are discussed every year in Asia-Pacific for gathering the recent advances in the fields of material preparation, modeling and fabrication of perovskite and hybrid and organic materials. Photovoltaic devices are analyzed from fundamental physics and materials properties to a broad set of applications. The conference also covers the developments of perovskite optoelectronics, including light-emitting diodes, lasers, optical devices, nanophotonics, nonlinear optical properties, colloidal nanostructures, photophysics and light-matter coupling.International Conference on Perovskite Thin Film Photovoltaics Perovskite Photonics and OptoelectronicsThe International Conference on Perovskite Thin Film Photovoltaics Perovskite Photonics and Optoelectronics (NIPHO) is the best place to hear the latest developments in perovskite solar cells as well as on recent advances in the fields of perovskite light-emitting diodes, lasers, optical devices, nanophotonics, nonlinear optical properties, colloidal nanostructures, photophysics and light-matter coupling.

DOI
10.29363/nanoge.matsus.2024.555

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Cooperative emission from solid-state quantum emittersMoritz Cygorek aa 1Open Quantum Systems Group, Technical University of Dortmund, 44227 Dortmund, GermanyMaterials for Sustainable Development Conference (MATSUS)Proceedings of MATSUS Spring 2024 Conference (MATSUS24)#PeroQuant24 - Halide perovskites for quantum technologiesBarcelona, Spain, 2024 March 4th - 8thOrganizers: Simon Boehme, Sascha Feldmann and Maksym KovalenkoInvited Speaker, Moritz Cygorek, presentation 555DOI: https://doi.org/10.29363/nanoge.matsus.2024.555Publication date: 18th December 2023Novel growth and fabrication technologies allow for an unprecedented level of control over nanoscale semiconductor quantum devices. Recently, several groups have demonstrated samples where multiple quantum dots can be tuned into resonance [1,2]. 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Research 5, 013176 (2023)© FUNDACIO DE LA COMUNITAT VALENCIANA SCITOnanoGe is a prestigious brand of successful science conferences that are developed along the year in different areas of the world since 2009. Our worldwide conferences cover cutting-edge materials topics like perovskite solar cells, photovoltaics, optoelectronics, solar fuel conversion, surface science, catalysis and two-dimensional materials, among many others.nanoGe Fall MeetingnanoGe Fall Meeting (NFM) is a multiple symposia conference celebrated yearly and focused on a broad set of topics of advanced materials preparation, their fundamental properties, and their applications, in fields such as renewable energy, photovoltaics, lighting, semiconductor quantum dots, 2-D materials synthesis, charge carriers dynamics, microscopy and spectroscopy semiconductors fundamentals, etc.nanoGe Spring MeetingThis conference is a unique series of symposia focused on advanced materials preparation and fundamental properties and their applications, in fields such as renewable energy (photovoltaics, batteries), lighting, semiconductor quantum dots, 2-D materials synthesis and semiconductors fundamentals, bioimaging, etc.International Conference on Hybrid and Organic PhotovoltaicsInternational Conference on Hybrid and Organic Photovoltaics (HOPV) is celebrated yearly in May. The main topics are the development, function and modeling of materials and devices for hybrid and organic solar cells. The field is now dominated by perovskite solar cells but also other hybrid technologies, as organic solar cells, quantum dot solar cells, and dye-sensitized solar cells and their integration into devices for photoelectrochemical solar fuel production.Asia-Pacific International Conference on Perovskite, Organic Photovoltaics and OptoelectronicsThe main topics of the Asia-Pacific International Conference on Perovskite, Organic Photovoltaics and Optoelectronics (IPEROP) are discussed every year in Asia-Pacific for gathering the recent advances in the fields of material preparation, modeling and fabrication of perovskite and hybrid and organic materials. Photovoltaic devices are analyzed from fundamental physics and materials properties to a broad set of applications. The conference also covers the developments of perovskite optoelectronics, including light-emitting diodes, lasers, optical devices, nanophotonics, nonlinear optical properties, colloidal nanostructures, photophysics and light-matter coupling.International Conference on Perovskite Thin Film Photovoltaics Perovskite Photonics and OptoelectronicsThe International Conference on Perovskite Thin Film Photovoltaics Perovskite Photonics and Optoelectronics (NIPHO) is the best place to hear the latest developments in perovskite solar cells as well as on recent advances in the fields of perovskite light-emitting diodes, lasers, optical devices, nanophotonics, nonlinear optical properties, colloidal nanostructures, photophysics and light-matter coupling.
Among different solid-state emitters of quantum light, epitaxial GaAs quantum dots (QDs) have recently emerged as nearly-ideal sources of triggered polarization entangled photon pairs [1]. This property, combined with the strongly suppressed probability of multiphoton emission under resonant excitation [2] has allowed the implementation of quantum teleportation using photons subsequently emitted by a single QD [3]. In this talk I will discuss the peculiar properties of GaAs QDs [4,5], their performance as emitters of both single and entangled photons, as well as possible methods to engineer their light emission characteristics [1,4] to meet the demanding requirements imposed by photonic quantum technologies. [1] D. Huber et al. Phys. Rev. Lett. 121, 033902 (2018). [2] L. Schweickert et al. Appl. Phys. Lett. 112, 093106 (2018). [3] M. Reindl et al. Science Adv. (2018). [4] X. Yuan et al. Nat. Comm. 9, 3058 (2018). [5] M. Reindl et al. https://arxiv.org/abs/1901.11251.
Even though the quantized interaction between light and matter in the photoelectric effect is considered one of the cornerstones in the development of quantum mechanics, it was long thought impossible to directly observe the quantized nature of light itself. The advent of light-intensity autocorrelation techniques in the 1950s, first developed to study the size of stars, changed little in this perception, until true single-photon correlation spectroscopy from trapped ions was proven to be possible in the late 1970s: Photons from a single quantum emitter tend to arrive in bunches, but each light quantum is spaced apart in time—it is antibunched. Initially considered only as the workhorse of atomic quantum optics, over the past two decades, photon correlation techniques have become a standard in fields as diverse as quantum-information processing, biological imaging, polymer physics, and materials science, in general. The technique is particularly useful for probing materials that are specifically designed to emit or absorb light in optoelectronic devices, such as light-emitting diodes, solar cells, or lasers. The central question in such studies is how large a mesoscopic piece of material can become and still behave as an atom-like source of single photons. What interactions may arise between multiple excitations within a material, and what sort of dark states may give rise to intermittency in the stream of photons? We review the many different classes of optoelectronic materials for which photon-correlation spectroscopy has proven to offer useful insight into excited-state dynamics, ranging from molecular, over semiconductor to metallic nanostructures. The technique is particularly suited to probing mesoscopic aggregates of organic semiconductors since each single molecule acts as a quantum emitter itself.
For future quantum technologies and in particular for quantum architecture systems, one needs to consider scalability and reproducibility in order to be able to handle and add easily as many qubits of information as possible on a given platform. Quantum coherence and quantum information are fragile and thus requires the need for many qubits to be created, to interact and quantum information to be preserved. Currently there are either very good qubits in terms of fidelity but poor scalability or very good scalability but poor fidelity thus requiring more qubits to compensate. Most of the current platforms are in solid-state physics such as superconducting, dopants in silicon, quantum dots in III-V semiconductors or defects in diamond. The main interest for condensed matter systems is the fact that it is potentially scalable as integration is possible in the future, already demonstrated in the ‘classical’ semiconductor industry. Nevertheless, there are some true challenges in controlling and understanding the mechanisms of decoherence, losses and unwanted effects in these ‘dirty’ systems. As quantum technologies require ultimate control of quantum effects such as maintaining quantum coherence, quantum superposition and entanglement, it pushes towards deeper knowledge of underlying material and condensed matter physics. Photons are of particular interest as they are good carriers of quantum information and one aim is to explore a fully integrated photonic quantum circuit which would be a hybrid system made of stationary solid-state qubits (we will call them quantum emitters) coupled together via single photons travelling within a common optical bus that is photonics-ready for quantum communications within a network of quantum nodes. In this presentation, we will present our latest developments and results towards the integration of quantum emitters with photonic structures with nanosize features. In the first part, our platform is described which consists of glass and thus directly compatible with optical fibres. It is based on the technique of exchanged ions within the glass in order to create locally a particular confinement of the light. The next part will concern our latest results on two different quantum emitters. The first one is based on perovskite nanocristals that can be synthetised chemically and giving rise to quantum optics-type of emitters. The second one is based on the so-called silicon-vacancy defect centre in nanodiamonds. These emitters are produced by the high-pressure/high-temperature method and lead to promising results for quantum technologies. Finally, the last part will treat the nanophotonics approaches in order to couple efficiently these emitters with our platform.
Abstract Photonic quantum science—which harnesses light-matter interactions down to the single photon level—provides advanced light sources for quantum sensing, communication, and computing. Integrating solid-state light sources on a photonic chip provides a means of creating scalable on-chip quantum networks with sophisticated optoelectronic circuitry. Extending beyond single emitters to multi-emitter systems is a frontier that offers substantial opportunities for fundamental scientific advances as well as applications that require multi-emitter quantum states. A key challenge in this endeavor is the spectral inhomogeneity of solid-state emitters, which results in non-identical emitters that cannot be interfaced with one another. This review describes recent advances in tailoring the emission properties of individual emitters and the multi-emitter demonstrations that are enabled by this control for a variety of prominent materials, as well as prospects for further development.
Superradiance is one of the many fascinating phenomena predicted by quantum electrodynamics that have first been experimentally demonstrated in atomic systems and more recently in condensed matter systems like quantum dots, superconducting q-bits, cyclotron transitions and plasma oscillations in quantum wells (QWs). It occurs when a dense collection of N identical two-level emitters are phased via the exchange of photons, giving rise to enhanced light-matter interaction, hence to a faster emission rate. Of great interest is the regime where the ensemble interacts with one photon only and therefore all of the atoms, but one, are in the ground state. In this case the quantum superposition of all possible configurations produces a symmetric state that decays radiatively with a rate N times larger than that of the individual oscillators. This phenomenon, called single photon superradiance, results from the exchange of real photons among the N emitters. Yet, to single photon superradiance is also associated another collective effect that renormalizes the emission frequency, known as cooperative Lamb shift. In this work, we show that single photon superradiance and cooperative Lamb shift can be engineered in a semiconductor device by coupling spatially separated plasma resonances arising from the collective motion of confined electrons in QWs. These resonances hold a giant dipole along the growth direction z and have no mutual Coulomb coupling. They thus behave as a collection of macro-atoms on different positions along the z axis. Our device is therefore a test bench to simulate the low excitation regime of quantum electrodynamics.
The emerging field of semiconductor quantum optics combines semiconductor physics and quantum optics, with the aim of developing quantum devices with unprecedented performance. In this book researchers and graduate students alike will reach a new level of understanding to begin conducting state-of-the-art investigations. The book combines theoretical methods from quantum optics and solid-state physics to give a consistent microscopic description of light-matter- and many-body-interaction effects in low-dimensional semiconductor nanostructures. It develops the systematic theory needed to treat semiconductor quantum-optical effects, such as strong light-matter coupling, light-matter entanglement, squeezing, as well as quantum-optical semiconductor spectroscopy. Detailed derivations of key equations help readers learn the techniques and nearly 300 exercises help test their understanding of the materials covered. The book is accompanied by a website hosted by the authors, containing further discussions on topical issues, latest trends and publications on the field. The link can be found at www.cambridge.org/9780521875097.