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Measuring non-linear Faraday rotation in cold atoms in presence of persistent transverse fields using tunable differential imaging

Sujit Garain, Surya Narayan Sahoo, Ashok Kumar Mohapatra

Published Mar 7, 2024• 4 citations

Abstract

Non-linear Faraday rotation in cold atoms promises precision magnetometry due to narrower magnetic resonance linewidth compared to the linear Faraday effect. Imaging techniques based on linear Faraday effect have emerged as a tool to characterize the dynamics of ultracold atomic clouds. Using a camera instead of balanced detectors, we can obtain the spatial distribution of polarization rotation in a uniformly intense optical beam. However, the finite dynamic range of the imaging device limits the sensitivity to measure non-linear Faraday rotation at a given incident power. Here, we experimentally demonstrate a differential imaging technique in which we can tune parameters to improve contrast and the sensitivity to the non-linear Faraday rotation signal by a factor of ≈7 over existing imaging methods. The atomic cloud experiences a uniform optical field even when shifted by persistent magnetic fields making the method robust. This allows us to study the effect of transverse fields on non-linear Faraday rotation in ultra-cold atoms, paving the way toward spatially resolved vector magnetometry.

DOI: 10.1364/oe.509923

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Non-linear Faraday rotation in cold atoms promises precision magnetometry due to narrower magnetic resonance linewidth compared to the linear Faraday effect. Imaging techniques based on linear Faraday effect have emerged as a tool to characterize the dynamics of ultracold atomic clouds. Using a camera instead of balanced detectors, we can obtain the spatial distribution of polarization rotation in a uniformly intense optical beam. However, the finite dynamic range of the imaging device limits the sensitivity to measure non-linear Faraday rotation at a given incident power. Here, we experimentally demonstrate a differential imaging technique in which we can tune parameters to improve contrast and the sensitivity to the non-linear Faraday rotation signal by a factor of ≈7 over existing imaging methods. The atomic cloud experiences a uniform optical field even when shifted by persistent magnetic fields making the method robust. This allows us to study the effect of transverse fields on non-linear Faraday rotation in ultra-cold atoms, paving the way toward spatially resolved vector magnetometry.

We describe an easily implementable method for non-destructive measurements of ultracold atomic clouds based on dark field imaging of spatially resolved Faraday rotation. The signal-to-noise ratio is analyzed theoretically and, in the absence of experimental imperfections, the sensitivity limit is found to be identical to other conventional dispersive imaging techniques. The dependence on laser detuning, atomic density, and temperature is characterized in a detailed comparison with theory. Due to low destructiveness, spatially resolved images of the same cloud can be acquired up to 2000 times. The technique is applied to avoid the effect of shot-to-shot fluctuations in atom number calibration, to demonstrate single-run vector magnetic field imaging and single-run spatial imaging of the system's dynamic behavior. This demonstrates that the method is a useful tool for the characterization of static and dynamically changing properties of ultracold atomic clouds.

We report on the observation of nonlinear Faraday rotation with cold atoms at a temperature of

~100

$\ensuremath{\mu}$K. The observed nonlinear rotation of the light polarization plane is up to

0.1

rad over the

1

-mm-size atomic cloud in approximately

10

-mG magnetic field. The nonlinearity of rotation results from long-lived coherence of ground-state Zeeman sublevels created by a near-resonant light. The method allows for creation, detection, and control of atomic superposition states. It also allows applications for precision magnetometry with high spatial and temporal resolution.

We present a differential technique for vector magnetic sensing based on a cold-atom cloud in a magnetic quadrupole trap. An external homogeneous magnetic field displaces the trap center in a direction and magnitude proportional to the field. By reversing the quadrupole polarity between experimental shots and comparing the resulting cloud positions, we extract a differential displacement signal that is free from common-mode effects such as gravity and weak magnetic-field inhomogeneities. The signal is directionally proportional to the external field and requires only absorption imaging, without spectroscopic interrogation. Assuming micron-scale position resolution, the technique enables field resolution at the milli-Gauss level. It offers a practical tool for field compensation in magnetically sensitive experimental stages, bridging operational regimes from Earth-level fields to atomic magnetometry. A straightforward extension to full three-dimensional sensing is possible with only a minimal addition to standard cold-atom infrastructure.

Application of nonlinear magneto-optical (Faraday) rotation to magnetometry is investigated. Our experimental setup consists of a modulation polarimeter that measures rotation of the polarization plane of a laser beam resonant with transitions in Rb. Rb vapor is contained in an evacuated cell with antirelaxation coating that enables atomic ground-state polarization to survive many thousand wall collisions. This leads to ultranarrow features $(\ensuremath{\sim}{10}^{\ensuremath{-}6} \mathrm{G})$ in the magnetic-field dependence of optical rotation. The potential sensitivity of this scheme to sub-$\ensuremath{\mu}\mathrm{G}$ magnetic fields as a function of atomic density, light intensity, and light frequency is investigated near the

D1

and

D2

lines of

{}^{85}\mathrm{Rb}.

It is shown that through an appropriate choice of parameters the shot-noise-limited sensitivity to small magnetic fields can reach $3\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}12} \mathrm{G}/\sqrt{\mathrm{Hz}}.$