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Frontiers in Physics

Experiment and analysis of state preparation for atom interferometry

Xu Zhang, Qixue Li, Huankai Zhang, Ji-Xun Liu, Guo-Chao Wang, Xiaoxiao Ma, Lingxiao Zhu, Shuhua Yan

Published Mar 8, 2024• 2 citations
Publisher

Abstract

The state preparation is a crucial procedure in atom interferometry; however, there is a shortage of detailed experimental studies on determining the optimal method for achieving this. This paper investigates and compares two methods for state preparation: the combined use of microwave and Raman light (M-R) and the combined use of optical pumping, microwave, and Raman light (O-M-W). The experimental results demonstrate that the M-R method improves the efficiency of Raman transitions for atom interference, which is helpful in enhancing the contrast of the interference fringes. The O-M-R method increases the quantity of prepared atoms, thereby enhancing the signal-to-noise ratio of the detected signals. This work helps provide a useful experimental basis and reference for researchers to design a suitable state preparation scheme.

DOI
10.3389/fphy.2024.1377829

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The state preparation is a crucial procedure in atom interferometry; however, there is a shortage of detailed experimental studies on determining the optimal method for achieving this. This paper investigates and compares two methods for state preparation: the combined use of microwave and Raman light (M-R) and the combined use of optical pumping, microwave, and Raman light (O-M-W). The experimental results demonstrate that the M-R method improves the efficiency of Raman transitions for atom interference, which is helpful in enhancing the contrast of the interference fringes. The O-M-R method increases the quantity of prepared atoms, thereby enhancing the signal-to-noise ratio of the detected signals. This work helps provide a useful experimental basis and reference for researchers to design a suitable state preparation scheme.
The coherent control of atomic wave packets in multiple momentum dimensions is a central challenge in Raman atom optics and a key requirement for multidimensional atom interferometry. In this paper, a momentum-basis theoretical framework is developed for two-dimensional Raman interactions. We formulate the atom-laser interaction for two-dimensional Raman beams and obtain the effective two-level ground-state Hamiltonian after adiabatic elimination of the excited states. The resulted Hamiltonian is constructed on the reachable momentum-state lattice and includes AC Stark shifts, intra-dimensional Raman couplings, and cross-dimensional Raman coupling terms, thereby describing multidimensional Raman dynamics beyond a simple superposition of independent single-dimensional models. The framework is used to analyze the principles and operating conditions of two-dimensional atom interferometry. Cross-dimensional Raman coupling and sequential reverse Raman transitions are identified as the main mechanisms that redistribute atoms into non-target momentum states and reduce the contrast of atomic interferometer fringe. Experimentally, Ramsey fringes are observed in a cold-atom fountain interferometer, with a contrast of 14.8%14.8\%14.8% at an interrogation time of T=10 msT=10~{\rm ms}T=10 ms, in good agreement with the theoretical calculation. The conditions required for velocity-sensitive multidimensional atom interferometry are further clarified, including detuning control, velocity-class selection, and suppression of undesired inter-dimensional transitions. This work provides a theoretical and experimental basis for multidimensional Raman atom interferometry.
The presented thesis describes the setting up of an inertial sensitive atom interferometer for navigation using Rubidium 87 atoms, which is able to perform horizontal acceleration measurement. An ultra-high vacuum interferometer chamber is designed and built. The cold atoms are prepared in a compact 2D MOT setup and loaded into the main MOT. These atoms are then cooled down to few K and prepared in a magnetically insensitive ground state using a sequence of optical and microwave pulses, after which atoms are selected in a narrow band of the velocity. A three-pulse Mach-Zehnder ( pi/2 -pi-pi/2) interferometer using stimulated Raman transitions is used to measure the horizontal acceleration. To improve the sensitivity to acceleration, the fringe contrast of the interferometer requires to be optimised. By investigating the intensity profile of the Raman beams using atoms, a procedure is developed to operate the interferometer in an improved condition, which is able to enhance the fringe contrast by a factor of 3. This procedure improves the shot-to-shot sensitivity of the interferometer below 5 um/s^2. In addition, the atom interferometer is compared with a classical state-of-the-art accelerometer.
Imperfect Raman pulses can lead to the formation of multiple interfering paths and affect the output of an atom interferometer in high-precision measurement.We study the effect of the imperfect Raman pulses on the interferometric fringe contrast and the phase shift in the three-pulse atom interferometer by using the evolution operator method.Analytical expressions expanded to the second-order fluctuation of imperfect pulses are derived, in which the effect of coupling the imperfect pulses with laser detuning and pulse duration is also considered.The result indicates that the second-order fluctuation of imperfect pulses is dominant, however, it can be nearly ignored in the current requirements of atomic experiments.Even so, theoretical analysis is very necessary as it may be helpful in proposing some schemes to improve the interference efficiency for future high-precision measurements with atomic interferometry.
The precision of atom interferometry is affected by system errors due to the laser parameters and atomic velocity. We propose the method of the Stimulated Raman Adiabatic Passage(STIRAP) to enhance the accuracy of the atom interferometry and its tolerance for the environment. We calculate the fidelity of the target atomic state for the cases of the STIRAP technique, rectangular pulse and Gaussian pulse. It is shown that the fidelity of the atomic state obtained with the STIRAP technique is higher than that with rectangular pulse and Gaussian pulse. In addition, higher interference fringe contrast of the atom interferometry can be obtained with the pulse sequence consisting of STIRAP than the rectangular pulse sequence and Gaussian pulse sequence. This scheme may have promising applications in precise measurements with atom interferometry.
This cumulative thesis consists of four publications [1-4], presented as three contributions (I) - (III), where the second one (II) consists of the joint publications [2,3]. All publications were written during the author's research activities at the Institute of Quantum Physics under the supervision of Prof. Dr. W. P. Schleich. All of the presented publications consider light-matter interactions and their potential application in atom interferometry, a comparatively young and rapidly evolving technique. Atom interferometers find application in high-precision measurements, the determination of physical constants, the testing of fundamental physics, and the provision of gravimeters and gyroscopes. The advancement of technology and science has led to significant improvements in performance and the development of ambitious mobile and space-based devices. The recent success of several experiments has led to the proposal of further experiments with the aim of opening up new frontiers. However, the construction of future devices necessitates a decision regarding the employed diffraction mechanism and geometry, depending on the specific technical and scientific requirements. Furthermore, it is necessary to enhance the sensitivity of future devices. The contributions in this dissertation address these issues. The first contribution (I) focuses on the diffraction of atoms by laser pulses which can be employed to generate atom-optical diffraction elements like beam splitters and mirrors. These diffraction elements can be combined to construct atom interferometers, which have been successfully employed for precision measurements regarding fundamental physics as well as practical applications. The article presents a numerical comparison of two distinct diffraction mechanisms (Bragg and Raman) and diffraction geometries (single and double diffraction) in microgravity. It discusses the fundamental differences between the mechanisms and geometries with respect to the diffraction efficiency, taking into account the width of the initial wave function and the duration of the light pulse. Additionally, it explores the transition between the two diffraction geometries when starting from an atom initially at rest and increasing its momentum. The results may serve as a reference for experimentalists in selecting the most suitable configuration, based on their aims and requirements in the realization of more advanced atom interferometers. The second contribution (II) is a follow-up to the previous one, but focuses exclusively on a single diffraction type in microgravity, namely the so-called double Raman diffraction. In contrast to the previous article, where we only discussed single two-photon processes, we consider in this article a six-photon process, also known as third-order diffraction, as well as three subsequent two-photon processes, which both lead to the same amount of transferred momentum and can both be used to realize large-momentum transfer (LMT). We demonstrate that third-order double Raman diffraction is a viable and advantageous method for the diffraction of small momentum distributions like Bose-Einstein condensates (BECs) compared to a sequence of three two-photon processes. Furthermore, we show that third-order Raman pulses can be successfully applied to create higher-order Raman atom interferometers. Third-order diffraction can be perfectly combined with other LMT techniques and, moreover, allows for a reduction in the overall duration of the diffraction process and the complexity of the experimental set-up, as only two distinct laser frequencies are required. Moreover, we present a third-order Mach-Zehnder interferometer with spurious paths being disregarded. As demonstrated later on in [3], this interferometer generates optimal contrast and a substantial amplitude. The third contribution (III) extends the semi-classical λ-scheme of single Raman diffraction, as discussed in detail in contribution (I), into a fully quantized multi-atom multi-λ configuration with center-of-mass motion inside a cavity. Therefore, the incorporation of an internal structure allows for a more realistic modeling of the atoms, which is relevant for multi-photon interaction or cooling processes. We use for our analysis the framework of second quantization, i.e., we take into account the field-theoretical nature of the multi-particle atomic field as well as of the diffracting light field. We reduce this model with a Hamiltonian averaging theory applied to the atomic field operators and obtain an effective Hamiltonian, which determines the time evolution of the system. We demonstrate the efficiency of our model by the application of a typical initial state. Moreover, for a specific input state, we obtain the Hong-Ou-Mandel effect simultaneously in the atomic and the optical system. Our many-body formalism is perfectly suited to theoretically describe contemporary high-precision atom interferometric experiments based on entanglement between the atoms, that aim to surpass the shot-noise limit.
The efficiency of an atomic interferometer in proximity of a surface is discussed. We first study which is the best choice of frequency for a pulse acting on internal atomic transitions in the same well. Then, considering the modification of atomic energy levels in vicinity of the surface, we propose the application of two simultaneous Raman lasers and numerically study the associated interference fringes. We show that the efficiency of the interferometric scheme is limited by the existence of a residual phase depending on the atomic path. We propose a symmetric scheme in order to avoid these contributions. We finally show that the suggested modifications make the contrast of the interference fringes close to 1 in any configuration, both close and far from the surface, and with one or more initially populated wells.