Once the concept of chiral molecules was proposed, the task of chiral resolution has accompanied around in the related area. Naturally, scientists need fast and accurate methods to distinguish different chiralities. Here, we show a feasible method based on non-adiabatic holonomic quantum computation (NHQC), which can achieve over 99% discrimination of different chiralities. Based on the original scheme, we studied the modified version, NHQC+. The experimental data proved that it has better robustness than the original protocol, indicating a promising development in the relevant fields.
Once the concept of chiral molecules was proposed, the task of chiral resolution has accompanied around in the related area. Naturally, scientists need fast and accurate methods to distinguish different chiralities. Here, we show a feasible method based on non-adiabatic holonomic quantum computation (NHQC), which can achieve over 99% discrimination of different chiralities. Based on the original scheme, we studied the modified version, NHQC+. The experimental data proved that it has better robustness than the original protocol, indicating a promising development in the relevant fields.
A novel optical method for distinguishing chiral molecules is proposed and validated within a quantum simulator employing a trapped-ion qudit. This approach correlates the sign disparity of the dipole moment of chiral molecules with distinct cyclic evolution trajectories, yielding the unity population contrast induced by the different non-Abelian holonomies corresponding to the chirality. Harnessing the principles of holonomic quantum computation (HQC), our method achieves highly efficient, non-adiabatic, and robust detection and separation of chiral molecules. Demonstrated in a trapped ion quantum simulator, this scheme achieves nearly 100% contrast between the two enantiomers in the population of a specific state, showcasing its resilience to the noise inherent in the driving field.
Abstract A novel optical method for distinguishing chiral molecules is proposed and tested within a quantum simulator employing a trapped-ion qudit. This approach correlates the sign disparity of the dipole moment of chiral molecules with distinct cyclic evolution trajectories, yielding the unity population contrast induced by the different non-Abelian holonomies corresponding to the chirality. Harnessing the principles of holonomic quantum computation, our method can achieve highly efficient, non-adiabatic, and robust detection and separation of chiral molecules. Demonstrated in a trapped 171 Yb + ion testbed, this scheme achieves high contrast in the population of a specific state, showcasing its resilience to the noise inherent in the driving field.
In quantum control, geometrical operations could provide an extra layer of robustness against control errors. However, the conventional non-adiabatic holonomic quantum computation (NHQC) is limited by the fact that all of the operations require exactly the same amount of evolution time, even for a small-angle rotation. Furthermore, NHQC confines the driving part of the Hamiltonian to strictly cover a fixed pulse area, making it sensitive to control errors. Here we present an unconventional approach of NHQC, termed brachistochronic NHQC, for bypassing these limitations. Specifically, with B-NHQC, non-Abelian geometric gates can be time-optimized by following the brachistochrone curve, minimizing the impact from the environmental decoherence. Additionally, we demonstrate that B-NHQC is compatible with composed pulses, which can further enhance the robustness against pulse errors. For benchmarking, we provide a thorough analysis on the performance of B-NHQC under experimental conditions; we found that the gate error can be reduced by as much as 64% compared with NHQC.
Non-adiabatic geometric quantum computation (NGQC) and non-adiabatic holonomic quantum computation (NHQC) have been proposed to reduce the run time of geometric quantum gates. However, in terms of robustness against experimental control errors, the existing NGQC and NHQC scenarios have no advantage over standard dynamical gates in most cases. Here, we give the reasons of why non-adiabatic geometric gates are sensitive to the control errors, and further, we propose a new class of geometric property condition (GPC)-based non-adiabatic geometric gates, in which the global control condition can guarantee both high speed and robustness of geometric gate. To illustrate the working mechanism of GPC-based geometric gates, we give two simple examples of GPC-NGQC and GPC-NHQC for two- and three-level quantum systems, respectively. Theoretical and numerical results with the experimental parameters indicate that our scheme can significantly improve the gate performance comparing with the previous NGQC, NHQC and standard dynamical schemes. GPC-based geometric quantum computation can be applied to various physical platforms such as superconducting qubits, quantum dots, and trapped ions. All of these sufficiently show that our scheme provides a promising way towards robust geometric quantum computation.
The schmeme of nonadiabatic holonomic quantum computation (NHQC) offers an error-resistant method for implementing quantum gates, capable of mitigating certain errors. However, the conventional NHQC schemes often entail longer operations concerning standard gate operations, making them more vulnerable to the effects of quantum decoherence. In this research, we propose an implementation of the Super-Robust NHQC scheme within the Decoherence-Free Subspace (DFS). SR-NHQC has demonstrated robustness against Global Control Errors (GCEs). By utilizing capacitance-coupled transmon qubits within a DFS, our approach enables universal gate operations on a scalable two-dimensional square lattice of superconducting qubits. Numerical simulations demonstrate the practicality of SR-NHQC in DFS, showcasing its superiority in mitigating GCEs and decoherence effects compared to conventional NHQC schemes. Our work presents a promising strategy for advancing the reliability of quantum computation in real-world applications.
Nonadiabatic holonomic quantum computation (NHQC) provides an essential way to construct robust and high-fidelity quantum gates due to its geometric features. However, NHQC is more sensitive to decay and dephasing errors than a conventional dynamical gate since it requires an ancillary intermediate state. Here, we utilize the Hamiltonian reverse engineering technique to study the influence of intermediate-state decoherence on NHQC gate fidelity, and propose schemes to construct an arbitrary single-qubit holonomic gate and nontrivial two-qubit holonomic gate with high fidelity and robustness to the decoherence. Although the proposed method is generic and can be applied to many experimental platforms, such as superconducting qubits, trapped ions, and quantum dots, here we take a nitrogen-vacancy center as an example to show that the gate fidelity can be significantly enhanced from 89% to 99.6% in contrast to recent experimental NHQC schemes [Phys. Rev. Lett. 119, 140503 (2017); Nat. Photonics 11, 309 (2017); Opt. Lett. 43, 2380 (2018)], and the robustness against decoherence can also be significantly improved. All in all, our scheme provides a promising way for fault-tolerant geometric quantum computation.