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Geometric interpretation and experimental test of Leggett inequalities with nonmaximally entangled states

Dongkai Zhang, Xiaodong Qiu, Lixiang Chen

Published Feb 22, 2024• 5 citations
Publisher

Abstract

Leggett inequality states that nonlocal hidden-variable models might still be incompatible with the predictions of quantum physics. However, its theoretical and experimental demonstration is only in the scenario of 2-dimensional maximally entangled systems. An open question remains as to whether the Leggett inequality can be violated by nonmaximally entangled states. Here, we answer this question both in theory and experiment. Specifically, from the point of view of geometry, we theoretically map the problem of maximizing the correlation measure in the Leggett inequality to maximizing the sum of an ellipse’s diameter and semi-diameter axes, accordingly, demonstrating that the violation of the Leggett inequality requires a more robust entanglement than that of Bell’s theory. Experimentally, by leveraging the controllable photonic orbital angular momentum entanglement, we demonstrate the violation of Leggett-type inequalities by more than 8.7 and 4.5 standard deviations under concurrence C = 0.95 and 0.9, respectively. Our observations indicate that, the requirement for quantum correlation should be increased to exclude a particular class of non-local hidden variable theories that abide by Leggett’s model, providing insights into the boundaries of quantum correlation and the limitations imposed by non-local hidden variables.

DOI
10.1364/oe.514423

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Leggett inequality states that nonlocal hidden-variable models might still be incompatible with the predictions of quantum physics. However, its theoretical and experimental demonstration is only in the scenario of 2-dimensional maximally entangled systems. An open question remains as to whether the Leggett inequality can be violated by nonmaximally entangled states. Here, we answer this question both in theory and experiment. Specifically, from the point of view of geometry, we theoretically map the problem of maximizing the correlation measure in the Leggett inequality to maximizing the sum of an ellipse’s diameter and semi-diameter axes, accordingly, demonstrating that the violation of the Leggett inequality requires a more robust entanglement than that of Bell’s theory. Experimentally, by leveraging the controllable photonic orbital angular momentum entanglement, we demonstrate the violation of Leggett-type inequalities by more than 8.7 and 4.5 standard deviations under concurrence C = 0.95 and 0.9, respectively. Our observations indicate that, the requirement for quantum correlation should be increased to exclude a particular class of non-local hidden variable theories that abide by Leggett’s model, providing insights into the boundaries of quantum correlation and the limitations imposed by non-local hidden variables.
We report the experimental violation of Leggett-type inequalities for a hybrid entangled state of spin and orbital angular momentum of a single photon. These inequalities give a physical criterion to verify the possible validity of a class of hidden-variable theories, originally named ``crypto nonlocal,'' that are not excluded by the violation of Bell-type inequalities. In our case, the tested theories assume the existence of hidden variables associated with independent degrees of freedom of the same particle, while admitting the possibility of an influence between the two measurements, i.e., the so-called contextuality of observables. We observe a violation of the Leggett inequalities for a range of experimental inputs, with a maximum violation of seven standard deviations, thus ruling out this class of hidden-variable models with a high level of confidence.
Bell's theorem states that no local hidden-variable model is compatible with quantum mechanics. Surprisingly, even if we release the locality constraint, certain nonlocal hidden-variable models, such as the one proposed by Leggett, may still be at variance with the predictions of quantum physics. Here, we report an experimental test of Leggett's nonlocal model with solid-state spins in a diamond nitrogen-vacancy center. We entangle an electron spin with a surrounding weakly coupled 13C^{13}\mathrm{C}13C nuclear spin and observe that the entangled states violate Leggett-type inequalities by more than four and seven standard deviations for six and eight measurement settings, respectively. Our experimental results are in full agreement with quantum predictions and violate Leggett's nonlocal hidden-variable inequality with a high level of confidence.
Whether quantum mechanics is predictively complete remains a fundamental question in its foundations. While most investigations have concentrated on two-dimensional systems, high-dimensional systems are more general and hold broader applicability. Extending the non-extensibility theorem by Colbeck and Renner [Nat. Commun.2, 411 (2011)10.1038/ncomms1416], we demonstrate that no alternative theory can enhance the predictive power of quantum mechanics in arbitrary dimensions. By linking the maximal predictive power achievable to experimentally observable correlations, we establish optimal experimental bounds exploiting orbital angular momentum entangled photon pairs. These results impose strict constraints and rule out a broad class of hidden-variable models, including Bell-type and Leggett-type theories, thereby reinforcing the completeness of quantum theory and advancing high-dimensional quantum cryptography.
Nonmaximally entangled states are pivotal for quantum technologies, offering enhanced noise resilience and resource efficiency for quantum communication tasks. However, the maximum violation of the multisetting Clauser–Horne–Shimony–Holt (CHSH) inequality in nonmaximally entangled systems has yet to be explored, primarily due to the algebraic complexity associated with such systems. Herein, it is demonstrated that the maximization of the correlation measure in the three‐setting CHSH inequality, for both pure and mixed states, can be elegantly reformulated as a geometric optimization problem: maximizing the perimeter of a triangle inscribed within an ellipse. Leveraging this analytical insight, the maximum violation of the three‐setting CHSH inequality using photonic orbital angular momentum entanglement and spatial light modulators for precise intensity measurements is experimentally realized, observing that the Bell parameter diminishes to the classical bound as entanglement decreases. The findings shed new light on optimal measurement strategies for nonmaximally entangled states, demonstrating conclusively that phase‐only measurements are insufficient for achieving maximum violations in such states. Thus, the work may offer valuable guidance for harnessing nonmaximally entangled states in practical quantum technologies.
Measurement scenarios containing events with relations of exclusivity represented by pentagons, heptagons, nonagons, etc., or their complements are the only ones in which quantum probabilities cannot be described classically. Interestingly, quantum theory predicts that the maximum values for any of these graphs cannot be achieved in Bell inequality scenarios. With the exception of the pentagon, this prediction remained experimentally unexplored. Here we test the quantum maxima for the heptagon and the complement of the heptagon using three- and five-dimensional quantum states, respectively. In both cases, we adopt two different encodings: linear transverse momentum and orbital angular momentum of single photons. Our results exclude maximally noncontextual hidden-variable theories and are in good agreement with the maxima predicted by quantum theory.
According to Bell's theorem, any model based on local variables cannot reproduce certain quantum correlations. A critical question is whether one could devise an alternative framework, based on nonlocal variables, to reproduce quantum correlations while adhering to fundamental principles. Leggett proposed a nonlocal model, termed crypto-nonlocality, rooted in considerations of the reality of photon polarization, but this property restricted it to being bi-dimensional. In this Letter, we extend the crypto-nonlocal model to higher dimensions and develop a framework for constructing experimentally testable Leggett-type inequalities for arbitrary dimensions. Our investigation into models that yield specific predictions exceeding those of quantum mechanics is intriguing from an information-theoretic perspective and is expected to deepen our understanding of quantum correlations.