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AIP Advances

Magnetization process of antiferromagnetic quantum spin chains with the biquadratic exchange interaction

Tôru Sakai

Published Jan 1, 2024• 0 citations
Publisher

Abstract

The magnetization processes of the S = 3/2 and S = 2 antiferromagnetic chains with the biquadratic interaction are investigated using the numerical diagonalization of the finite-size cluster. It is found that the system does not exhibit the spin nematic phase, which was predicted to occur for the S = 1 antiferromagnetic chain. Instead, the present analysis reveals that the quantum spin triatic and quatic liquid phases appear below the saturation magnetization for sufficiently large negative biquadratic interaction, for S = 3/2 and S = 2 chains, respectively. In addition it is also found that the magnetization jump up to the saturation magnetization appears for the small negative biquadratic interaction. The phase diagrams with respect to the negative biquadratic interaction and the magnetization are presented for the S = 3/2 and S = 2 antiferromagnetic chains.

DOI
10.1063/9.0000656

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The magnetization processes of the S = 3/2 and S = 2 antiferromagnetic chains with the biquadratic interaction are investigated using the numerical diagonalization of the finite-size cluster. It is found that the system does not exhibit the spin nematic phase, which was predicted to occur for the S = 1 antiferromagnetic chain. Instead, the present analysis reveals that the quantum spin triatic and quatic liquid phases appear below the saturation magnetization for sufficiently large negative biquadratic interaction, for S = 3/2 and S = 2 chains, respectively. In addition it is also found that the magnetization jump up to the saturation magnetization appears for the small negative biquadratic interaction. The phase diagrams with respect to the negative biquadratic interaction and the magnetization are presented for the S = 3/2 and S = 2 antiferromagnetic chains.
The magnetization process of the S = 1 antiferromagnetic chain with the biquadratic interaction is investigated using the numerical diagonalization. As a result, it is found that the quantum spin nematic liquid phase appears below the saturation magnetization for sufficiently large negative biquadratic interaction. The ground state phase diagram is also presented. This result is consistent with the previous density matrix renormalization group study. In addition the present study confirms that the two magnon excitation is gapless, while the single magnon one is gapped in the spin nematic liquid phase.
The magnetization process of the S = 1 antiferromagnetic chain with the biquadratic interaction is investigated using the numerical diagonalization. As a result, it is found that the quantum spin nematic liquid phase appears below the saturation magnetization for sufficiently large negative biquadratic interaction. The ground state phase diagram is also presented. This result is consistent with the previous density matrix renormalization group study. In addition the present study confirms that the two magnon excitation is gapless, while the single magnon one is gapped in the spin nematic liquid phase.
The magnetization process of the S = 1 antiferromagnetic chain with the single-ion anisotropy D and the biquadratic interaction is investigated using the numerical diagonalization.Both interactions stabilize the 2-magnon Tomonaga-Luttinger liquid (TLL) phase in the magnetization process. Based on several excitation gaps calculated by the numerical diagonalization, some phase diagrams of the magnetization process are presented. These phase diagrams reveal that the spin nematic dominant TLL phase appears at higher magnetizations for sufficiently large negative D.
Abstract The magnetization process of the S = 1 antiferromagnetic chain with the single-ion anisotropy D and the biquadratic interaction is investigated using the numerical diagonalization. Both interactions stabilize the 2-magnon Tomonaga-Luttinger liquid (TLL) phase in the magnetization process. Based on several excitation gaps calculated by the numerical diagonalization, some phase diagrams of the magnetization process are presented. These phase diagrams reveal that the spin nematic dominant TLL phase appears at higher magnetizations for sufficiently large negative D.
The S=2S=2S=2 quantum spin chain with the single-ion anisotropy DDD and the biquadratic exchange interaction JBQJ_{\rm BQ}JBQ​ is investigated using the numerical diagonalization of finite-size clusters and the level spectroscopy analysis. It is found that the intermediate-DDD phase corresponding to the symmetry protected topological (SPT) phase appears in a wide region of the ground state phase diagram. We also obtain the phase diagram at the half of the saturation magnetization which includes the SPT plateau phase.
We investigate the S=2S=2S=2 antiferromagnetic quantum spin chain with the exchange and single-ion anisotropies in a magnetic field, using the numerical exact diagonalization of finite-size clusters and the level spectroscopy analysis. It is found that a magnetization plateau possibly appears at half of the saturation magnetization for some suitable anisotropy parameters. The level spectroscopy analysis indicates that the 1/2 magnetization plateau is formed by two different mechanisms, depending on the anisotropy parameters. The phase diagram of the 1/2 plateau states and some typical magnetization curves are also presented. In addition, the biquadratic interaction is revealed to enhance the plateau induced by the Haldane mechanism.