Abstract Understanding and controlling engineered quantum systems is key to developing practical quantum technology. However, given the current technological limitations, such as fabrication imperfections and environmental noise, this is not always possible. To address these issues, a great deal of theoretical and numerical methods for quantum system identification and control have been developed. These methods range from traditional curve fittings, which are limited by the accuracy of the model that describes the system, to machine learning (ML) methods, which provide efficient control solutions but no control beyond the output of the model, nor insights into the underlying physical process. Here we experimentally demonstrate a ‘graybox’ approach to construct a physical model of a quantum system and use it to design optimal control. We report superior performance over model fitting, while generating unitaries and Hamiltonians, which are quantities not available from the structure of standard supervised ML models. Our approach combines physics principles with high-accuracy ML and is effective with any problem where the required controlled quantities cannot be directly measured in experiments. This method naturally extends to time-dependent and open quantum systems, with applications in quantum noise spectroscopy and cancellation.
Abstract Understanding and controlling engineered quantum systems is key to developing practical quantum technology. However, given the current technological limitations, such as fabrication imperfections and environmental noise, this is not always possible. To address these issues, a great deal of theoretical and numerical methods for quantum system identification and control have been developed. These methods range from traditional curve fittings, which are limited by the accuracy of the model that describes the system, to machine learning (ML) methods, which provide efficient control solutions but no control beyond the output of the model, nor insights into the underlying physical process. Here we experimentally demonstrate a ‘graybox’ approach to construct a physical model of a quantum system and use it to design optimal control. We report superior performance over model fitting, while generating unitaries and Hamiltonians, which are quantities not available from the structure of standard supervised ML models. Our approach combines physics principles with high-accuracy ML and is effective with any problem where the required controlled quantities cannot be directly measured in experiments. This method naturally extends to time-dependent and open quantum systems, with applications in quantum noise spectroscopy and cancellation.
Understanding and controlling engineered quantum systems is key to developing practical quantum technology. However, given the current technological limitations, such as fabrication imperfections and environmental noise, this is not always possible. To address these issues, a great deal of theoretical and numerical methods for quantum system identification and control have been developed. These methods range from traditional curve fittings, which are limited by the accuracy of the model that describes the system, to machine learning methods, which provide efficient control solutions but no control beyond the output of the model, nor insights into the underlying physical process. Here we experimentally demonstrate a "graybox" approach to construct a physical model of a quantum system and use it to design optimal control. We report superior performance over model fitting, while generating unitaries and Hamiltonians, which are quantities not available from the structure of standard supervised machine learning models. Our approach combines physics principles with high-accuracy machine learning and is effective with any problem where the required controlled quantities cannot be directly measured in experiments. This method naturally extends to time-dependent and open quantum systems, with applications in quantum noise spectroscopy and cancellation.
Quantum sensors offer significant advantages over classical devices in spatial resolution and sensitivity, enabling transformative applications across materials science, healthcare, and beyond. Their practical performance, however, is often constrained by unmodelled effects, including noise, imperfect state preparation, and non-ideal control fields. In this work, we report the first experimental implementation of a graybox modelling strategy for a solid-state open quantum system. The graybox framework integrates a physics-based system model with a data-driven description of experimental imperfections, achieving higher fidelity than purely analytical (whitebox) approaches while requiring fewer training resources than fully deep-learning blackbox models. We experimentally validate the method on the task of estimating a static magnetic field using a single-spin quantum sensor, performing Bayesian inference with a graybox model trained on prior experimental data. Using roughly 10,000 training datapoints, the graybox model yields several orders of magnitude improvement in mean squared error over the corresponding physics-only model, as well as significant improvement over a blackbox model with comparable size. These results are broadly applicable to a wide range of quantum sensing platforms, not limited to single-spin systems, and are particularly valuable for real-time adaptive protocols, where model inaccuracies can otherwise lead to suboptimal control and degraded performance.
The tasks of characterization and control of quantum systems are becoming more challenging with the advancement of quantum technology. Standard methods that were successful for simple quantum systems are becoming inadequate for more complex engineered systems. Modelling assumptions and approximations (such as Markovianity) are not justifiable anymore. As a result, the usual models fail to fit experimental measurements. In this thesis, we use state-of-the-art machine learning methods, assisted by tools from information theory as needed, to develop new frameworks that try to address these challenges. We focus on three directions. The first is developing an efficient online quantum state estimation algorithm with provable convergence properties. The second is developing a deep learning framework for characterizing and controlling closed quantum systems. The final direction is upgrading that framework to be suitable for characterization and control of open quantum systems. This thesis opens the door for a novel way of utilizing machine learning techniques for applications in quantum information specially and physics in general.
Controlling quantum systems under correlated non-Markovian noise, particularly when strongly coupled, poses significant challenges in the development of quantum technologies. Traditional quantum control strategies, heavily reliant on precise models, often fail under these conditions. Here, we address the problem by utilizing a data-driven graybox model, which integrates machine learning structures with physics-based elements. We demonstrate single-qubit control, implementing a universal gate set as well as a random gate set, achieving high fidelity under unknown, strongly-coupled non-Markovian non-Gaussian noise, significantly outperforming traditional methods. Our method is applicable to all open finite-dimensional quantum systems, regardless of the type of noise or the strength of the coupling.
While the Graybox characterization method allows for implicit noise models and is platform-agnostic, the method lacks uncertainty quantification. Characterization of quantum devices is a crucial process that enables researchers to gain insight from experimental settings. Graybox characterization combines known system dynamics with unknown transformations, where the latter is modeled using machine learning. Prediction uncertainty helps researchers make informed decisions. It allows valuable insights from the devices without overconfidence. We therefore develop a probabilistic Graybox characterization model using probabilistic machine learning, specifically Bayesian Neural Networks, and utilize binary measurement outcomes directly for inference. With stochastic noise in a quantum device, we analyze statistical properties of the measurement data. Our results show that the model's prediction performance solely depends on its ability to capture the expected value of the true expectation value. Our proposed probabilistic Graybox model outperforms the original model by up to 1.9 times in capturing the distribution of observed data. We expect that our results will serve as an additional tool for characterizing quantum devices with uncertainty estimation, as they provide a flexible choice that can be utilized even without extensive prior knowledge of the noise model of the devices.
Abstract This work addresses the problem of developing a machine-learning approach for the generation of a desired quantum process, i.e., a predefined trajectory in the set of quantum channels. To this end, a physical model of N-level quantum systems driven by coherent and incoherent controls is constructed, in which both Hamiltonian and dissipative dynamics are controlled. The main challenge in generating a target quantum process is the high complexity of finding optimal controls with conventional local-search optimization methods. To efficiently solve this problem, we develop a machine learning method that leverages a special representation of the dynamics. The proposed machine learning method achieves high efficiency and fast execution times: it delivers significantly higher accuracy (by an order of magnitude) and accelerates the generation of target quantum processes compared to standard local search methods for qubit, qutrit, and qudit (five-level) systems.