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International Electronic Conference on Applied Sciences (ASEC)

Absorption and Dispersion Properties of a Coupled Asymmetric Double Quantum Dot Molecule–Metal Nanoparticle Structure

Spyridon G. Kosionis, Emmanuel Paspalakis

Published Oct 26, 2023• 1 citation
Publisher

Abstract

The interaction of excitons with localized surface plasmons in hybrid nanostructures containing semiconductor quantum dots and metal nanoparticles, under specific conditions, may generate products with collective optical properties that have an abundance of potential applications in the area of nanotechnology. In the present study, we explore the behavior of the linear absorption and dispersion properties of the double-semiconductor quantum dot molecule in the presence of a spherical metal nanoparticle. We find that a transparency window arises in the absorption spectrum, the width of which decreases with the decrease in the electron tunnelling rate. In the low-electron-tunnelling regime, slow light is generated, an effect closely associated with tunneling-induced transparency. The enhancement of the tunneling rate induces a broadening in the transparency window, occurring due to the Autler–Townes splitting. The investigation of the impact of the distance between the quantum dot and the metal nanoparticle on the slowdown factor and the width of the transparency window shows that, by transposing the metal nanoparticle closer to the double-semiconductor quantum dot molecule, the transparency window widens.

DOI
10.3390/asec2023-15299

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The interaction of excitons with localized surface plasmons in hybrid nanostructures containing semiconductor quantum dots and metal nanoparticles, under specific conditions, may generate products with collective optical properties that have an abundance of potential applications in the area of nanotechnology. In the present study, we explore the behavior of the linear absorption and dispersion properties of the double-semiconductor quantum dot molecule in the presence of a spherical metal nanoparticle. We find that a transparency window arises in the absorption spectrum, the width of which decreases with the decrease in the electron tunnelling rate. In the low-electron-tunnelling regime, slow light is generated, an effect closely associated with tunneling-induced transparency. The enhancement of the tunneling rate induces a broadening in the transparency window, occurring due to the Autler–Townes splitting. The investigation of the impact of the distance between the quantum dot and the metal nanoparticle on the slowdown factor and the width of the transparency window shows that, by transposing the metal nanoparticle closer to the double-semiconductor quantum dot molecule, the transparency window widens.
We investigate the optical properties appearing in a nanostructure that is composed of an asymmetric double semiconductor quantum dot (SQD) molecule and a metal nanoparticle (MNP). The profile of the total linear absorption spectrum is proportional to the SQD contribution, while the MNP contribution is important. The profile of the doublet of resonances detected on the total linear absorption spectrum creates a transparency window. The doublet is asymmetric for small SQD-MNP distances and has a narrow peak and a wide peak. The width of the transparency window is increased, either with the enhancement of the rate at which the electron tunneling effect takes place within the double SQD molecule or with the decrease of the distance that separates the SQD molecule from the center of the MNP. The steep slope detected on the linear dispersion spectrum for frequencies laying within the transparency window owes its presence to the tunneling induced transparency and leads to slow light production. The corresponding value of the slow down factor is maximized for low values of the electron tunneling rate as well as for low center-to-center distances between the components of the hybrid nanostructure.
In the present work, we investigate the modified nonlinear pump-probe optical properties due to the excitonic–plasmonic interaction of a double semiconductor quantum dot (SQD) molecule coupled to a metal nanoparticle (MNP). More specifically, we study the absorption and the dispersion spectra of a weak electromagnetic field in a hybrid structure with two counterparts, a molecule of two coupled SQDs, and a spherical MNP driven by a field of high intensity. We solve the relevant density matrix equations, calculate the first-order optical susceptibility of the probe field in the strong pumping regime, and investigate the way in which the distance between the two counterparts modifies the optical response, for a variety of values of the physical constants of the system, including the pump-field detuning, the tunnelling rate, and the energy separation gap associated with the excited states of the coupled SQDs.
The group velocity of light is investigated in a hybrid nanostructure comprised of semiconductor quantum dot (SQD) and metal nanoparticle (MNP). In the presence of MNP, the hybrid absorption of the system can be eliminated and forms a broad transparency window even though related dipole transition is not forbidden. Owing to the presence of MNP, there is the formation of the steep dispersion at the transparency regime, thus, the controllable group velocity of light can be implemented. The group velocity of light is changed from subluminal to superluminal via adjusting the inter-particle distance between SQD and MNP.
This work studies the energy absorption rates in the case of plasmonic electromagnetically induced transparency (PEIT) from the double quantum dot (DQD)–metal nanoparticle (MNP) system. The orthogonalized plane wave between the wetting layer (WL) and QD transitions is considered. PEIT is not attained under a single applied field. It is obtained under a probe, pump, and two tunneling components. Two asymmetric PEIT windows can result from the transitions between the sixth energy states of the DQD structure. A huge Qtotal value (10−5 W) under 0.2 W/cm2 is obtained. Compared with other works, this result is higher by four orders, and the power applied is less by six orders than that used in earlier works. Our results exceed those obtained with double MNP-QD, QD-six MNP, and MNP-ten QDs. Such a vast result is ascribed to the manipulation flexibility in the DQD system, which is not found in all other structures. This possibility increases quantum correlation and the nonlinear optical properties of the DQD and the DQD–MNP system. The QD ( QQD) and MNP ( QMNP) absorption energy rates are also studied. Applying two tunneling components restores the system to peak at resonance due to the coupled work of the two dots as a DQD system. Strong plasmon–exciton coupling occurs when the probe power becomes considerable. Thus, the probe must not be so small.
We study optical effects in a hybrid system composed of a semiconductor quantum dot (SQD) and a spherical metal nanoparticle (MNP) that interacts with a weak probe and a strong pump electromagnetic field. We use modified nonlinear density matrix equations for the description of the optical properties of the system and calculate, numerically, the first-order susceptibilities of the SQD, the MNP, and the total hybrid nanostructure of the probe field in the presence of the pump field. We investigate the dependence of the probe absorption and dispersion spectra of the SQD, the MNP, and the total nanostructure on the interparticle distance and the detuning of the pump field, and stress the influence of the MNP contribution to the total optical response. The results we find are explained according to the theory of two distinct metastates, which constitute conjugations of the SQD excitonic and the MNP plasmonic excitations. We also show that the optical response strongly depends on the actual values of the SQD material parameters.
A slow light effect in a hybrid nanocrystal complex composed of a semiconductor quantum dot (SQD) and a metal nanoparticle (MNP) is investigated theoretically. It is shown that a hole induced by coherent population oscillation appears at the absorption spectrum of the probe when an exciton and plasmon interact. Then a slow light effect may become possible. The numerical results further indicate that the slow light effect is greatly modified by the distance between the SQD and the MNP due to the coupling of the exciton and plasmon. For experimental conditions, the group velocity indexes with Gauss distribution and Lorenz distribution of the distance between the SQD and the MNP are evaluated. It is found that for small dispersion, almost the same values of the group velocity index can be obtained in these different distributions.