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Solid-state quantum nodes based on color centers and rare-earth ions coupled with fiber Fabry–Pérot microcavities

Ruo-Ran Meng, Xiao Liu, Ming Jin, Zong‐Quan Zhou, Chuan‐Feng Li, Guang‐Can Guo

Published Jan 5, 2024• 16 citations
Publisher

Abstract

High-performance optical quantum memories serving as quantum nodes are crucial for the distribution of remote entanglement and the construction of large-scale quantum networks. Notably, quantum systems based on single emitters can achieve deterministic spin-photon entanglement, greatly simplifying the difficulty of constructing quantum network nodes. Among them, optically interfaced spins embedded in solid-state systems, as atomic-like emitters, are important candidate systems for implementing long-lived quantum memory due to their stable physical properties and robustness to decoherence in scalable and compact hardware. To enhance the light-matter-interaction strength, optical microcavities can be exploited as an important tool to generate high-quality spin-photon entanglement for scalable quantum networks. They can enhance the photon collection probability and photon generation rate of specific optical transitions and improve the coherence and spectral purity of emitted photons. For solid-state systems, open Fabry-Pérot cavities can couple single emitters that are not in proximity to the surface, avoiding significant spectral diffusion induced by the interfaces while maintaining the wide tunability, which enables addressing of multiple single emitters in the frequency and spatial domain within a single device. This review describes the characteristics of single emitters as quantum memories with a comparison to atomic ensembles, the cavity-enhancement effect for single emitters and the advantages of different cavities, especially fiber Fabry-Pérot microcavities. Finally, recent experimental progress on solid-state single emitters coupled with fiber Fabry-Pérot microcavities is reviewed, with a focus on color centers in diamond and silicon carbide, as well as rare-earth dopants.

DOI
10.1016/j.chip.2023.100081

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Coherent interfaces between optical photons and long-lived matter qubits form a key resource for a broad range of quantum technologies. Cavity quantum electrodynamics (cQED) offers a route to achieve such an interface by enhancing interactions between cavity-confined photons and individual emitters. Over the last two decades, a promising new class of emitters based on defect centers in diamond has emerged, combining long spin coherence times with atom-like optical transitions. More recently, advances in optical resonator technologies have made it feasible to realize cQED in diamond. This article reviews progress towards coupling color centers in diamond to optical resonators, focusing on approaches compatible with quantum networks. We consider the challenges for cQED with solid-state emitters and introduce the relevant properties of diamond defect centers before examining two qualitatively different resonator designs: micrometer-scale Fabry–Perot cavities and diamond nanophotonic cavities. For each approach, we examine the underlying theory and fabrication, discuss strengths and outstanding challenges, and highlight state-of-the-art experiments.
Coherent interfaces between optical photons and long-lived matter qubits form a key resource for a broad range of quantum technologies. Cavity quantum electrodynamics (cQED) offers a route to achieve such an interface by enhancing interactions between cavity-confined photons and individual emitters. Over the last two decades, a promising new class of emitters based on defect centers in diamond have emerged, combining long spin coherence times with atom-like optical transitions. More recently, advances in optical resonator technologies have made it feasible to realize cQED in diamond. This article reviews progress towards coupling color centers in diamond to optical resonators, focusing on approaches compatible with quantum networks. We consider the challenges for cQED with solid-state emitters and introduce the relevant properties of diamond defect centers before examining two qualitatively different resonator designs: micron-scale Fabry-Perot cavities and diamond nanophotonic cavities. For each approach, we examine the underlying theory and fabrication, discuss strengths and outstanding challenges, and highlight state-of-the-art experiments.
Chapter 1 reviews recent advances towards the realization of quantum networks based on atom-like solid-state quantum emitters coupled to nanophotonic devices. Specifically, focus is on experiments involving the negatively charged silicon-vacancy color center in diamond. These emitters combine homogeneous, coherent optical transitions and a long-lived electronic spin quantum memory. Optical and spin properties of this system at cryogenic temperatures and experiments where silicon-vacancy centers are coupled to nanophotonic cavities are discussed. Finally, the chapter discusses experiments demonstrating quantum nonlinearities at the single-photon level and two-emitter entanglement in a single nanophotonic device.
We review recent advances towards the realization of quantum networks based on atom-like solid-state quantum emitters coupled to nanophotonic devices. Specifically, we focus on experiments involving the negatively charged silicon-vacancy color center in diamond. These emitters combine homogeneous, coherent optical transitions and a long-lived electronic spin quantum memory. We discuss optical and spin properties of this system at cryogenic temperatures and describe experiments where silicon-vacancy centers are coupled to nanophotonic devices. Finally, we discuss experiments demonstrating quantum nonlinearities at the single-photon level and two-emitter entanglement in a single nanophotonic device.
Single photons enable the distribution of quantum information over large distances and thus play a major role in quantum technologies such as communication and computing. Solid-state emitters are practical and efficient sources of single photons that can be manufactured in large numbers. When combined with a spin, the resulting spin-photon interfaces can store quantum states for extended periods and serve as the basis for quantum networks and repeaters. Among the many host materials explored over the past few decades, silicon stands out for its advanced nanofabrication, the maturity of its integrated photonics and microelectronics, and its high isotopic purity, which leads to exceptionally long spin coherence. These properties position silicon single-photon emitters and spin-photon interfaces among the most promising hardware platforms for implementing quantum networks and distributed quantum information processors. This review summarizes the current state of the art and open challenges towards coherent single-photon sources and scalable spin-photon interfaces based on color centers and erbium dopants in nanophotonic silicon structures.
Quantum networks based on nitrogen-vacancy (N-VVV) color centers in diamond will enable technology such as communication secured by the laws of nature, and blind quantum computation in the cloud. However, scaling to large distances and many nodes is hindered by the small coherent photon emission and collection from N-VVV centers. By embedding a thin diamond membrane bearing coherent color centers into an open, tunable fiber-based optical microcavity, the authors demonstrate that the centers' emission can be enhanced in a fashion compatible with entanglement generation. This work is an important step toward employing N-VVV centers in large-scale quantum networks with long coherence.