For a Rydberg atom-based sensor to change its sensing frequency, the wavelength of the Rydberg state excitation laser must be altered. The wavelength shifts required can be on the order of 10 nm. A fast-tunable narrow-linewidth laser with broadband tuning capability is required. Here, we present a demonstration of a laser system that can rapidly switch a coupling laser as much as 8 nm in less than 50 μs. The laser system comprises a frequency-stabilized continuous wave laser and an electro-optic frequency comb. A filter enables selection of individual comb lines. A high-speed electro-optic modulator is used to tune the selected comb line to a specific frequency, i.e., an atomic transition. Through Rydberg atom-based sensing experiments, we demonstrate frequency hopping between two Rydberg states and a fast switching time of 400 μs, which we show can be reduced to ∼50 μs with a ping-pong scheme. If updating the RF frequency is not required during frequency hopping, a 200 ns switching time can be achieved. These results showcase the potential of the laser system for advanced Rydberg atom-based radio frequency sensing applications, like communications and radar.
For a Rydberg atom-based sensor to change its sensing frequency, the wavelength of the Rydberg state excitation laser must be altered. The wavelength shifts required can be on the order of 10 nm. A fast-tunable narrow-linewidth laser with broadband tuning capability is required. Here, we present a demonstration of a laser system that can rapidly switch a coupling laser as much as 8 nm in less than 50 μs. The laser system comprises a frequency-stabilized continuous wave laser and an electro-optic frequency comb. A filter enables selection of individual comb lines. A high-speed electro-optic modulator is used to tune the selected comb line to a specific frequency, i.e., an atomic transition. Through Rydberg atom-based sensing experiments, we demonstrate frequency hopping between two Rydberg states and a fast switching time of 400 μs, which we show can be reduced to ∼50 μs with a ping-pong scheme. If updating the RF frequency is not required during frequency hopping, a 200 ns switching time can be achieved. These results showcase the potential of the laser system for advanced Rydberg atom-based radio frequency sensing applications, like communications and radar.
While Rydberg atoms have shown tremendous potential to serve as accurate and sensitive detectors of microwaves and millimeter waves, their response is generally limited to a single, narrow frequency band around a chosen transition. As a result, their potential to serve as agile and wideband electromagnetic receivers has not been fully realized. Here we demonstrate the use of a mid-infrared, frequency agile optical frequency comb as the coupling laser for three-photon Rydberg atom electrometry. This approach allows for rapid switching between as many as seven individual Rydberg states, allowing for multichannel detection across a frequency range from 1 GHz to 40 GHz. The generality and flexibility of this method for wideband multiplexing is anticipated to have transformative effects in the field of Rydberg electrometry, paving the way for advanced information coding, arbitrary signal detection, and the simultaneous detection of ultra-broadband radiofrequency radiation. Rydberg atoms have the potential to serve as broadband receivers but require lasers with > 100 GHz scan ranges to observe multiple states. We bridge this major gap with an optical frequency comb for rapid preparation of over 7 Rydberg states.
Precision atomic and quantum experiments rely on ultra-stable narrow linewidth lasers constructed using table-top ultra-low expansion reference cavities. These experiments often require multiple lasers, operating at different wavelengths, to perform key steps used in state preparation and measurement required in quantum sensing and computing. This is traditionally achieved by disciplining a cavity-stabilized laser to a key atomic transition and then transferring the transition linewidth and stability to other lasers using the same reference cavity in combination with bulk-optic frequency shifting such as acousto-optic modulators. Transitioning such capabilities to a future potentially low-cost photonic-integrated platform will enable a wide range of portable, low power, scalable quantum experiments and applications. Yet, today’s bulk optic approaches pose challenges related to lack of cavity tunability, large free spectral range, and limited photonic integration potential. Here, we address these challenges with demonstration of an agile photonic-integrated 780 nm ultra-high-Q tunable silicon nitride reference cavity that performs multiple critical experimental steps including laser linewidth narrowing, high resolution rubidium spectroscopy, dual-stage stabilization to a rubidium transition, and stability transfer to other lasers. We achieve up to 20 dB of frequency noise reduction at 10 kHz offset, precision spectroscopy over a 250 MHz range, and dual-stage locking to rubidium with an Allan deviation of 8.5 × 10 −12 at 1 s and up to 40 dB frequency noise reduction at 100 Hz frequency offset. We further use the rubidium-disciplined cavity to provide atomic-referenced frequency stability to a second laser and demonstrate multi-wavelength Rydberg electrometry quantum sensing. These results pave the path for integrated, compact, and scalable solutions for quantum sensing, computing, and other atomic and trapped ion applications.
In this work, theoretical and experimental works on Rydberg-atom based radio-frequency (RF) sensors are presented. The results were obtained in close collaboration with the Quantum Valley Ideas Lab, whose goal is the miniaturization and prototyping of these sensors. The Rydberg-atom based RF sensors utilize lasers to coherently excite an atomic vapor in a vapor cell at room temperature to a highly excited Rydberg state, which is extremely sensitive to external environmental influences. In this work, Rydberg-atom based RF sensing is described as coherent multi-photon interference in the atom-light coupled system by introducing atom-light coherences. The presence of the RF wave influences the absorption of a probe laser propagating through the atomic medium. The atomic response of the Rydberg-atoms can be engineered by changing the atom-light coherences through laser power and frequency. Analytic expressions for the atomic response to the incident RF wave are derived in the weak probe limit and provide a deeper understanding of the underlying coherent multi-photon interference processes, which help to further tailor the Rydberg-atom for the purpose of the application. Good agreement with full numerical simulations of the Lindblad-master equation is found. An analysis of the various Doppler limits strongly motivates an excitation scheme where the effective wave vector mismatch on the Rydberg transition vanishes, as a promising candidate to achieve narrower spectral linewidths and, consequently, a higher sensitivity. The level structure of cesium presents a unique three-photon excitation scheme where residual Doppler shifts become comparable to the spectral linewidth of the coupling lasers. The experimental realization of this excitation scheme is demonstrated. A spectral linewidth of the Rydberg transition of 190 kHz is achieved. The measurements present the world record sensitivity, 45 nV/cm/Hz^1/2, for all-optical RF sensing with room temperature operation. These results make the three-photon excitation scheme a prime candidate for the next generation of Rydberg-atom based RF sensor prototypes. Finally, all-optical phase-sensitive RF detection is theoretically investigated in a closed-loop excitation scheme. An analytic expression is derived that intuitively describes the atomic response. Furthermore, it provides insights into the probe intensity dynamics that occur when the system is operated under finite detuning. These oscillatory dynamics allow for the extraction of the in- (I) and out- (Q) of-phase response to the RF wave, thereby enabling the simultaneous detection of the RF E-field amplitude and phase. A blueprint for the experimental realization is presented, and angle-of-arrival tolerances for the RF wave are estimated. A quadrature amplitude modulation (QAM) sequence was modelled and the simultaneous extraction of the phase and amplitude of the RF wave of interest was successfully demonstrated.
We demonstrate a straightforward frequency-locking technique that employs external modulation saturation absorption spectroscopy to achieve a high-performance 780 nm laser system. By externally modulating the laser frequency through a fiber electro-optic modulator, this scheme can stabilize multiple transitions of the 87Rb D2 line with excellent performance. Experimental results establish fractional frequency instability of 2.21 × 10-13 at 1 s with a linewidth of 1.46 kHz for the cycling transition 5S1/2(Fg = 2) → 5P3/2(Fe = 3). Notably, we have locked the system to the repumping transition 5S1/2(Fg = 1) → 5P3/2(Fe = 2), achieving a record-low instability of 1.98 × 10-12 at 1 s averaging time. This simplified laser system, featuring exceptional short-term frequency stability and multi-frequency locking capability, serves as a critical subsystem for the compact cold-atom optical clock, enabling advanced precision metrology applications. Furthermore, its metrological performance enables immediate applications in other quantum sensors, such as Rydberg electrometry, atomic magnetometry, and matter-wave interferometry.
We present a standalone frequency-offset locking system for controlling narrow-linewidth lasers using off-the-shelf electronic components. We lock two frequency-doubled 1560 nm lasers to a stable primary laser operating at 780 nm via their optical beat note. This radio-frequency beat note is fed through a broadband variable divider, a frequency-to-voltage converter, and a proportional-integrator controller to lock each follower laser to a tunable offset frequency relative to the primary. This architecture provides a large capture range (>1 GHz), fast response times (<1 ms), and high linearity. We achieve a frequency resolution of 1.9 kHz and a short-term fractional frequency instability 10−11/τ(s) at 780 nm without the need for a dedicated, precise clock reference. We perform high-resolution spectroscopy of cold 87Rb atoms to demonstrate the tunability and precision of our locking system. We designed the system to be modular and extensible, making it applicable to a wide variety of atomic physics experiments, including laser cooling, spectroscopy, and quantum sensing with atoms, ions, and molecules.
A laser with a switchable wavelength between 770 nm and 767 nm, corresponding to the potassium D1 and D2 lines, is a promising tool for manipulating potassium atoms. Here, we develop a potassium Faraday laser using a potassium atom-based Faraday anomalous dispersion optical filter (FADOF) as its frequency selection element. By dynamically adjusting the central frequency of the peak transmission across the entire transmitted spectrum of the potassium FADOF, the laser can operate either in single mode at either 770 nm or 767 nm, or emit both simultaneously. In single-mode operation, the laser wavelength remains aligned with the atomic transitions, exhibiting a narrow linewidth of 14.96 kHz at 770 nm and 13.07 kHz at 767 nm. In dual-mode operation, both modes are sustained continuously, with frequency drifts of less than 0.3 GHz for 200 minutes. Furthermore, we perform modulation transfer spectroscopy (MTS) and stabilize the laser to the 39 K 4S 1/2 F = (1, 2) → 4P 1/2 F ′ = 2 and 4S 1/2 F = (1, 2) → 4P 3/2 F ′ transitions. The corresponding frequency stability, measured by the optical heterodyne beat note between two identical systems, is 1.57 × 10 −12 and 8.77 × 10 −13 at 1 s, respectively. This architecture introduces a novel approach to the generation of wide-range wavelength switching within a single laser. In addition, with its narrow linewidth and impressive frequency stability, it serves as a reliable source for ultracold atom physics and quantum precision measurement.