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Physical Review A

Short-range physics of the three-body recombination for ultracold helium atoms

Binbin Wang, Yong‐Chang Han

Published Dec 6, 2023• 1 citation
Publisher

Abstract

Generally, the three-body recombination (TBR) of the ultracold helium atoms in the zero-collision-energy limit could be described by the original zero-range (Efimov) universal function [E. Braaten, D. Kang, and L. Platter, Phys. Rev. A 75, 052714 (2007)] using the scattering length $a$ of the He-He interaction and a three-body parameter ${a}_{*}$ as input, where ${a}_{*}$ is associated with the positive scattering length at which an interference minimum in the TBR rate occurs at the threshold. This universal property has been reinvestigated by considering various post-Born-Oppenheimer (post-BO) effects on the relevant scattering process. It is found that a linear correction to $1/{a}_{*}$ versus $1/a$ should be introduced to give a better description of these considered TBR cases because of the finite-range effects. Particularly, such a correction may be ascribed not only to the general scattering properties associated with the Efimov channel at the short hyperradial distance, but also to the tunneling probability in the lowest incident channel. In addition, a successful fit of the modified universal function that includes correctly the finite-range effects [E. Garrido, M. Gattobigio, and A. Kievsky, Phys. Rev. A 88, 032701 (2013)] or the zero-range universal function with a linearly variational $1/{a}_{*}$ versus $1/a$ to numerically accurate data also indicates a clear manifestation of the van der Waals universality. Finally, the post-BO effects on the TBR process for the partial wave with the total angular momentum $J>0$ are also discussed.

DOI
10.1103/physreva.108.062805

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Generally, the three-body recombination (TBR) of the ultracold helium atoms in the zero-collision-energy limit could be described by the original zero-range (Efimov) universal function [E. Braaten, D. Kang, and L. Platter, Phys. Rev. A 75, 052714 (2007)] using the scattering length aaa of the He-He interaction and a three-body parameter a∗{a}_{*}a∗​ as input, where a∗{a}_{*}a∗​ is associated with the positive scattering length at which an interference minimum in the TBR rate occurs at the threshold. This universal property has been reinvestigated by considering various post-Born-Oppenheimer (post-BO) effects on the relevant scattering process. It is found that a linear correction to 1/a∗1/{a}_{*}1/a∗​ versus 1/a1/a1/a should be introduced to give a better description of these considered TBR cases because of the finite-range effects. Particularly, such a correction may be ascribed not only to the general scattering properties associated with the Efimov channel at the short hyperradial distance, but also to the tunneling probability in the lowest incident channel. In addition, a successful fit of the modified universal function that includes correctly the finite-range effects [E. Garrido, M. Gattobigio, and A. Kievsky, Phys. Rev. A 88, 032701 (2013)] or the zero-range universal function with a linearly variational 1/a∗1/{a}_{*}1/a∗​ versus 1/a1/a1/a to numerically accurate data also indicates a clear manifestation of the van der Waals universality. Finally, the post-BO effects on the TBR process for the partial wave with the total angular momentum J>0J>0J>0 are also discussed.
The scattering length scaling rules for three-body recombination (TBR) of the 4He4He6Li- system in the zero-energy limit (E → 0) are investigated by considering various post-Born-Oppenheimer (post-BO) contributions to the standard BO potential of He-He interaction. It is found that these post-BO effects on the TBR rates that lead to different dimer products could be well fitted by the scattering length scalings Cab with a being the scattering length of the He-He interaction, and b and C the constants. It is interesting to find that the powers b about both the weakly and deeply bound dimer products are quite different from the well-known powers given by the scattering length scaling laws in the fields of ultracold neutral atomic gases. Such difference and the distinct powers associated with various dimer products are qualitatively accounted for by the properties of the major effective potentials and relatively long-range nonadiabatic couplings. Particularly, from these properties, the scaling powers are expected to be dependent on systems, but the power scattering length scaling behaviors to be universal, which has also been checked to apply to a wide range of a by tuning the He-He interaction.
For a system of three identical bosons interacting via short-range forces, when two of the atoms are about to form a two-body sss-wave dimer, the Efimov effect takes place leading to the formation of an infinite number of three-body (Efimov) states. The lowest Efimov state crosses the three-body break-up threshold when the sss-wave two-body scattering length is $a\ensuremath{\approx}\ensuremath{-}9.73{r}_{\mathrm{vdW}}$, rvdW{r}_{\mathrm{vdW}}rvdW​ being the van der Waals length. This article focuses on a generalized version of this Efimov scenario, where two of the atoms are about to form a two-body ddd-wave dimer, resulting in strong ddd-wave interactions. In his paper [Phys. Rev. A 62, 050702(R) (2000)], Bo Gao predicted that for broad resonances the ddd-wave dimer is always formed when $a\ensuremath{\approx}0.956{r}_{\mathrm{vdW}}$. Here we find that a single universal three-body state associated with the ddd-wave dimer is also formed near the three-body breakup threshold at $a\ensuremath{\approx}1.09{r}_{\mathrm{vdW}}$, or alternatively a2=0.902rvdW{a}_{2}=0.902{r}_{\mathrm{vdW}}a2​=0.902rvdW​, where a2{a}_{2}a2​ is the two-body ddd-wave scattering length. The signature of such a universal three-body state is signaled experimentally by an enhancement of the three-body recombination rate. The three-body effective potential curves that are crucial for understanding the recombination dynamics are also calculated and analyzed. An improved method to calculate the couplings, effective potential curves, and recombination rate coefficients is presented.
The increase of the number of the two-body recombination channels strongly challenges the numerical calculation of the accurate rates for the three-body recombination (TBR) process and its reverse process, collision-induced dissociation (CID), at ultracold temperatures. By taking the 4He–4He–20Ne collision system as an example, we have obtained the rates for its TBR and CID processes involving all four recombination channels, including the two-body states 4He2 (l = 0) and 4He20Ne (l = 0, 1, 2) with l the rotational quantum number. By using the adiabatic hyperspherical method, we have considered not only total angular momentum J = 0 but also J > 0 in the ultracold collision energies (E = 0.01 − 100 mK × kB). It is found that 4He2 (l = 0) is the major product after the TBR process in the ultracold limit (E ≤ 0.1 mK × kB). The TBR rate into 4He2 (l = 0) is nearly one order of magnitude larger than the sum of the other three products, 4He20Ne (l = 0, 1, 2). Moreover, the CID rates for the three 4He20Ne (l = 0, 1, 2) + 4He initial states are close to each other and are smaller than that for the 4He2 (l = 0) + 20Ne initial state. Additionally, we have, for the first time, performed the channel-resolved scattering calculation that can explain the above-mentioned findings quantitatively.
We calculated, using seven realistic $^{4}\mathrm{He}\text{\ensuremath{-}}^{4}\mathrm{He}$ potentials in the literature, the Efimov spectra of the 4He^{4}\mathrm{He}4He trimer and tetramer and analyzed the universality of the systems. The three-(four-)body Schr\"odinger equations were solved fully nonadiabatically with the high-precision calculation method employed in our previous work on the 4He^{4}\mathrm{He}4He trimer and tetramer [Phys. Rev. A 85, 022502 (2012); Phys. Rev. A 85, 062505 (2012)]. We found the following universality in the four-boson system: (i) The critical scattering lengths at which the tetramer ground and excited states couple to the four-body threshold are independent of the choice of the two-body realistic potentials in spite of the difference in the short-range details and do not contradict the corresponding values observed in the experiments in ultracold alkali-metal atoms when scaled with the van der Waals length rvdW{r}_{\mathrm{vdW}}rvdW​, and (ii) the four-body hyperradial potential has a repulsive barrier at the four-body hyperradius ${R}_{4}\ensuremath{\approx}3\phantom{\rule{0.16em}{0ex}}{r}_{\mathrm{vdW}}$, which prevents the four particles from getting close together to explore nonuniversal features of the interactions at short distances. This result is an extension of the universality in Efimov trimers that the appearance of the repulsive barrier at the three-body hyperradius ${R}_{3}\ensuremath{\approx}2\phantom{\rule{0.16em}{0ex}}{r}_{\mathrm{vdW}}$ makes the critical scattering lengths independent of the short-range details of the interactions as reported in the literature and also in the present work for the 4He^{4}\mathrm{He}4He trimer with the realistic potentials.
Few-body effects play an important role for the understanding of ultracold quantum gases. We make use of an effective field theory approach to investigate various aspects of universal few-body physics close to a Feshbach resonance. That is the regime where the scattering length is large compared to all other length scales of the system and thus determines the observables. It is also the regime where the Efimov effect whose main characteristic is the occurrence of a sequence of three-body bound states becomes important. At unitarity, i.e., for diverging scattering length, the ratio of binding energies of neighboring states approaches a constant. The existence of those trimers can be captured by a single three-body parameter and influences observables such as recombination rates. Starting from adequate Lagrangians, we derive atom-dimer scattering amplitudes that contain all information of interest about the three-particle systems. With this method, we first investigate the scattering of atoms and dimers at finite temperature in the presence of the Efimov effect. We calculate the dimer relaxation rate and obtain good agreement with available experimental data. Furthermore, heteronuclear mixtures exhibiting large interspecies scattering length are studied in detail. If bosons are the majority species, the Efimov effect occurs in an S-wave channel and we are able to compute three-body recombination and dimer relaxation rates. The results are compared to the outcome of two existing experiments. For mainly fermionic systems, the Efimov effect is only present in an overall P-wave and three-body recombination at threshold vanishes. However, in mixtures of atoms and dimers, scattering cross sections and dimer relaxation show the typical Efimov behavior of log-periodicity. We also consider two-dimensional Bose gases, where the Efimov effect does not occur. For those systems, we derive an equation including the first non-universal corrections and deduce three-body observables such as binding energies and atom-dimer scattering parameters.