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Optics Express

Plasmon-modulated bistable second-harmonic generation in a nonlinear microcavity coupled to a metallic nanoparticle

Shuang Zhou, Ying Li, Zhenzhen Song, Xiyun Li, Yong Pu

Published Nov 10, 2023• 2 citations
Publisher

Abstract

Multiple nonlinear effects with second-harmonic (SH) generation and optical bistability (OB) are highly desired but rather rare due to insufficient intrinsic nonlinearity in most nonlinear media. Here, a nonlinear microcavity coupled to a metallic nanoparticle (MNP) is suggested to realize the bistable SH generation. When two counterpropagating driving fields are injected into the cavity, a traditional SH pathway is constructed via the two-photon process of fundamental-harmonic (FH) photons. In addition, we report the coexistence between the SH and OB effects under the condition that the strong excitation and the detuning management for the driving fields boost system nonlinear responses. In the presence of a control field toward the MNP, our calculation finds that the traditional and plasmon-induced SH pathways in the present system allow enhancing the SH conversion efficiency and reducing the OB thresholds simultaneously. With the control field intensity increasing, a linear growth rate for the SH efficiency maximum is achieved. Furthermore, the relative phase between the driving and control fields has profound effects on modulating the bistable SH efficiency, the bistable interval and the thresholds.

DOI
10.1364/oe.505752

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Multiple nonlinear effects with second-harmonic (SH) generation and optical bistability (OB) are highly desired but rather rare due to insufficient intrinsic nonlinearity in most nonlinear media. Here, a nonlinear microcavity coupled to a metallic nanoparticle (MNP) is suggested to realize the bistable SH generation. When two counterpropagating driving fields are injected into the cavity, a traditional SH pathway is constructed via the two-photon process of fundamental-harmonic (FH) photons. In addition, we report the coexistence between the SH and OB effects under the condition that the strong excitation and the detuning management for the driving fields boost system nonlinear responses. In the presence of a control field toward the MNP, our calculation finds that the traditional and plasmon-induced SH pathways in the present system allow enhancing the SH conversion efficiency and reducing the OB thresholds simultaneously. With the control field intensity increasing, a linear growth rate for the SH efficiency maximum is achieved. Furthermore, the relative phase between the driving and control fields has profound effects on modulating the bistable SH efficiency, the bistable interval and the thresholds.
We show that, nonlinear optical processes in a plasmonic metal nanoparticle (MNP) dimer can be controlled by the presence of a molecule or a quantum dot. (i) Frequency conversion can be suppressed if the dimer is coupled to a quantum object which is resonant to the generated frequency. This occurs simply because, EIT does not allow an excitation at the converted frequency frequency. (ii) On the contrary, a similar effect can be used to enhance the frequency conversion. Nonlinear processes can be brought to resonance without tuning the dimer modes. Path interference effect cancels the nonresonant frequency terms. Here, we consider the second harmonic generation (SHG) as an example to demonstrate the control mechanism. However, the method can be easily generalized to other nonlinear processes.
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Abstract In this paper, we study the tunneling induced optical bistability (OB) in a quantum dot (QD)-metallic nanoparticle (MNP) hybrid system via surface plasmon effects. We realized that in the presence of the tunneling effect, OB arises when the probe light is parallel to the major axis of the hybrid system. We realized the threshold of OB can be controlled by controlling the distance parameter between the QD and MNP. For appropriate distance between the QD and MNP, we find that optical multistability (OM) appears in the system. We find that the threshold of OM can be adjusted when we consider the radius effect of the MNP, respectively.
Energy-time entangled photon pairs (EPPs), which are at the heart of numerous quantum light applications, are commonly generated in nonlinear crystals. Some highly sensitive quantum applications require the use of ultra-broadband entangled photons that cannot be generated in nonlinear crystals due to phase-matching requirements. Here, we investigate the possibility of using metallic nanoparticles (MNPs) as a means for generating entangled photons through spontaneous parametric down-conversion (SPDC). MNPs are known for their strong light-matter coupling at their localized surface plasmon resonance, and since the propagation length through them is negligible relative to optical wavelengths, we consider them as excellent candidates to serve as non-phase matched sources of ultra-broadband entangled photons. To that end, we report experimental results of classical-light second-harmonic generation in silver nanotriangles and nanocubes embedded in polyvinyl alcohol. Based on the results of our experiments, performed using the reference-free hyper-Rayleigh scattering method [A. Ashkenazy et al., J. Phys. B 145401, 2019], we present an estimation of the characteristics of SPDC in MNPs. We show that, despite of the metals' centrosymmetric structure, MNPs exhibit second order nonlinearity that is mainly of an electric dipole nature, and so they are suitable for SPDC. Moreover, we show that localized surface-plasmon resonance can play a significant role in enhancing the generated EPPs flux. Finally, we compare the SPDC capabilities of MNPs to that of commonly used nonlinear crystals and show that the expected EPPs flux from MNPs is weaker but the EPPs have very large bandwidth, which could be helpful for advanced quantum sensing, spectroscopy and communication applications.