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The Wave-Optical Description Of Potential Scattering

Peter Fröbrich, R. Lipperheide

Published Jul 4, 1996• 0 citations
Publisher

Abstract

Abstract In the preceding chapter we have discussed the semiclassical approximation to quantum scattering theory, where the dynamics is described in terms of classical trajectories. By analytic continuation of these trajectories into the complex plane the treatment has even been extended to the scattering by complex, i.e. absorptive, potentials.

DOI
10.1093/oso/9780198537830.003.0003

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Abstract In the preceding chapter we have discussed the semiclassical approximation to quantum scattering theory, where the dynamics is described in terms of classical trajectories. By analytic continuation of these trajectories into the complex plane the treatment has even been extended to the scattering by complex, i.e. absorptive, potentials.
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The scattering properties of any complex scattering potential, , can be obtained from the dynamics of a particular non-unitary two-level quantum system . The application of the adiabatic approximation to yields a semiclassical treatment of the scattering problem. We examine the adiabatic series expansion for the evolution operator of and use it to obtain corrections of arbitrary order to the semiclassical formula for the transfer matrix of v. This results in a high-energy approximation scheme that unlike the semiclassical approximation can be applied for potentials with large derivatives.
We have directed much attention towards developing quantum trajectory methods which can accurately predict the transmission probabilities for a variety of quantum mechanical barrier scattering processes. One promising method involves solving the complex quantum Hamilton-Jacobi equation with the Derivative Propagation Method (DPM). We present this method, termed complex valued DPM (CVDPM(n)). CVDPM(n) has been successfully employed in the Lagrangian frame to accurately compute transmission probabilities on 'thick' one dimensional Eckart and Gaussian potential surfaces. CVDPM(n) is able to reproduce accurate results with a much lower order of approximation than is required by real valued quantum trajectory methods, from initial wave packet energies ranging from the tunneling case (E[subscript o]=0) to high energy cases (twice the barrier height). We successfully extended CVDPM(n) to two-dimensional problems (one translational degree of freedom representing an Eckart or Gaussian barrier coupled to a vibrational degree of freedom) in the Lagrangian framework with great success. CVDPM helps to explain why barrier scattering from "thick" barriers is a much more well posed problem than barrier scattering from "thin" barriers. Though results in these two cases are in very good agreement with grid methods, the search for an appropriate set of initial conditions (termed an 'isochrone) from which to launch the trajectories leads to a time-consuming search problem that is reminiscent of the rootsearching problem from semi-classical dynamics. In order to circumvent the isochrone problem, we present CVDPM(n) equations of motion which are derived and implemented in the arbitrary Lagrangian-Eulerian frame for a metastable potential as well as the Eckart and Gaussian surfaces. In this way, the isochrone problem can be circumvented but at the cost of introducing other computational difficulties. In order to understand why CVDPM may give better transmission probabilities than real valued counterparts, much attention we have been studying and applying numerical analytic continuation techniques to visualize complex-extended wave packets as well as the complex-extended quantum potential. Numerical analytic continuation techniques have also been used to analytically continue a discrete real-valued potential into the complex plane for CVDPM with very promising results.
In Chapter 3, we move to a semiclassical treatment (quantum theory) of light absorption and scattering, specifically from atoms. We start with a description of how lidar measures Doppler shift, and the fundamental difference between the measurement when the laser is in resonance with an atomic transition (resonant) and when it is not (nonresonant). We follow with a treatment of quantum polarizability and the resulting absorption cross section, leading to the differential resonance scattering cross section and its contrast with the classical result. After quantum polarizability, we demonstrate the radiation pattern of coherently excited atoms. This takes us to an interpretation of the Hanle Effect. Following these descriptions of the phenomena that impact resonance lidar, we extend our understanding by closing the chapter with an overview of the rudimentary physics of sodium laser guide stars.