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Annual Meeting Optical Society of America

Cross correlations between fluorescent and transmitted photons in single-atom cavity-enhanced absorption

Perry R. Rice, Xiaoyi Wang, H. J. Carmichael

Published Jan 1, 1988• 1 citation
Publisher

Abstract

We study a single two-level atom interacting on resonance with a weakly driven optical cavity mode. In earlier work on this system we calculated the degree of second-order coherence, the optical spectrum, and the spectrum of squeezing for both the transmitted light and fluorescence out the sides of the cavity.1,2 We present results for the cross-correlation functions that determine joint probabilities for a photodetection in transmission (fluorescence) followed by a photodetection in fluorescence (transmission). We compute these correlation functions numerically for arbitrary values of the three rates that govern the system dynamics: the atomic decay rate γ to modes other than the cavity mode, the photon escape rate from the cavity 2K, and the atom-field coupling constant g. Analytical results provide insight for the following limits of the parameters: (1) the bad-cavity limit, κ/γ→∞,κ/g→∞,g2/κγ constant; (2) the atomic-loss limit, κ/γ→0,κ/g→0,γ/g constant; (3) the cavity-loss limit, γ/κ→0,γ/g→0,g/κ constant; and (4) the good-cavity limit, k/γ→0,k/g→0,g2/κγ constant. In the bad-cavity limit the cross-correlation functions are symmetric with respect to the order of detection in transmission and fluorescence; in general they are not symmetric.

DOI
10.1364/oam.1988.ms9

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Annual Meeting Optical Society of America•Jan 1, 1989•0 citations
We study a single two-level atom interacting on resonance with a weakly driven optical cavity mode. In earlier work on this system we calculated the degree of second-order coherence, the optical spectrum, and the spectrum of squeezing for both the transmitted light and fluorescence out the sides of the cavity.1,2 We present results for the cross-correlation functions that determine joint probabilities for a photodetection in transmission (fluorescence) followed by a photodetection in fluorescence (transmission). We compute these correlation functions numerically for arbitrary values of the three rates that govern the system dynamics: the atomic decay rate γ to modes other than the cavity mode, the photon escape rate from the cavity 2K, and the atom-field coupling constant g. Analytical results provide insight for the following limits of the parameters: (1) the bad-cavity limit, κ/γ→∞,κ/g→∞,g2/κγ constant; (2) the atomic-loss limit, κ/γ→0,κ/g→0,γ/g constant; (3) the cavity-loss limit, γ/κ→0,γ/g→0,g/κ constant; and (4) the good-cavity limit, k/γ→0,k/g→0,g2/κγ constant. In the bad-cavity limit the cross-correlation functions are symmetric with respect to the order of detection in transmission and fluorescence; in general they are not symmetric.
We consider an optical cavity containing a single two-level atom driven on resonance by an external laser source.1 We focus on the limit of weak excitation where the dynamic response of this system is governed by just three parameters: the atom-field coupling constant g, spontaneous emission rate γ for the atom, and cavity decay rate κ. The statistics of the transmitted light are analyzed as a function of g, γ, and κ, in terms of the second-order correlation function g(2)(τ), and the quadrature variances measured in a homodyne detection scheme. Squeezing and photon antibunching exist over a wide range of parameters. For γ ~ κ, the system can exhibit an oscillatory response, even when the mean intracavity photon number is much less than unity.2 The oscillations can be understood in terms of the coupling between the free atom-field eigenstates |0,−>, |0,+>, and |1,−>. The oscillation frequency is determined by the energy level splitting produced between the degenerate one-quantum states |0,+> and |1,−> by the atom-field interaction. The second-order correlation function can exhibit a novel nonclassical effect, where, for g(2)(0) ≠ 0, at some finite delay τ0, the correlation function dips exactly to zero—g(2)(τ0) = 0.
The photon statistics of the transmitted light from a driven cavity containing a single resonant two-level atom are studied in the bad-cavity limit. For weak driving fields, the second-order intensity correlation function shows novel nonclassical behavior due to the interference of the driving field and forward reradiation from the atom. This behavior is related to squeezing in the cavity transmission. A physical interpretation is given in terms of the reduced quantum state of the coupled atom-field system following photodetection.>
We consider a single two-level atom in an optical cavity, in which the system is driven by a coherent driving field. In the bad-cavity limit, when the cavity loss rate is taken to be large compared to the atomic decay rate and atom-field coupling, the cavity field can be adiabatically eliminated from the equations of motion for the atomic operators. The main effect of the cavity in this limit is the enhancement of spontaneous emission into the cavity mode. For this model, the second-order intensity correlation function g(2)() has been shown to exhibit photon antibunching, sub-Poissonian photon number distributions, and other nonclassical effects.1 In this paper, analytic results are presented for g(2)() for both the transmitted and fluorescent light fields when broadband squeezed light is injected into the cavity. Effects of the squeezing on nonclassical behavior is examined.
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We recently reported that the transmitted light from a driven optical cavity containing a single-atom absorber shows strong nonclassical features.1 Also, Savage and Carmichael2 have shown that this single-atom system can be operated in a regime in which the transmitted light has a bimodal photon-counting distribution; as the saturation photon number is increased this bimodality develops into a single-atom version of absorptive optical bistability. We present results for the degree of second-order coherence and the spectrum of the transmitted light in the operating regime at the onset of bimodality. In this regime we can study the onset of low frequency behavior associated with transitions between the local states defined by the peaks of the bimodal distribution. Our results are calculated numerically, using a supercomputer to solve matrix element equations derived in the Fock-state basis. Our numerical approach also allows us to extend our analytical study of nonclassical effects in single-atom cavity-enhanced absorption. Our analytical results are restricted either to the bad-cavity limit1 or to weak driving fields outside this limit. We can now study how the nonclassical effects identified in these analytical calculations are changed by using finite driving fields outside the bad-cavity limit.
The standard theory of resonance fluorescence is a weak-coupling theory.1 If n ¯ is the mean photon number for the driving field, g is the atom field coupling constant, and γ is the Einstein A coefficient, formally the standard theory of resonance fluorescence assumes the limit n ¯ → ∞ , g/ γ → 0, with the ratio of Rabi frequency to atomic linewidth 2 n ¯ n g / γ finite. The limit g/γ → 0 allows the variation of the Rabi frequency 2 n g across the photon number distribution of the driving field to be neglected. By placing the atom inside an optical cavity the ratio g/γ can be changed. In this paper we calculate spectra for intracavity resonance fluorescence in the strong-coupling limit g/γ ≫ 1, g/κ ≫ 1, where κ is the cavity linewidth. We consider a single two-level atom interacting on resonance with a single cavity mode driven by a resonant coherent field. The cavity subtends a small solid angle at the atom, so that the spontaneous emission into free-space modes is not negligible. We calculate the spectrum of the light transmitted by the cavity (the transmitted spectrum) and the spectrum of the light radiated by the atom into free space (the fluorescent spectrum). The transmitted and fluorescent spectra show fundamental differences from the (weak-coupling) spectrum of free-space resonance fluorescence.