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Chinese Physics B

Optimal and robust control of population transfer in asymmetric quantum-dot molecules

Yu 裕 Guo 郭, Songshan Ma, Chuan‐Cun Shu

Published Oct 24, 2023• 4 citations
Publisher

Abstract

We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot molecules. We derive a long-duration control scheme that allows for highly efficient population transfer by accurately controlling the amplitude of a narrow-bandwidth pulse. To overcome fluctuations in control field parameters, we employ a frequency-domain quantum optimal control theory method to optimize the spectral phase of a single pulse with broad bandwidth while preserving the spectral amplitude. It is shown that this spectral-phase-only optimization approach can successfully identify robust and optimal control fields, leading to efficient population transfer to the target state while concurrently suppressing population transfer to undesired states. The method demonstrates resilience to fluctuations in control field parameters, making it a promising approach for reliable and efficient population transfer in practical applications.

DOI
10.1088/1674-1056/ad0627

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We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot molecules. We derive a long-duration control scheme that allows for highly efficient population transfer by accurately controlling the amplitude of a narrow-bandwidth pulse. To overcome fluctuations in control field parameters, we employ a frequency-domain quantum optimal control theory method to optimize the spectral phase of a single pulse with broad bandwidth while preserving the spectral amplitude. It is shown that this spectral-phase-only optimization approach can successfully identify robust and optimal control fields, leading to efficient population transfer to the target state while concurrently suppressing population transfer to undesired states. The method demonstrates resilience to fluctuations in control field parameters, making it a promising approach for reliable and efficient population transfer in practical applications.
Achieving fast and efficient quantum state transfer is a fundamental task in physics, chemistry and quantum information science. However, the successful implementation of the perfect quantum state transfer also requires robustness under practically inevitable perturbative defects. Here, we demonstrate how an optimal and robust quantum state transfer can be achieved by shaping the spectral phase of an ultrafast laser pulse in the framework of frequency domain quantum optimal control theory. Our numerical simulations of the single dibenzoterrylene molecule as well as in atomic rubidium show that optimal and robust quantum state transfer via spectral phase modulated laser pulses can be achieved by incorporating a filtering function of the frequency into the optimization algorithm, which in turn has potential applications for ultrafast robust control of photochemical reactions.
Coherent single-electron control in a realistic semiconductor double quantum dot is studied theoretically. Using optimal-control theory, we show that the energy spectrum of a two-dimensional double quantum dot has a fully controllable transition line. We find that optimized picosecond laser pulses generate population transfer at significantly higher fidelities (>0.99)(>0.99)(>0.99) than conventional sinusoidal pulses. Finally, we design a robust and fast charge switch driven by optimal pulses that are within reach of terahertz laser technology.
We present a way to realize selective, robust, and efficient population transfer in a ladder-type four-level system with an equally populated doublet in the initial state. By merging stimulated Raman adiabatic passage and chirped adiabatic passage techniques, we show that selective and complete population transfer from either of the initial doublet levels to the final state can be achieved with chirped pump and Stokes pulse pairs when the spectral resolution constraint of a frequency swept pulse holds (the energy separation of doublet levels should be much larger than the pulse bandwidth). We further demonstrate that the spectral resolution of selective population transfer can be enhanced significantly by using pump pulse pair and Stokes pulse due to temporal quantum interference between the sequential transitions in the time domain, which can also be well followed as a result of the frequency-domain formation of a comblike structure of the pulse pair spectrum. The proposals take into account the case of population transfer in realistic atomic and molecular systems, and may have applications in quantum coherent control of systems with equally populated initial manifolds.
Abstract High-fidelity entangled-state generation in driven two-atom systems is often optimized at a nominal transition frequency, which can produce control pulses that are fragile against detuning errors and experimental imperfections. To address this limitation, we develop a sampled-detuning quantum optimal-control approach in which different detuning values are treated as control scenarios driven by a common laser field. Time-domain equality constraints, including zero pulse area and fixed fluence, are incorporated directly into the pulse update. The resulting constraint-projected update provides a common ascent direction for the sampled detuning objectives while preserving the imposed pulse constraints. Numerical simulations show that the optimized robust pulses maintain a high target-state population over a wider detuning interval than resonant Gaussian pulses and conventional single-objective optimal pulses. The results further reveal a fluence-bandwidth trade-off for robust plateau formation. Frequency-domain analysis indicates that the enhanced robustness is associated with optimized off-resonant spectral components, and the robustness window can be tuned by selecting the sampled-detuning training range.
The stimulated Raman adiabatic passage shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity in three-level quantum systems based on adiabatic evolution. This technique has widely theoretical and experimental applications in many fields of physics, chemistry, and beyond. Here, we present a general approach to robust stimulated Raman shortcut-to-adiabatic passage with invariant-based optimal control. By controlling the dynamical process, we inversely design a family of Hamiltonians with non-divergent Rabi frequencies that can realize fast and accurate population transfer from the first to the third level, while the systematic errors are largely suppressed in general. Furthermore, a detailed trade-off relation between the population of the intermediate state and the amplitudes of Rabi frequencies in the transfer process is illustrated. These results provide an optimal route toward manipulating the evolution of three-level quantum systems in future quantum information processing.
We study the potential for optimal control of a symmetric double quantum-dot structure interacting with a single pulsed electromagnetic field. We first use the rotating wave and resonant approximations and reduce the dynamics of the system to that of a degenerate three-level $\ensuremath{\Lambda}$-type system. We also formulate the optimal control problem in terms of differential equations that have to be fulfilled by the optimal electromagnetic fields. We then obtain general analytical expressions for the optimal pulse shapes that lead to global maximization of the final population of the target state and of the time-averaged population of the target state in the quantum-dot structure.