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Frontiers in Physics

Fabrication and quantum sensing of spin defects in silicon carbide

Qin‐Yue Luo, Qiang Li, Junfeng Wang, Pei‐Jie Guo, Wu-Xi Lin, Shuang Zhao, Qi‐Cheng Hu, Ziqi Zhu, Jin‐Shi Xu, Chuan‐Feng Li, Guang‐Can Guo

Published Sep 26, 2023• 30 citations
Publisher

Abstract

In the past decade, color centers in silicon carbide (SiC) have emerged as promising platforms for various quantum information technologies. There are three main types of color centers in SiC: silicon-vacancy centers, divacancy centers, and nitrogen-vacancy centers. Their spin states can be polarized by laser and controlled by microwave. These spin defects have been applied in quantum photonics, quantum information processing, quantum networks, and quantum sensing. In this review, we first provide a brief overview of the progress in single-color center fabrications for the three types of spin defects, which form the foundation of color center-based quantum technology. We then discuss the achievements in various quantum sensing, such as magnetic field, electric field, temperature, strain, and pressure. Finally, we summarize the current state of fabrications and quantum sensing of spin defects in SiC and provide an outlook for future developments.

DOI
10.3389/fphy.2023.1270602

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In the past decade, color centers in silicon carbide (SiC) have emerged as promising platforms for various quantum information technologies. There are three main types of color centers in SiC: silicon-vacancy centers, divacancy centers, and nitrogen-vacancy centers. Their spin states can be polarized by laser and controlled by microwave. These spin defects have been applied in quantum photonics, quantum information processing, quantum networks, and quantum sensing. In this review, we first provide a brief overview of the progress in single-color center fabrications for the three types of spin defects, which form the foundation of color center-based quantum technology. We then discuss the achievements in various quantum sensing, such as magnetic field, electric field, temperature, strain, and pressure. Finally, we summarize the current state of fabrications and quantum sensing of spin defects in SiC and provide an outlook for future developments.
Solid-state color-center spin defects provide a versatile platform for quantum sensing with applications ranging from nanoscale magnetometry to thermometry and electrometry. This review surveys recent progress in nitrogen-vacancy centers in diamond and defect spins in silicon carbide (SiC), with emphasis on their material properties, fabrication strategies, and coherence engineering. Key defect creation and optimization techniques, including ion implantation, femtosecond laser writing, focused ion beam nanofabrication, isotopic engineering, and surface passivation, are discussed in the context of improving spin coherence and optical performance. Fundamental quantum measurement protocols, optically detected magnetic resonance, Rabi oscillations, Ramsey interferometry, and spin echo, are reviewed as a hierarchical framework for characterizing spin control, dephasing, and intrinsic coherence. The review further highlights microscale sensing architectures and examines the growing role of machine learning in pulse optimization, adaptive estimation, and data-driven imaging. Finally, current challenges and future directions are outlined, focusing on scalability, environmental robustness, and autonomous operation. Together, these developments position diamond and SiC color centers as leading platforms for next-generation solid-state quantum sensors.
Deep-level defects are usually considered undesirable in semiconductors as they typically interfere with the performance of present-day electronic and optoelectronic devices. However, the electronic spin states of certain atomic-scale defects have recently been shown to be promising quantum bits for quantum information processing as well as exquisite nanoscale sensors due to their local environmental sensitivity. In this review, we will discuss recent advances in quantum control protocols of several of these spin defects, the negatively charged nitrogen-vacancy (NV-) center in diamond and a variety of forms of the neutral divacancy (VV0) complex in silicon carbide (SiC). These defects exhibit a spin-triplet ground state that can be controlled through a variety of techniques, several of which allow for room temperature operation. Microwave control has enabled sophisticated decoupling schemes to extend coherence times as well as nanoscale sensing of temperature along with magnetic and electric fields. On the other hand, photonic control of these spin states has provided initial steps toward integration into quantum networks, including entanglement, quantum state teleportation, and all-optical control. Electrical and mechanical control also suggest pathways to develop quantum transducers and quantum hybrid systems. The versatility of the control mechanisms demonstrated should facilitate the development of quantum technologies based on these spin defects.
This review provides an overview of defects in silicon carbide (SiC) with potential applications as quantum qubits. It begins with a brief introduction to quantum qubits and existing qubit platforms, outlining the essential criteria a defect must meet to function as a viable qubit. The focus then shifts to the most promising defects in SiC, notably the silicon vacancy (VSi) and divacancy (VC-VSi). A key challenge in utilizing these defects for quantum applications is their precise and controllable creation. Various fabrication techniques, including irradiation, ion implantation, femtosecond laser processing, and focused ion beam methods, have been explored to create these defects. Designed as a beginner-friendly resource, this review aims to support early-career experimental researchers entering the field of SiC-related quantum qubits. Providing an introduction to defect-based qubits in SiC offers valuable insights into fabrication strategies, recent progress, and the challenges that lie ahead.
Point defects in diamond, particularly nitrogen-vacancy (NV) centers, have emerged as powerful tools for a broad range of quantum technologies. These defects are promising candidates for quantum information science, serving as deterministic single-photon sources and solid-state quantum memories. They have also been employed as nanoscale quantum sensors to detect various physical quantities, including magnetic fields, electric fields, and temperature, owing to their long spin coherence time at room temperature. Development of these diamond-based quantum technologies has been rapidly boosted by a recent quantum leap in nanofabrication technologies for high-quality single-crystal diamond. Incorporating these color centers into diamond nanostructures with mature integrated photonics provides a promising route to build scalable and practical systems for quantum applications. This review discusses recent progress and challenges in the hybrid integration of diamond color centers on cutting-edge photonic platforms. Nitrogen-vacancy centers in diamond have emerged as powerful tools for a broad range of quantum technologies. This review discusses recent progress and challenges in the hybrid integration of diamond color centers on cutting-edge photonic platforms.
Engineering the photonic interface with spins in color centers, such as the $N\phantom{\rule{0}{0ex}}V$ center in diamond or the neutral divacancy in silicon carbide, is crucial for applications in quantum communication and precision sensing. Exploiting SiC's compatibility with conventional thin-film fabrication, the authors use on-chip nanoscale photonic crystal cavities to dramatically enhance the measurement of the spin and optical properties of color-center ensembles. These results bring us a step closer to realizing scaled-up defect-based quantum technologies.
Abstract Color centers in diamond, silicon carbide, and related materials have recently emerged as one of the most promising platforms for quantum technology applications. These optically active point defects in the crystal lattice demonstrate outstanding optical and spin properties at room and even higher temperatures, which can hardly be achieved using other quantum systems. For a long time, the host material was considered only as a mechanical carrier of color centers, and the fact that it is a semiconductor and, therefore, can contain high densities of electrons and holes, was ignored. However, recent studies have demonstrated that color centers can exchange electrons and holes with the valence or conduction bands of the host material, which enables novel functionalities, ranging from ultrabright electrically driven single‐photon sources to protected quantum memories. This review summarizes recent advances in understanding this interaction.