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The Journal of Chemical Physics

Publisher’s Note: “Theory of entangled two-photon emission/absorption [E2P-EA] between molecules” [J. Chem. Phys. 159, 074103 (2023)]

Tse-Min Chiang, George Chappell Schatz

Published Sep 22, 2023• 0 citations
Publisher

Abstract

This is a correction to: Theory of entangled two-photon emission/absorption [E2P-EA] between molecules
DOI
10.1063/5.0175173

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Theory of entangled two-photon emission/absorption [E2P-EA] between molecules

Tse-Min Chiang, George Chappell Schatz

This paper presents a comprehensive study of the theory of entangled two-photon emission/absorption (E2P-EA) between a many-level cascade donor and a many-level acceptor (which could be quantum dots or molecules) using second-order perturbation theory and where the donor-acceptor pair is in a homogeneous but dispersive medium. To understand the mechanism of E2P-EA, we analyze how dipole orientation, radiative lifetime, energy detuning between intermediate states, separation distance, and entanglement time impact the E2P-EA rate. Our study shows that there are quantum interference effects in the E2P-EA rate expression that lead to oscillations in the rate as a function of entanglement time. Furthermore, we find that the E2P-EA rate for a representative system consisting of two quantum dots can be comparable to one-photon emission/absorption (OP-EA) when donor and acceptor are within a few nm. However, the E2P-EA rate falls off much more quickly with separation distance than does OP-EA.

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On the enhancement of the back-to-back two-electron-one photon ionization in molecules

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Quantum Entanglement in Photon-Induced Electron Spectroscopy of Atoms and Molecules

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This paper presents a comprehensive study of the theory of entangled two-photon emission/absorption (E2P-EA) between a many-level cascade donor and a many-level acceptor (which could be quantum dots or molecules) using second-order perturbation theory and where the donor-acceptor pair is in a homogeneous but dispersive medium. To understand the mechanism of E2P-EA, we analyze how dipole orientation, radiative lifetime, energy detuning between intermediate states, separation distance, and entanglement time impact the E2P-EA rate. Our study shows that there are quantum interference effects in the E2P-EA rate expression that lead to oscillations in the rate as a function of entanglement time. Furthermore, we find that the E2P-EA rate for a representative system consisting of two quantum dots can be comparable to one-photon emission/absorption (OP-EA) when donor and acceptor are within a few nm. However, the E2P-EA rate falls off much more quickly with separation distance than does OP-EA.