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Physical Review A

Extreme violation of the Leggett-Garg inequality in nonunitary dynamics with complex energies

Anant Vijay Varma, Jacob Muldoon, Sourav Paul, Yogesh N. Joglekar, Sourin Das

Published Sep 5, 2023• 9 citations
Publisher

Abstract

We study the Leggett-Garg inequality (LGI) of a two-level system (TLS) undergoing coherent dynamics described by a non-Hermitian Hamiltonian and Lindblad equation with no quantum jumps. The nonlinear Bloch equation for the TLS density matrix predicts violations of LGI above the TLS L\"uders bound of $3/2$, approaching the extremal case of LGI parameter ${K}_{3}=3$ in the $\mathcal{PT}$-symmetric region and the $\mathcal{PT}$-broken region. We show that these findings are reproduced by using postselection to remove instantaneous quantum jumps from a three-level system described by the Lindblad equation with a single spontaneous emission dissipator. We trace the ${K}_{3}$ excesses beyond the standard quantum limit of $3/2$ to a nonuniform speed of evolution on the Bloch sphere. Finally, we consider the effects of competing Lindblad dissipators on the postselected non-Hermitian dynamics and the viability of observing ${K}_{3}$ exceeding the L\"uder bound and approaching its algebraic maximum of three in current experimental setups.

DOI
10.1103/physreva.108.032202

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We study the Leggett-Garg inequality (LGI) of a two-level system (TLS) undergoing coherent dynamics described by a non-Hermitian Hamiltonian and Lindblad equation with no quantum jumps. The nonlinear Bloch equation for the TLS density matrix predicts violations of LGI above the TLS L"uders bound of 3/23/23/2, approaching the extremal case of LGI parameter K3=3{K}_{3}=3K3​=3 in the PT\mathcal{PT}PT-symmetric region and the PT\mathcal{PT}PT-broken region. We show that these findings are reproduced by using postselection to remove instantaneous quantum jumps from a three-level system described by the Lindblad equation with a single spontaneous emission dissipator. We trace the K3{K}_{3}K3​ excesses beyond the standard quantum limit of 3/23/23/2 to a nonuniform speed of evolution on the Bloch sphere. Finally, we consider the effects of competing Lindblad dissipators on the postselected non-Hermitian dynamics and the viability of observing K3{K}_{3}K3​ exceeding the L"uder bound and approaching its algebraic maximum of three in current experimental setups.
We study Leggett-Garg inequality (LGI) of a two level system (TLS) undergoing non-Hermitian dynamics governed by a non-linear Bloch equation (derived in J. Phys. A: Math. Theor. 54, 115301 (2021)) across a PT-transition. We present an algebraic identification of the parameter space for the maximum violation of LGI (in particular K3K_{3}K3​). In the PT-symmetric regime the maximum allowed value for K3K_{3}K3​ is always found to be greater than the quantum bound (Lüders bound) of 3/23/23/2 but it does not reach the algebraic maximum of K3=3K_{3}=3K3​=3 in general. However, in the limit where PT-symmetry breaking parameter approaches the exceptional point from the PT-symmetric side, K3K_{3}K3​ is found to asymptotically approach its algebraic maximum of 3. In contrast, the maximum value of K3K_{3}K3​ always reaches its algebraic maximum in the PT-broken phase i.e.i.e.i.e. K3→3K_{3}\rightarrow 3K3​→3. We find that (i) the speed of evolution (SOE) must reach its maximum value (in the parameter space of initial state and the time interval between successive measurements) to facilitate the value of K3→3K_{3} \rightarrow 3K3​→3, (ii) together with the constraint that its minimum value must run into SOE equals to zero during the evolution of the state. In fact we show that the minimum speed of evolution can serve as an order parameter which is finite on the PT-symmetric side and identically zero on the PT-broken side. Finally, we discuss a possible experimental realization of this dynamics by quantum measurement followed by post-selection procedure in a three level atom coupled to cavity mode undergoing a Lindbladian dynamics.
Violations of the Leggett-Garg inequality (LGI) up to its algebraic bound under non-Hermitian dynamics are well established theoretically. Here, we demonstrate that such extreme violations are intrinsically fragile when realistic measurement processes are taken into account. We consider an open two-level system described by a time-local hybrid Liouvillian, with a continuous parameter q∈[0,1]q \in [0,1]q∈[0,1], representing detector efficiency, i.e., the fraction of quantum jump trajectories that are retained in the ensemble. This parameter interpolates between trace-preserving Lindblad dynamics (q=1q=1q=1) and non-Hermitian ``no-jump" evolution (q=0q=0q=0). While K3K_3K3​ approaches its algebraic maximum of 3 in the null-efficiency limit, even an infinitesimal increase in detector efficiency induces a rapid, highly nonlinear suppression toward the classical bound. This logarithmic sensitivity reveals that maximal LGI violations are not robust physical features but rather singular limits of idealized measurement conditions. Our results have direct experimental implications: achieving algebraic LGI violations in systems undergoing continuous time evolution requires near-perfect suppression of detected quantum jumps (i.e., effective post-selection), placing stringent constraints on detector performance. In contrast to discrete protocols based on time-non-divisible dynamics, our framework shows that extreme violations arising within continuous, divisible quantum trajectory evolution constitute a fundamentally fragile regime.
Abstract We study the dynamics of a non-Hermitian PT- symmetric Hamiltonian of a two level system (TLS) which has real eigenvalues. Within the framework of Hermitian quantum mechanics, it is known that maximal violation of Leggett–Garg inequality (LGI) is bounded by K 3 = 3/2 (Luder’s bound). We show that this absolute bound can be evaded when dynamics is governed by non-Hermitian PT- symmetric Hamiltonians with real eigenvalues. Moreover, the extent of violation can be optimized to asymptotically approach the algebraic maximum of K 3 max = 3 , which is otherwise observed for Hermitian Hamiltonian with infinite dimensional Hilbert space. The extreme violation of LGI is shown to be directly related to the two basic ingredients: (i) the Bloch equation for the TLS having a non-linear terms which allow for accelerated dynamics of states on the Bloch sphere exceeding all known quantum speed limits of state evolution; and (ii) quantum trajectory of states lie on a great circle (geodesic path) on the Bloch sphere at all times. We demonstrate that such extreme temporal correlation of TLS can be simulated in realistic system by embedding the TLS into a higher dimensional Hilbert space such that the composite system obeys unitary dynamics. Specifically we show that a four dimensional embedding of non-Hermitian PT- symmetric TLS is enough to host K 3 → 3 limit. We also discuss the effect of random noise on our results. Finally we conclude with a comparative study of our results with existing experimental realization of embedding.
The Leggett-Garg inequality (LGI) delineates a boundary between quantum and classical systems. While the temporal quantum correlations represented by LGIs have been extensively investigated in the Hermitian domain, the exploration of LGIs under non-Hermitian conditions remains scarce. Theoretical conjectures posit that nonunitary dynamics could transcend the boundary of LGIs set by Hermitian quantum mechanics, yet its empirical validation is lacking. Here, we demonstrate the enhanced violation of LGIs in a non-Hermitian system of a parity-time (PT\mathcal{PT}PT)-symmetric trapped-ion qubit. The upper bounds of both the third-order parameter K3{K}_{3}K3​ and fourth-order parameter K4{K}_{4}K4​ increase with dissipation and can reach the maximum value when the system approaches the exceptional point, where ${K}_{3}={C}_{21}+{C}_{32}\ensuremath{-}{C}_{31}$ is comprising three two-time correlations and ${K}_{4}={C}_{21}+{C}_{32}+{C}_{43}\ensuremath{-}{C}_{41}$ is comprising four correlations. We also find that the lower bounds of K3{K}_{3}K3​ and K4{K}_{4}K4​ exhibit distinctive behaviors, where the lower bound of K3{K}_{3}K3​ remains constant, but that of K4{K}_{4}K4​ depends on the target states and measurement operators. These findings reveal a pronounced correlation between the dissipative nature of a quantum system and its temporal correlations.
Quantum theory provides rules governing much of the microscopic world, and among its counter-intuitive consequences are correlations that exceed the bounds from local, classical theories. In two-level quantum systems - qubits - unitary dynamics theoretically limit these spatiotemporal quantum correlations, called Bell/Clauser-Horn-Shimony-Holt or Leggett-Garg inequalities, to 222\sqrt{2}22​ or 1.5 respectively. Experiments with state-of-the-art qubits have approached the spatial, Bell and temporal, Leggett-Garg quantum correlation bounds. Here, using a dissipative, trapped 40^{40}40Ca+^++ ion governed by a two-level, non-Hermitian Hamiltonian, we observe temporal correlation values up to 1.703(4) for the Leggett-Garg parameter K3K_3K3​, clearly exceeding the hitherto inviolable Lüder's bound of 1.5. These excesses occur across the exceptional point of the parity-time symmetric Hamiltonian responsible for the qubit's non-unitary, coherent dynamics. Distinct evolution speeds for antipodal qubit states, which violate the unified (Mendelstam-Tamm or Margolus-Levitin) bound τQSLτ_{\textrm{QSL}}τQSL​ for the transit time based on quantum speed limit, result in the super-quantum K3K_3K3​ values observed over a wide parameter range. Our results demonstrate that post-selected, coherent dynamics of non-Hermitian Hamiltonians pave the way for enhanced quantum correlations that exceed protocols based on unitary or dissipative dynamics.
The Leggett-Garg inequality (LGI) is a powerful tool for distinguishing between quantum and classical properties in studies of macroscopic systems. Applying the LGI to non-Hermitian systems with dissipation presents a fascinating opportunity, as competing mechanisms can either strengthen or weaken LGI violations. On one hand, dissipation-induced nonlinear interactions amplify LGI violations compared to Hermitian systems; on the other hand, dissipation leads to decoherence, which could weaken the LGI violation. In this paper, we investigate a non-Hermitian system of ultracold Fermi gas with dissipation. Our experiments reveal that as dissipation increases, the upper bound of the third-order LGI parameter K 3 initially rises, reaching its maximum at the exceptional point, where K 3 = C 21 + C 32 − C 31 , encompassing three two-time correlation functions. Beyond a certain dissipation threshold, the LGI violation weakens, approaching the classical limit, indicating a quantum-to-classical transition (QCT). Furthermore, we observe that the LGI violation decreases with increasing evolution time, reinforcing the QCT in the time domain. This study provides a crucial stepping stone for using the LGI to explore the QCT in many-body open quantum systems.