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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Quantum Engineering of Light with an Intracavity Rydberg Superatom

Valentin Magro, Julien Vaneecloo, Sébastien Garcia, Alexei Ourjoumtsev

Published Jun 26, 2023• 0 citations
Publisher

Abstract

Engineering quantum states of free-propagating light is of paramount importance for quantum technologies. Coherent states ubiquitous in classical and quantum communications, squeezed states used in quantum sensing, and even highly-entangled cluster states studied in the context of quantum computing can be produced deterministically, but they obey quasi-classical optical field statistics described by Gaussian, positive Wigner functions. Fully harnessing the potential of many quantum engineering protocols requires using Wigner-negative states, so far produced using intrinsically probabilistic methods. We achieved the first fully deterministic preparation of Wigner-negative free-propagating states of light by mapping the internal state of an intracavity Rydberg superatom onto an optical qubit encoded as a superposition of 0 and 1 photons [1]. This approach allows us to reach a 60% photon generation efficiency in a well-controlled spatio-temporal mode, while maintaining a strong photon antibunching. By changing the qubit rotation angle, we observe an evolution from quadrature squeezing to Wigner negativity. Our experiment sets this new technique as a viable method to deterministically generate highly non-classical photonic resources, lifting several major roadblocks in optical quantum engineering.

DOI
10.1109/cleo/europe-eqec57999.2023.10231476

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Engineering quantum states of free-propagating light is of paramount importance for quantum technologies. Coherent states ubiquitous in classical and quantum communications, squeezed states used in quantum sensing, and even highly-entangled cluster states studied in the context of quantum computing can be produced deterministically, but they obey quasi-classical optical field statistics described by Gaussian, positive Wigner functions. Fully harnessing the potential of many quantum engineering protocols requires using Wigner-negative states, so far produced using intrinsically probabilistic methods. We achieved the first fully deterministic preparation of Wigner-negative free-propagating states of light by mapping the internal state of an intracavity Rydberg superatom onto an optical qubit encoded as a superposition of 0 and 1 photons [1]. This approach allows us to reach a 60% photon generation efficiency in a well-controlled spatio-temporal mode, while maintaining a strong photon antibunching. By changing the qubit rotation angle, we observe an evolution from quadrature squeezing to Wigner negativity. Our experiment sets this new technique as a viable method to deterministically generate highly non-classical photonic resources, lifting several major roadblocks in optical quantum engineering.
We demonstrate a new approach for creating deterministic photon-photon interactions for optical quantum engineering, based on a single-ended medium-finesse optical cavity containing a mesoscopic atomic ensemble. This ensemble is made transparent by a laser beam mapping intracavity photons into Rydberg polaritons. The transparency vanishes when the cloud, acting as a single collective two-level "superatom" with an enhanced coupling to light, is driven from the ground to a Rydberg state. We observe collectively-enhanced Rabi oscillations between these states, optically discriminate them in a single shot with a 95% effciency, and show that a change between the two internal states of the superatom induces a π phase rotation on the light reflected off of the cavity. These ingredients form a complete set of tools for implementing deterministic photonic entangling gates and for generating highly non-classical light without the need for a low-volume high-finesse cavity.
Wigner-negative states of light are key resources for quantum advantage in continuous-variable optical quantum computing. They can be produced probabilistically via frequency conversion and photon detection, or deterministically by exploiting the single-photon nonlinearity of a quantum emitter. Here, we generate such Wigner-negative states of light with a tunable negativity using a single semiconductor quantum dot in a cavity. Optical coherent control of the quantum-dot transition allows to generate a quantum superposition of zero and one photon. The generated quantum states are characterized point-by-point in the phase space through homodyne measurement. The emergence of Wigner-function negativity is observed as the excitation power is increased. After correcting for collection and propagation losses, we obtain fidelities to the ideal state and quantum purities above 95%, together with near-optimal quadrature squeezing. The ability to generate a wide variety of Wigner-negative states with mature semiconductor technology opens promising opportunities for continuous-variable optical quantum technologies.
We demonstrate a new versatile building block for optical quantum technologies, enabling deterministic quantum engineering of light by combining the advantages of two complementary approaches: cavity quantum electrodynamics and interacting atomic ensembles.Our system is based on an intracavity Rydberg-blockaded atomic ensemble acting as a single two-level superatom.We coherently control its state and optically detect it in a single shot with 95% efficiency.Crucially, we demonstrate a superatom-statedependent π phase rotation on the light reflected from the cavity.Together with the state manipulation and detection, it is a key ingredient for implementing deterministic photonic entangling gates and for generating highly nonclassical light states.
Pulsed coherent and squeezed driving of a spin-SSS emitter as a deterministic source of Wigner-negative light
Generating propagating Wigner-negative states of light is an important and difficult task for many quantum technologies. Historically, the proposed methods of creating such states have been intrinsically probabilistic, relying on conditional measurements or photon heralding. More recently, methods have been proposed involving the steady-state driving of two-level emitters, where Wigner-negative temporal modes are present in the outgoing field. We theoretically demonstrate through the simulation of a cascaded-systems model that this approach can be improved significantly with pulsed coherent or squeezed driving of a spin-1/2 emitter. This enables the deterministic generation of strongly Wigner-negative states, using only driving-source states with positive Gaussian Wigner distributions. This method is extended to the driving of a spin-SSS emitter with S≥1S\geq 1S≥1 to generate still more exotic, highly non-classical states. The array of states demonstrated in this work includes close approximations to displaced N-photon states, squeezed Schrödinger cat states, and finite-energy Gottesman-Kitaev-Preskill (GKP) states.
Engineering non-classical states of the electromagnetic field is a central quest for quantum optics1,2. Beyond their fundamental significance, such states are indeed the resources for implementing various protocols, ranging from enhanced metrology to quantum communication and computing. A variety of devices can be used to generate non-classical states, such as single emitters, light-matter interfaces or non-linear systems3. We focus here on the use of a continuous-wave optical parametric oscillator3,4. This system is based on a non-linear χ2 crystal inserted inside an optical cavity and it is now well-known as a very efficient source of non-classical light, such as single-mode or two-mode squeezed vacuum depending on the crystal phase matching. Squeezed vacuum is a Gaussian state as its quadrature distributions follow a Gaussian statistics. However, it has been shown that number of protocols require non-Gaussian states5. Generating directly such states is a difficult task and would require strong χ3 non-linearities. Another procedure, probabilistic but heralded, consists in using a measurement-induced non-linearity via a conditional preparation technique operated on Gaussian states. Here, we detail this generation protocol for two non-Gaussian states, the single-photon state and a superposition of coherent states, using two differently phase-matched parametric oscillators as primary resources. This technique enables achievement of a high fidelity with the targeted state and generation of the state in a well-controlled spatiotemporal mode.
Engineering non-classical states of the electromagnetic field is a central quest for quantum optics(1,2). Beyond their fundamental significance, such states are indeed the resources for implementing various protocols, ranging from enhanced metrology to quantum communication and computing. A variety of devices can be used to generate non-classical states, such as single emitters, light-matter interfaces or non-linear systems(3). We focus here on the use of a continuous-wave optical parametric oscillator(3,4). This system is based on a non-linear χ(2) crystal inserted inside an optical cavity and it is now well-known as a very efficient source of non-classical light, such as single-mode or two-mode squeezed vacuum depending on the crystal phase matching. Squeezed vacuum is a Gaussian state as its quadrature distributions follow a Gaussian statistics. However, it has been shown that number of protocols require non-Gaussian states(5). Generating directly such states is a difficult task and would require strong χ(3) non-linearities. Another procedure, probabilistic but heralded, consists in using a measurement-induced non-linearity via a conditional preparation technique operated on Gaussian states. Here, we detail this generation protocol for two non-Gaussian states, the single-photon state and a superposition of coherent states, using two differently phase-matched parametric oscillators as primary resources. This technique enables achievement of a high fidelity with the targeted state and generation of the state in a well-controlled spatiotemporal mode.