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Nature

Emergent ferromagnetic states revealed in a geometrically frustrated triangular lattice

Published Aug 2, 2023• 0 citations
Publisher
DOI
10.1038/d41586-023-02387-x

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Understanding ferromagnetism mechanism in doped Mott insulators on frustrated lattices remains challenging at intermediate coupling and finite doping. Here, we study the itinerant ferromagnetism and propose its mechanism in doped Mott insulators on a geometrically frustrated triangular lattice. Using large-scale density matrix renormalization group (DMRG) and unrestricted Hartree–Fock mean-field methods, we reveal that itinerant ferromagnetism appears at intermediate coupling (10 ≲ U ≪ ∞) near 50% electron doping in the triangular-lattice Hubbard model. By analyzing all microscopic hopping processes, we find that doublon-singlon exchange alone drives the fully polarized ferromagnetism and uncovers the particle-hole asymmetry. We also establish the magnetic phase diagram and compare local spin correlations with recent experiments. Random phase approximation and DMRG calculations consistently confirm that the ferromagnetism persists when SU(2) symmetry is explicitly broken by magnetic anisotropy. These results clarify a microscopic route to itinerant ferromagnetism at intermediate coupling and finite doping in doped Mott insulators. Understanding the mechanism of ferromagnetism in strongly correlated systems is an ongoing theoretical challenge and the Hubbard model is typically adopted to investigate such systems. Here, the authors numerically investigate the doped triangular Fermi-Hubbard model and show ferromagnetism at intermediate coupling and finite doping, which results from the interplay of kinetic doublon-singlon exchange and lattice geometry.

arXiv:2408.05971•Communications Physics•Oct 10, 2025•1 citation
We consider a frustrated anti-ferromagnetic triangular lattice Hamiltonian and show that the properties of the manifold of its degenerated ground state are represented by a novel type of tensor networks. These tensor networks are not based on ancillary maximally entangled pairs, but rather on triangular W-like simplices. Anti-ferromagnetic triangular frustration is then related to ancillary W-states in contrast to ferromagnetic order which emerges from the contraction of GHZ-like triangular simplices. We further discuss the outwards entangling power of various simplices. This analysis suggests the emergence of distinct macroscopic types of order from the classification of entanglement residing on the simplices that define a tensor network.
We study the hard-core Fermi-Hubbard model in the crossover between square and triangular lattices near half-filling. As was recognized by Nagaoka in the 1960s, on the square lattice the presence of a single hole leads to ferromagnetic spin ordering. On the triangular lattice, geometric frustration instead leads to a spin-singlet ground state, which can be associated with a 120-degree spiral order. On lattices which interpolate between square and triangular, there is a phase transition at which the ferromagnetic order becomes unstable to a spin spiral. We model this transition, finding the exact location of the spin-spiral instability.
Understanding ferromagnetism mechanism in doped Mott insulators on frustrated lattices remains challenging at intermediate coupling and finite doping. Here, we study the itinerant ferromagnetism and propose its mechanism in doped Mott insulators on a geometrically frustrated triangular lattice. Using large-scale density matrix renormalization group (DMRG) and unrestricted Hartree–Fock mean-field methods, we reveal that itinerant ferromagnetism appears at intermediate coupling (10 ≲ U ≪ ∞) near 50% electron doping in the triangular-lattice Hubbard model. By analyzing all microscopic hopping processes, we find that doublon-singlon exchange alone drives the fully polarized ferromagnetism and uncovers the particle-hole asymmetry. We also establish the magnetic phase diagram and compare local spin correlations with recent experiments. Random phase approximation and DMRG calculations consistently confirm that the ferromagnetism persists when SU(2) symmetry is explicitly broken by magnetic anisotropy. These results clarify a microscopic route to itinerant ferromagnetism at intermediate coupling and finite doping in doped Mott insulators. Understanding the mechanism of ferromagnetism in strongly correlated systems is an ongoing theoretical challenge and the Hubbard model is typically adopted to investigate such systems. Here, the authors numerically investigate the doped triangular Fermi-Hubbard model and show ferromagnetism at intermediate coupling and finite doping, which results from the interplay of kinetic doublon-singlon exchange and lattice geometry.